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arXiv:1208.2067 · Physical Review Letters

Measurement of the Homogeneous Contact of a Unitary Fermi Gas

Yoav Sagi, Tara E. Drake, Rabin Paudel, Deborah Jin

Published Nov 27, 2012• 145 citations
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Abstract

By selectively probing the center of a trapped gas, we measure the local, or homogeneous, contact of a unitary Fermi gas as a function of temperature. Tan's contact, C, is proportional to the derivative of the energy with respect to the interaction strength and is thus an essential thermodynamic quantity for a gas with short-range correlations. Theoretical predictions for the temperature dependence of C differ substantially, especially near the superfluid transition, T(c), where C is predicted to either sharply decrease, sharply increase, or change very little. For T/T(F)>0.4, our measurements of the homogeneous gas contact show a gradual decrease of C with increasing temperature, as predicted by theory. We observe a sharp decrease in C at T/T(F)=0.16, which may be due to the superfluid phase transition. While a sharp decrease in C below T(c) is predicted by some many-body theories, we find that none of the predictions fully account for the data.

DOI
10.1103/physrevlett.109.220402

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By selectively probing the center of a trapped gas, we measure the local, or homogeneous, contact of a unitary Fermi gas as a function of temperature. Tan's contact, C, is proportional to the derivative of the energy with respect to the interaction strength and is thus an essential thermodynamic quantity for a gas with short-range correlations. Theoretical predictions for the temperature dependence of C differ substantially, especially near the superfluid transition, T(c), where C is predicted to either sharply decrease, sharply increase, or change very little. For T/T(F)>0.4, our measurements of the homogeneous gas contact show a gradual decrease of C with increasing temperature, as predicted by theory. We observe a sharp decrease in C at T/T(F)=0.16, which may be due to the superfluid phase transition. While a sharp decrease in C below T(c) is predicted by some many-body theories, we find that none of the predictions fully account for the data.
The contact I, introduced by Tan, has emerged as a key parameter characterizing universal properties of strongly interacting Fermi gases. For ultracold Fermi gases near a Feshbach resonance, the contact depends upon two quantities: the interaction parameter 1/(k(F)a), where k(F) is the Fermi wave vector and a is the s-wave scattering length, and the temperature T/T(F), where T(F) is the Fermi temperature. We present the first measurements of the temperature dependence of the contact in a unitary Fermi gas using Bragg spectroscopy. The contact is seen to follow the predicted decay with temperature and shows how pair-correlations at high momentum persist well above the superfluid transition temperature.
A quantity known as the contact is a fundamental thermodynamic property of quantum many-body systems with short-range interactions. Determination of the temperature dependence of the contact for the unitary Fermi gas of infinite scattering length has been a major challenge, with different calculations yielding qualitatively different results. Here we use finite-temperature auxiliary-field quantum Monte Carlo (AFMC) methods on the lattice within the canonical ensemble to calculate the temperature dependence of the contact for the homogeneous spin-balanced unitary Fermi gas. We extrapolate to the continuum limit for 40, 66, and 114 particles, eliminating systematic errors due to finite-range effects. We observe a dramatic decrease in the contact as the superfluid critical temperature is approached from below, followed by a gradual weak decrease as the temperature increases in the normal phase. Our theoretical results are in excellent agreement with the most recent precision ultracold atomic gas experiments. We also present results for the energy as a function of temperature in the continuum limit.
A key quantity in strongly interacting resonant Fermi gases is the contact C, which characterizes numerous properties such as the momentum distribution at large momenta or the pair correlation function at short distances. The temperature dependence of C was measured at unitarity, where existing theoretical predictions differ substantially even at the qualitative level. We report accurate data for the contact and the momentum distribution of the unitary gas in the normal phase, obtained by bold diagrammatic Monte Carlo and Borel resummation. Our results agree with experimental data within error bars and provide crucial benchmarks for the development of advanced theoretical treatments and precision measurements.
We measure radio frequency (rf) spectra of the homogeneous unitary Fermi gas at temperatures ranging from the Boltzmann regime through quantum degeneracy and across the superfluid transition. For all temperatures, a single spectral peak is observed. Its position smoothly evolves from the bare atomic resonance in the Boltzmann regime to a frequency corresponding to nearly one Fermi energy at the lowest temperatures. At high temperatures, the peak width reflects the scattering rate of the atoms, while at low temperatures, the width is set by the size of fermion pairs. Above the superfluid transition, and approaching the quantum critical regime, the width increases linearly with temperature, indicating non-Fermi-liquid behavior. From the wings of the rf spectra, we obtain the contact, quantifying the strength of short-range pair correlations. We find that the contact rapidly increases as the gas is cooled below the superfluid transition.
The recently discovered universal thermodynamic behavior of dilute, strongly interacting Fermi gases also implies a universal structure in the many-body pair-correlation function at short distances, as quantified by the contact . Here, we theoretically calculate the temperature dependence of this universal contact for a Fermi gas in free space and in a harmonic trap. At high temperatures above the Fermi degeneracy temperature, T ≳ T F , we obtain a reliable non-perturbative quantum virial expansion up to third order. At low temperatures, we compare different approximate strong-coupling theories. These make different predictions, which need to be tested either by future experiments or by advanced quantum Monte Carlo simulations. We conjecture that in the universal unitarity limit, the contact or correlation decreases monotonically with increasing temperature, unless the temperature is significantly lower than the critical temperature, T ≪ T c ∼0.2 T F . We also discuss briefly how to measure the universal contact in either homogeneous or harmonically trapped Fermi gases.
The nature of the normal phase of an ultracold Fermi gas in the BCS-BEC crossover regime is an interesting and unresolved question. As interactions increase, while the many-body ground state remains a condensate of paired fermions, the normal state must evolve from a Fermi liquid to a Bose gas of molecules. In this thesis, I present a technique to spatially select a homogeneous sample from the center of a trapped gas to explore this crossover. Combining this technique with RF spectroscopy, we locally measure Tan's contact as a function of temperature and compare to various many-body theories. In another experiment, we measure the distribution of single-particle energies and momenta for a normal gas across the BCS-BEC crossover. We find that the data fit well to a two-part function that includes a peak corresponding to fermionic quasiparticles and an "incoherent background" that is modeled using the dispersion of thermal molecules. I also describe the construction of a new-generation Fermi gas apparatus.