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arXiv:1210.0337 · Physical Review B

Unconventional quantum ordered and disordered states in the highly frustrated spin- 12 Ising-Heisenberg model on triangles-in-triangles lattices

Jana Čisárová, Jozef Strečka

Published Jan 29, 2013• 19 citations
arXivHTMLPDF

Abstract

The spin-$\frac{1}{2}$ Ising-Heisenberg model on two geometrically related triangles-in-triangles lattices is exactly solved through the generalized star-triangle transformation, which establishes a rigorous mapping correspondence with the effective spin-$\frac{1}{2}$ Ising model on a triangular lattice. Basic thermodynamic quantities were exactly calculated within this rigorous mapping method along with the ground-state and finite-temperature phase diagrams. Apart from the classical ferromagnetic phase, both investigated models exhibit several unconventional quantum ordered and disordered ground states. A mutual competition between two ferromagnetic interactions of basically different character generically leads to the emergence of a quantum ferromagnetic phase, in which a symmetric quantum superposition of three up-up-down states of the Heisenberg trimers accompanies a perfect alignment of all Ising spins. In the highly frustrated regime, we have either found the disordered quantum paramagnetic phase with a substantial residual entropy or a similar but spontaneously ordered phase with a nontrivial criticality at finite temperatures. The latter quantum ground state exhibits a striking coexistence of imperfect spontaneous order with partial disorder, which is evidenced by a quantum reduction of the spontaneous magnetization of Heisenberg spins that indirectly causes a small reduction of the spontaneous magnetization of otherwise classical Ising spins.

DOI
10.1103/physrevb.87.024421

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The spin-12\frac{1}{2}21​ Ising-Heisenberg model on two geometrically related triangles-in-triangles lattices is exactly solved through the generalized star-triangle transformation, which establishes a rigorous mapping correspondence with the effective spin-12\frac{1}{2}21​ Ising model on a triangular lattice. Basic thermodynamic quantities were exactly calculated within this rigorous mapping method along with the ground-state and finite-temperature phase diagrams. Apart from the classical ferromagnetic phase, both investigated models exhibit several unconventional quantum ordered and disordered ground states. A mutual competition between two ferromagnetic interactions of basically different character generically leads to the emergence of a quantum ferromagnetic phase, in which a symmetric quantum superposition of three up-up-down states of the Heisenberg trimers accompanies a perfect alignment of all Ising spins. In the highly frustrated regime, we have either found the disordered quantum paramagnetic phase with a substantial residual entropy or a similar but spontaneously ordered phase with a nontrivial criticality at finite temperatures. The latter quantum ground state exhibits a striking coexistence of imperfect spontaneous order with partial disorder, which is evidenced by a quantum reduction of the spontaneous magnetization of Heisenberg spins that indirectly causes a small reduction of the spontaneous magnetization of otherwise classical Ising spins.
The spin-1/2 Ising-Heisenberg model on martini and martini-diced lattices is exactly solved using a star-triangle transformation, which affords an exact mapping correspondence to an effective spin-1/2 Ising model on a triangular lattice. The ground-state phase diagram of both investigated quantum spin models display two spontaneously ordered ferromagnetic phases and one macroscopically degenerate disordered phase. In contrast to a classical ferromagnetic phase where the spontaneous magnetization of the Ising as well as Heisenberg spins acquire fully saturated values, the spontaneous magnetization of the Heisenberg spins is subject to a quantum reduction to one-third of its saturated value within a quantum ferromagnetic phase. The spontaneous magnetization and logarithmic divergence of the specific heat as the most essential features of both ferromagnetic phases disappear whenever the investigated quantum spin model is driven to the highly degenerate disordered phase. The disordered phase with nonzero residual entropy originates either from a geometric spin frustration caused by antiferromagnetic interactions or more strikingly it may also alternatively arise from a competition of the ferromagnetic Ising and Heisenberg interactions of easy-axis and easy-plane type, respectively. All three available ground states coexist together at a single triple point, around which anomalous magnetic and thermodynamic behavior can be detected.
The spin-1/2 Ising-Heisenberg model on martini and martini-diced lattice is exactly solved using a star-triangle transformation, which affords an exact mapping correspondence to an effective spin-1/2 Ising model on a triangular lattice. The ground-state phase diagram of both investigated quantum spin models display two spontaneously ordered ferromagnetic phases and one macroscopically degenerate disordered phase. In contrast to a classical ferromagnetic phase where the spontaneous magnetization of the Ising as well as Heisenberg spins acquire fully saturated values the spontaneous magnetization of the Heisenberg spins is subject to a quantum reduction to one-third of its saturated value within a quantum ferromagnetic phase. The spontaneous magnetization and logarithmic divergence of the specific heat as the most essential features of both ferromagnetic phases disappear whenever the investigated quantum spin model is driven to the highly degenerate disordered phase. The disordered phase with nonzero residual entropy originates either from a geometric spin frustration caused by antiferromagnetic interactions or more strikingly it may also alternatively arise from a competition of the ferromagnetic Ising and Heisenberg interactions of easy-axis and easy-plane type, respectively. All three available ground states coexist together at a single triple point, around which anomalous magnetic and thermodynamic behavior can be detected.
The geometrically frustrated spin-1/2 Ising-Heisenberg model on triangulated Husimi lattices is exactly solved by combining the generalized star-triangle transformation with the method of exact recursion relations. The ground-state and finite-temperature phase diagrams are rigorously calculated along with both sublattice magnetizations of the Ising and Heisenberg spins. It is evidenced that the Ising-Heisenberg model on triangulated Husimi lattices with two or three interconnected triangles-in-triangles units displays in a highly frustrated region a quantum disorder irrespective of temperature, whereas the same model on triangulated Husimi lattices with a greater connectivity of triangles-in-triangles units exhibits at low enough temperatures an outstanding quantum order due to the order-by-disorder mechanism. The quantum reduction of both sublattice magnetizations in the peculiar quantum ordered state gradually diminishes upon increasing the coordination number of the underlying Husimi lattice.
We study the spin-1/2 Ising-XXZ model on a decorated honeycomb lattice composed of five spins per unit cell, one Ising spin, and four Heisenberg spins. This model involving the Heisenberg exchange interaction is one of the few models that can be exactly solvable through the generalized star-triangle transformation. The significance of this model is its close relationship to the fully decorated quantum Heisenberg honeycomb lattice since 4/5 of the particles are Heisenberg spins. We investigate the phase diagram at zero temperature and identify a relevant quantum spin frustrated phase resulting from the contribution of quantum Heisenberg exchange interaction. We obtain an exact residual entropy for the quantum spin frustrated phase, which coincides with the residual entropy of the antiferromagnetic spin-1/2 Ising model on a triangular lattice. We also thoroughly explore its thermodynamic properties, focusing mainly on the frustrated region such as entropy, specific heat, spontaneous magnetization, and critical temperature under several conditions.
The ground state and zero-temperature magnetization process of the spin-1/2 Ising-Heisenberg model on two-dimensional triangles-in-triangles lattices are exactly calculated using eigenstates of the smallest commuting spin clusters. Our ground-state analysis of the investigated classical-quantum spin model reveals three unconventional dimerized or trimerized quantum ground states besides two classical ground states. It is demonstrated that the spin frustration is responsible for a variety of magnetization scenarios with up to three or four intermediate magnetization plateaus of either quantum or classical nature. The exact analytical results for the Ising-Heisenberg model are confronted with the corresponding results for the purely quantum Heisenberg model, which were obtained by numerical exact diagonalizations based on the Lanczos algorithm for finite-size spin clusters of 24 and 21 sites, respectively. It is shown that the zero-temperature magnetization process of both models is quite reminiscent, and hence, one may obtain some insight into the ground states of the quantum Heisenberg model from the rigorous results for the Ising-Heisenberg model even though exact ground states for the Ising-Heisenberg model do not represent true ground states for the pure quantum Heisenberg model.
Motivated by the search for unconventional orders in frustrated quantum magnets, we present a multi-method investigation into the nature of the quantum phase diagram of the spin-1/21/21/2 Heisenberg model on the maple-leaf lattice with three symmetry-inequivalent nearest-neighbor interactions. It has been argued that the parameter regime with antiferromagnetic couplings on hexagons JhJ_hJh​ and ferromagnetic couplings on triangles JtJ_tJt​ and dimer JdJ_dJd​ bonds, is potentially host to a cornucopia of emergent phases with unconventional orders. Our analysis indeed identifies an extended region where any conventional dipolar magnetic order is absent. A hexagonal singlet state is found in the region around Jd=Jt=0J_{d}=J_{t}=0Jd​=Jt​=0, while a dimerized hexagonal singlet order of a lattice nematic character appears proximate to the phase boundary with the c120∘120^\circ120∘ antiferromagnetic order. Interestingly, upon traversing the bulk of the paramagnetic (PM) region, we find a variety of distinct correlation profiles, which are qualitatively different from those of the hexagonal singlet and dimerized hexagonal singlet orders but feature no appreciable spin-nematic response, while the boundary with the ferromagnetic phase shows evidence of spin-nematic order. This PM region is thus likely host to an ensemble of nonmagnetic phases which could putatively include quantum spin liquids. Our phase diagram is built from a complementary application of state-of-the-art implementations of the cluster mean-field and pseudo-fermion functional renormalization group approaches, together with an unconstrained Luttinger-Tisza treatment of the model providing insights from the semi-classical limit.