For an open quantum system, we investigate the pumped current induced by a slow modulation of control parameters on the basis of the quantum master equation and full counting statistics. We find that the average and the cumulant generating function of the pumped quantity are characterized by the geometrical Berry-phase-like quantities in the parameter space, which is associated with the generator of the master equation. From our formulation, we can discuss the geometrical pumping under the control of the chemical potentials and temperatures of reservoirs. We demonstrate the formulation by spinless electrons in coupled quantum dots. We show that the geometrical pumping is prohibited for the case of noninteracting electrons if we modulate only temperatures and chemical potentials of reservoirs, while the geometrical pumping occurs in the presence of an interaction between electrons.
For an open quantum system, we investigate the pumped current induced by a slow modulation of control parameters on the basis of the quantum master equation and full counting statistics. We find that the average and the cumulant generating function of the pumped quantity are characterized by the geometrical Berry-phase-like quantities in the parameter space, which is associated with the generator of the master equation. From our formulation, we can discuss the geometrical pumping under the control of the chemical potentials and temperatures of reservoirs. We demonstrate the formulation by spinless electrons in coupled quantum dots. We show that the geometrical pumping is prohibited for the case of noninteracting electrons if we modulate only temperatures and chemical potentials of reservoirs, while the geometrical pumping occurs in the presence of an interaction between electrons.
We set up a general density-operator approach to geometric steady-state pumping through slowly driven open quantum systems. This approach applies to strongly interacting systems that are weakly coupled to multiple reservoirs at high temperature, illustrated by an Anderson quantum dot. Pumping gives rise to a nonadiabatic geometric phase that can be described by a framework originally developed for classical dissipative systems by Landsberg. This geometric phase is accumulated by the transported observable (charge, spin, energy) and not by the quantum state. It thus differs radically from the adiabatic Berry-Simon phase, even when generalizing it to mixed states, following Sarandy and Lidar. As a key feature, our geometric formulation of pumping stays close to a direct physical intuition (i) by tying gauge transformations to calibration of the meter registering the transported observable and (ii) by deriving a geometric connection from a driving-frequency expansion of the current. Furthermore, our approach provides a systematic and efficient way to compute the geometric pumping of various observables, including charge, spin, energy, and heat. These insights seem to be generalizable beyond the present paper's working assumptions (e.g., Born-Markov limit) to more general open-system evolutions involving memory and strong-coupling effects due to low-temperature reservoirs as well. Our geometric curvature formula reveals a general experimental scheme for performing geometric transport spectroscopy that enhances standard nonlinear spectroscopies based on measurements for static parameters. We indicate measurement strategies for separating the useful geometric pumping contribution to transport from nongeometric effects. A large part of the paper is devoted to an explicit comparison with the Sinitsyn-Nemenmann full-counting-statistics (FCS) approach to geometric pumping, restricting attention to the first moments of the pumped observable. Covering all key aspects, gauge freedom, pumping connection, curvature, and gap condition, we argue that our approach is physically more transparent and, importantly, simpler for practical calculations. In particular, this comparison allows us to clarify how in the FCS approach an ``adiabatic'' approximation leads to a manifestly nonadiabatic result involving a finite retardation time of the response to parameter driving.
We consider the process of pumping charge through an open quantum system, motivated by the example of a quantum dot with strong repulsive or attractive electron-electron interaction. Using the geometric formulation of adiabatic nonunitary evolution put forward by Sarandy and Lidar, we derive an encompassing approach to ideal charge measurements of time-dependently driven transport, that stays near the familiar approach to closed systems. Following Schaller, Kießlich and Brandes we explicitly account for a meter that registers the transported charge outside the system. The gauge freedom underlying geometric pumping effects in all moments of the transported charge emerges naturally as the calibration of this meter. Remarkably, we find that geometric and physical considerations cannot be applied independently as done in closed systems: physical recalibrations do not form a group due to constraints of positivity (Bochner's theorem). This complication goes unnoticed when considering only the average charge but it is relevant for understanding the origin of geometric effects in the higher moments of the charge-transport statistics. As an application we derive two prominent existing approaches to pumping, based on full-counting-statistics (FCS) and adiabatic-response (AR), respectively, from our approach in a transparent way. This allows us to reconcile all their apparent incompatibilities, in particular the puzzle how for the average charge the nonadiabatic stationary-state AR result can exactly agree with the adiabatic nonstationary FCS result. We relate this and other difficulties to a single characteristic of geometric approaches to open systems: the system-environment boundary can always be chosen to either include or exclude the ideal charge meter. This leads to a physically motivated relation between the mixed-state Berry phase and the entirely different geometric phase of Landsberg.
The concept of Geometric Phase in Quantum Mechanics is generally formulated en- tirely in terms of geometric structure of complex Hilbert Space. This tutorial article gives a general mathematical overview of the Geometric phase introduced by Berry with the conditions over the system’s evolution embedded through adiabaticity and cyclicity, which were subsequently relaxed sequentially by Aharonov-Anandan, Samuel-Bhandari, and later by Mukunda and Simon by using the idea of Bargmann Invariants. The arti- cle presents a thorough and illustrative overview regarding the mathematical derivation behind the upliftment of the conditions, which results in the generalized definition of the Geometric phase for quantum systems. In addition to that, the article also gives an overall idea about the general analytical aspects of finding the Geometric phase for three level open quantum systems undergoing decoherence and dephasing due to interaction with the surroundings in the weak system reservoir coupling limit described by quantum master equations.
We consider a finite quantum system under slow driving and weakly coupled to thermal reservoirs at different temperatures. We present a systematic derivation of the quantum master equation for the density matrix and the out-of-time-order correlators. We start from the microscopic Hamiltonian and we formulate the equations ruling the dynamics of these quantities by recourse to the Schwinger-Keldysh nonequilibrium Green's function formalism, performing a perturbative expansion in the coupling between the system and the reservoirs. We focus on the adiabatic dynamics, which corresponds to considering the linear response in the ratio between the relaxation time due to the system-reservoir coupling and the time scale associated to the driving. We calculate the particle and energy fluxes. We illustrate the formalism in the case of a qutrit coupled to bosonic reservoirs and of a pair of interacting quantum dots attached to fermionic reservoirs, also discussing the relevance of coherent effects.
We present a detailed analysis of slowly driven quantum thermal machines based on interacting qubits within the framework of the Lindblad master equation. By implementing a systematic expansion in the driving rate, we derive explicit expressions for the rate of work of the driving forces, the heat currents exchanged with the reservoirs, and the entropy production up to second order, ensuring full thermodynamic consistency in the linear-response regime. The formalism naturally separates geometric and dissipative contributions, identified by a Berry curvature and a metric in parameter space, respectively. Analytical results show that the geometric heat pumped per cycle is bounded by kBTNqln2 for Nq non-interacting qubits, in direct analogy with the Landauer limit for entropy change. This bound can be surpassed when qubit interactions and asymmetric couplings to the baths are introduced. Numerical results for the interacting two-qubit system reveal a non-trivial role of the interaction between qubits and the coupling between the qubits and the baths in the behavior of the dissipated power. The approach provides a general platform for studying dissipation, pumping, and performance optimization in driven quantum devices operating as heat engines.
For quantum transport through mesoscopic systems, a quantum master-equation approach is developed in terms of compact expressions for the transport current and the reduced density matrix of the system. The present work is an extension of Gurvitz's approach for quantum transport and quantum measurement, namely, to finite temperature and arbitrary bias voltage. Our derivation starts from a second-order cumulant expansion of the tunneling Hamiltonian; then follows the conditional average over the electrode reservoir states. As a consequence, in the usual weak-tunneling regime, the established formalism is applicable for a wide range of transport problems. The validity of the formalism and its convenience in application are well illustrated by a number of examples.