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arXiv:1209.4166 · Journal of Physics A Mathematical and Theoretical

Quantum correlations in a system of nuclears= 1/2 spins in a strong magnetic field

Edward B. Fel’dman, E. I. Kuznetsova, M. A. Yurishchev

Published Nov 8, 2012• 25 citations
arXivHTMLPDF

Abstract

Entanglement and quantum discord for a pair of nuclear spins s = 1/2 in a nanopore filled with a gas of spin-carrying molecules (atoms) are studied. The correlation functions describing dynamics of dipolar-coupled spins in a nanopore are found. The dependence of spin-pair entanglement on the temperature and the number of spins is obtained from the reduced density matrix, which is centrosymmetric (CS). An analytic expression for the concurrence is obtained for an arbitrary CS density matrix. It is shown that the quantum discord as a measure of quantum correlations attains a significant value at low temperatures. It is also shown that the discord in the considered model has 'flickering' character and disappears periodically in the course of time evolution of the system. The geometric discord is studied for arbitrary 4 × 4 CS density matrices.

DOI
10.1088/1751-8113/45/47/475304

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Entanglement and quantum discord for a pair of nuclear spins s = 1/2 in a nanopore filled with a gas of spin-carrying molecules (atoms) are studied. The correlation functions describing dynamics of dipolar-coupled spins in a nanopore are found. The dependence of spin-pair entanglement on the temperature and the number of spins is obtained from the reduced density matrix, which is centrosymmetric (CS). An analytic expression for the concurrence is obtained for an arbitrary CS density matrix. It is shown that the quantum discord as a measure of quantum correlations attains a significant value at low temperatures. It is also shown that the discord in the considered model has 'flickering' character and disappears periodically in the course of time evolution of the system. The geometric discord is studied for arbitrary 4 × 4 CS density matrices.
A local orthogonal transformation that transforms any centrosymmetric density matrix of a two-qubit system to the X form has been found. A piecewise-analytic-numerical formula Q = min{Q π/2, Q θ, Q 0}, where Q π/2 and Q 0 are analytical expressions and the branch Q 0 θ can be obtained only by numerically searching for the optimal measurement angle θ ∈ (0, π/2), is proposed to calculate the quantum discord Q of a general X state. The developed approaches have been applied for a quantitative description of the recently predicted flickering (periodic disappearance and reappearance) of the quantum-information pair correlation between nuclear 1/2 spins of atoms or molecules of a gas (for example, 129Xe) in a bounded volume in the presence of a strong magnetic field.
The quantum properties of dynamic correlations in a system of an electron spin surrounded by nuclear spins under the conditions of free induction decay (FID) and spin echo have been studied. Analytical results for the time evolution of mutual information, classical part of correlations, and quantum part characterized by quantum discord have been obtained within the central spin model in the high-temperature approximation. The same formulas describe the quantum discord in both the FID and the spin echo although the forms of the dependences are different because of difference in the parameters entering into the formulas. Discord of the spin echo compared with the FID has a strong dependence on time at short times, and it tends to zero with decreasing of the magnetic field, whereas in the case of the FID it reaches a plateau.
We describe the dynamics of quantum discord of two interacting spin-1/2’s subjected to controllable time-dependent magnetic fields. The exact time evolution of discord is given for various input mixed states consisting of classical mixtures of two Bell states. The quantum discord manifests a complex oscillatory behaviour in time and is compared with that of quantum entanglement, measured by concurrence. The interplay of the action of the time-dependent magnetic fields and the spin-coupling mechanism in the occurrence and evolution of quantum correlations is examined in detail.
We investigate evolution of quantum correlations in ensembles of two-qubit nuclear spin systems via nuclear magnetic resonance techniques. We use discord as a measure of quantum correlations and the Werner state as an explicit example. We, first, introduce different ways of measuring discord and geometric discord in two-qubit systems and then describe the following experimental studies: (a) We quantitatively measure discord for Werner-like states prepared using an entangling pulse sequence. An initial thermal state with zero discord is gradually and periodically transformed into a mixed state with maximum discord. The experimental and simulated behavior of rise and fall of discord agree fairly well. (b) We examine the efficiency of dynamical decoupling sequences in preserving quantum correlations. In our experimental setup, the dynamical decoupling sequences preserved the traceless parts of the density matrices at high fidelity. But they could not maintain the purity of the quantum states and so were unable to keep the discord from decaying. (c) We observe the evolution of discord for a singlet-triplet mixed state during a radio-frequency spin-lock. A simple relaxation model describes the evolution of discord, and the accompanying evolution of fidelity of the long-lived singlet state, reasonably well.
The quantum properties of dynamic correlations in a system of an electron spin surrounded by nuclear spins under the conditions of free induction decay and electron spin echo have been studied. Analytical results for the time evolution of mutual information, classical part of correlations, and quantum part characterized by quantum discord have been obtained within the central-spin model in the high-temperature approximation. The same formulas describe discord in both free induction decay and spin echo although the time and magnetic field dependences are different because of difference in the parameters entering into the formulas. Changes in discord in the presence of the nuclear polarization β I in addition to the electron polarization β S have been calculated. It has been shown that the method of reduction of the density matrix to a two-spin electron-nuclear system provides a qualitatively correct description of pair correlations playing the main role at β S ≈ β I and small times. At large times, such correlations decay and multispin correlations ensuring nonzero mutual information and zero quantum discord become dominant.
We describe the dynamics of quantum discord of two interacting spin-1/2 subjected to controllable time-dependent magnetic fields. The exact time evolution of discord is given for various input mixed states consisting of classical mixtures of two Bell states. The quantum discord manifests a complex oscillatory behaviour in time and is compared with that of quantum entanglement, measured by concurrence. The interplay of the action of the time-dependent magnetic fields and the spin-coupling mechanism in the occurrence and evolution of quantum correlations is examined in detail.