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arXiv:1210.1150 · Physical Review Letters

Experimental Characterization of Bosonic Creation and Annihilation Operators

Rupesh Kumar, E. Barrios, Connor Kupchak, Alexander I. Lvovsky

Published Mar 25, 2013• 58 citations
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Abstract

The photon creation and annihilation operators are cornerstones of the quantum description of the electromagnetic field. They signify the isomorphism of the optical Hilbert space to that of the harmonic oscillator and the bosonic nature of photons. We perform complete experimental characterization (quantum process tomography) of these operators. By measuring their effect on coherent states by means of homodyne tomography, we obtain their process tensor in the Fock basis, which explicitly shows the "raising" and "lowering" properties of these operators with respect to photon number states. This is the first experimental demonstration of complete tomography of nondeterministic quantum processes.

DOI
10.1103/physrevlett.110.130403

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The photon creation and annihilation operators are cornerstones of the quantum description of the electromagnetic field. They signify the isomorphism of the optical Hilbert space to that of the harmonic oscillator and the bosonic nature of photons. We perform complete experimental characterization (quantum process tomography) of these operators. By measuring their effect on coherent states by means of homodyne tomography, we obtain their process tensor in the Fock basis, which explicitly shows the "raising" and "lowering" properties of these operators with respect to photon number states. This is the first experimental demonstration of complete tomography of nondeterministic quantum processes.
The recent development of experimental techniques to implement the creation and the annihilation operators in the optical domain has found great interest for quantum information manipulation and processing. Quantum states of light obtained by the application of alternated sequences of the creation and annihilation operators a^†\hat{a}^\daggera^† and a^\hat{a}a^ to a thermal state of light depend on the order in which the two operations are performed. The non-commutativity of the bosonic operators, a^a^†≠a^†a^≠1\hat{a}\hat{a}^\dagger\ne \hat{a}^\dagger\hat{a}\ne 1a^a^†=a^†a^=1, has been experimentally verified in terms of density matrixes and Wigner functions, which are reconstructed by quantum homodyne tomography. Recently, a setup has been proposed to directly and completely prove the bosonic commutation relation where a single-photon interferometer is used to create coherent superpositions of two alternated sequences of operators, such as [a^a^†±a^†a^][\hat{a}\hat{a}^\dagger \pm \hat{a}^\dagger\hat{a}][a^a^†±a^†a^]. Some of the latest experimental results are discussed.
We report a technique for experimental characterization of an M -mode quantum optical process, generalizing the single-mode coherent-state quantum-process tomography method [ 1 , 2 ]. By measuring the effect of the process on multi-mode coherent states via balanced homodyne tomography, we obtain the process tensor in the Fock basis. This rank- tensor, which predicts the effect of the process on an arbitrary density matrix, is iteratively reconstructed directly from the experimental data via the maximum-likelihood method. We demonstrate the capabilities of our method using the example of a beam splitter, reconstructing its process tensor within the subspace spanned by the first three Fock states. In spite of using purely classical probe states, we recover quantum properties of this optical element, in particular the Hong–Ou–Mandel effect.
A new class of non-classical light states has been experimentally generated and their complete phase-space characterization has been achieved by quantum homodyne tomography. Such states are produced by the action of the photon creation operator on a coherent light field and are thus the result of the elementary excitation process of a classical field by a single quantum. Being intermediate between a single-photon Fock state and a coherent one, they offer the unique opportunity to closely follow the smooth evolution between the particle-like and the wave-like behavior of the light field.
Conditional quantum optical processes enable a wide range of technologies from generation of highly non-classical states to implementation of quantum logic operations. The process fidelity that can be achieved in a realistic implementation depends on a number of system parameters. Here we experimentally examine Fock state filtration, a canonical example of a broad class of conditional quantum operations acting on a single optical field mode. This operation is based upon interference of the mode to be manipulated with an auxiliary single-photon state at a beam splitter, resulting in the entanglement of the two output modes. A conditional projective measurement onto a single photon state at one output mode heralds the success of the process. This operation, which implements a measurement-induced nonlinearity, is capable of suppressing particular photon-number probability amplitudes of an arbitrary quantum state. We employ coherent-state process tomography to determine the precise operation realized in our experiment, which is mathematically represented by a process tensor. To identify the key sources of experimental imperfection, we develop a realistic model of the process and identify three main contributions that significantly hamper its efficacy. The experimentally reconstructed process tensor is compared with the model, yielding a fidelity better than 0.95. This enables us to identify three key challenges to overcome in realizing a filter with optimal performance—namely the single-photon nature of the auxiliary state, high mode overlap of the optical fields involved, and the need for photon-number-resolving detection when heralding. The results show that the filter does indeed exhibit a non-linear response as a function of input photon number and preserves the phase relation between Fock layers of the output state, providing promise for future applications.
This thesis introduces and implements a characterization procedure called coherent state quantum process tomography and applies it to a selection of quantum operations. The procedure holds advantages over previous quantum process tomography methods, a pri- mary one is that a process can be characterized by measuring its effect on a set of coherent states which are readily available from a laser source. After introduction of the characterization procedure, the method is tested on a simple process of an electro-optical modulator and polarizing beam splitter. The accuracy of the characterization is verified by comparison of the predicted action of the reconstructed process tensor versus the actual experiment involving a squeezed vacuum state. The algorithm is then implemented and verified on a quantum memory system based on electromagnetically induced transparency, a system that was previously shown capable of storing a squeezed vacuum state. Lastly, a new optical storage system based on a gradient echo memory scheme is con- structed and optimized to achieve memory retrieval efficiencies of >80%. To characterize this system, a modified coherent state quantum process tomography algorithm based on the method of maximum likelihood estimation is employed. Despite the high efficiency values, the presence of excess noise resulted in the degradation of the storage device per- formance to be below the benchmarks of a quantum memory system. This estimation algorithm is also successfully implemented on the non-deterministic processes of photon creation and annihilation.
Displaced Fock states of the electromagnetic field have been synthesized by overlapping the pulsed optical single-photon Fock state ∣1〉|1〉∣1〉 with coherent states on a high-reflection beam splitter and completely characterized by means of quantum homodyne tomography. The reconstruction reveals nonclassical properties of displaced Fock states, such as negativity of the Wigner function and photon number oscillations. To our knowledge, this is the first time complete tomographic reconstruction has been performed on a highly nonclassical optical state.