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arXiv:1207.1106 · Physical Review B

Breakdown of Fermi liquid behavior at the (π,π)=2kF spin-density wave quantum-critical point: The case of electron-doped cuprates

Dominic Bergeron, Debanjan Chowdhury, Matthias Punk, Subir Sachdev A, A.–M. S. Tremblay

Published Oct 11, 2012• 29 citations
arXivHTMLPDF

Abstract

Many correlated materials display a quantum-critical point between a paramagnetic and a spin-density wave (SDW) state. The SDW wave vector connects points, so-called hot spots, on opposite sides of the Fermi surface. The Fermi velocities at these pairs of points are in general not parallel. Here, we consider the case where pairs of hot spots coalesce, and the wave vector $(\ensuremath{\pi},\ensuremath{\pi})$ of the SDW connects hot spots with parallel Fermi velocities. Using the specific example of electron-doped cuprates, we first show that Kanamori screening and generic features of the Lindhard function make this case experimentally relevant. The temperature dependence of the correlation length, the spin susceptibility, and the self-energy at the hot spots are found using the two-particle self-consistent theory and specific numerical examples worked out for band and interaction parameters characteristic of the electron-doped cuprates. While the curvature of the Fermi surface at the hot spots leads to deviations from perfect nesting, the pseudonesting conditions lead to drastic modifications of the temperature dependence of these physical observables: Neglecting logarithmic corrections, the correlation length $\ensuremath{\xi}$ scales like $1/T$, namely, $z=1$ instead of the naive $z=2$, the $(\ensuremath{\pi},\ensuremath{\pi})$ static spin susceptibility $\ensuremath{\chi}$ like $1/\sqrt{T}$, and the imaginary part of the self-energy at the hot spots like ${T}^{3/2}$. The correction ${T}_{1}^{\ensuremath{-}1}\ensuremath{\sim}{T}^{3/2}$ to the Korringa NMR relaxation rate is subdominant. We also consider this problem at zero temperature, or for frequencies larger than temperature, using a field-theoretical model of gapless collective bosonic modes (SDW fluctuations) interacting with fermions. The imaginary part of the retarded fermionic self-energy close to the hot spots scales as $\ensuremath{-}{\ensuremath{\omega}}^{3/2}\mathrm{ln}\ensuremath{\omega}$. This is less singular than earlier predictions of the form $\ensuremath{-}\ensuremath{\omega}\mathrm{ln}\ensuremath{\omega}$. The difference arises from the effects of umklapp terms that were not included in previous studies.

DOI
10.1103/physrevb.86.155123

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Many correlated materials display a quantum-critical point between a paramagnetic and a spin-density wave (SDW) state. The SDW wave vector connects points, so-called hot spots, on opposite sides of the Fermi surface. The Fermi velocities at these pairs of points are in general not parallel. Here, we consider the case where pairs of hot spots coalesce, and the wave vector (\ensuremathπ,\ensuremathπ)(\ensuremath{\pi},\ensuremath{\pi})(\ensuremathπ,\ensuremathπ) of the SDW connects hot spots with parallel Fermi velocities. Using the specific example of electron-doped cuprates, we first show that Kanamori screening and generic features of the Lindhard function make this case experimentally relevant. The temperature dependence of the correlation length, the spin susceptibility, and the self-energy at the hot spots are found using the two-particle self-consistent theory and specific numerical examples worked out for band and interaction parameters characteristic of the electron-doped cuprates. While the curvature of the Fermi surface at the hot spots leads to deviations from perfect nesting, the pseudonesting conditions lead to drastic modifications of the temperature dependence of these physical observables: Neglecting logarithmic corrections, the correlation length \ensuremathξ\ensuremath{\xi}\ensuremathξ scales like 1/T1/T1/T, namely, z=1z=1z=1 instead of the naive z=2z=2z=2, the (\ensuremathπ,\ensuremathπ)(\ensuremath{\pi},\ensuremath{\pi})(\ensuremathπ,\ensuremathπ) static spin susceptibility \ensuremathχ\ensuremath{\chi}\ensuremathχ like 1/T1/\sqrt{T}1/T​, and the imaginary part of the self-energy at the hot spots like T3/2{T}^{3/2}T3/2. The correction T1\ensuremath−1\ensuremath∼T3/2{T}_{1}^{\ensuremath{-}1}\ensuremath{\sim}{T}^{3/2}T1\ensuremath−1​\ensuremath∼T3/2 to the Korringa NMR relaxation rate is subdominant. We also consider this problem at zero temperature, or for frequencies larger than temperature, using a field-theoretical model of gapless collective bosonic modes (SDW fluctuations) interacting with fermions. The imaginary part of the retarded fermionic self-energy close to the hot spots scales as \ensuremath−\ensuremathω3/2ln\ensuremathω\ensuremath{-}{\ensuremath{\omega}}^{3/2}\mathrm{ln}\ensuremath{\omega}\ensuremath−\ensuremathω3/2ln\ensuremathω. This is less singular than earlier predictions of the form \ensuremath−\ensuremathωln\ensuremathω\ensuremath{-}\ensuremath{\omega}\mathrm{ln}\ensuremath{\omega}\ensuremath−\ensuremathωln\ensuremathω. The difference arises from the effects of umklapp terms that were not included in previous studies.
We analyze quantum fluctuation effects at the onset of incommensurate 2 k F charge- or spin-density-wave order in two-dimensional metals for a model in which the ordering wave vector Q connects a single pair of hot spots on the Fermi surface with a vanishing Fermi surface curvature. The tangential momentum dependence of the bare dispersion near the hot spots is proportional to | k t | α with α > 2 . We first compute the order parameter susceptibility and the fermion self-energy in a random phase approximation (RPA). Logarithmic divergences are subsequently treated by a renormalization-group analysis. The coupling between the order parameter fluctuations and the fermions vanishes logarithmically in the low-energy limit. As a consequence, the logarithmic divergences found in the RPA do not sum up to anomalous power laws. Instead, only logarithmic corrections to Fermi liquid behavior are obtained. In particular, the quasiparticle weight and the Fermi velocity vanish logarithmically at the hot spots. Published by the American Physical Society 2024
We report on numerically exact determinantal quantum Monte Carlo simulations of the onset of spin-density-wave (SDW) order in itinerant electron systems captured by a sign-problem-free two-dimensional lattice model. Extensive measurements of the SDW correlations in the vicinity of the phase transition reveal that the critical dynamics of the bosonic order parameter are well described by a dynamical critical exponent z=2z=2z=2, consistent with Hertz-Millis theory, but are found to follow a finite-temperature dependence that does not fit the predicted behavior of the same theory. The presence of critical SDW fluctuations is found to have a strong impact on the fermionic quasiparticles, giving rise to a dome-shaped superconducting phase near the quantum critical point. In the superconducting state we find a gap function that has an opposite sign between the two bands of the model and is nearly constant along the Fermi surface of each band. Above the superconducting Tc{T}_{c}Tc​, our numerical simulations reveal a nearly temperature and frequency independent self-energy causing a strong suppression of the low-energy quasiparticle weight in the vicinity of the hot spots on the Fermi surface. This indicates a clear breakdown of Fermi liquid theory around these points.
The spin-fermion (SF) model postulates that the dominant coupling between low-energy fermions in near critical metals is mediated by collective spin fluctuations (paramagnons) peaked at the Néel wave vector, Q N , connecting hot spots on opposite sides of the Fermi surface. It has been argued that strong correlations at hot spots lead to a Fermi surface deformation (FSD) featuring flat regions and increased nesting. This conjecture was confirmed in the perturbative self-consistent calculations when the paramagnon propagator dependence on momentum deviation from Q N is given by χ − 1 ∝ | Δ q | . Using diagrammatic Monte Carlo (diagMC) technique we show that such a dependence holds only at temperatures orders of magnitude smaller than any other energy scale in the problem, indicating that a different mechanism may be at play. Instead, we find that a χ − 1 ∝ | Δ q | 2 dependence yields a robust finite- T scenario for achieving FSD. To link phenomenological and microscopic descriptions, we applied the connected determinant diagMC method to the ( t − t ′ ) Hubbard model and found that at large U / t > 5.5 before the formation of electron and hole pockets (i) the FSD defined as a maximum of the spectral function is not very pronounced; instead, it is the lines of zeros of the renormalized dispersion relation that deforms toward nesting, and (ii) the static spin susceptibility is well described by χ − 1 ∝ | Δ q | 2 . Flat FS regions yield a nontrivial scenario for realizing a non-Fermi liquid state. Published by the American Physical Society 2024
We study superfluidity in strongly correlated systems by focusing three features as follows. First, interplay between superfluidity and other order parameters near quantum critical points is studied. The onset positions of the order parameters with or without superconductivity determines how they interact with each other. For the spin density wave (SDW) transition, we find that the quantum critical point shifts by order |∆|, where ∆ is pairing amplitude, so that the region of SDW order is smaller in the superconductor than in the metal. This shift is larger than the |∆|2 shift predicted by theories of competing orders which ignore Fermi surface effects. Second, we study a doped antiferromagnetic Mott insulator motivated by copper based high temperature superconductors. Based on spin and charge fractionalization, the algebraic charge liquid phase whose bosonic spinons have energy gap but fermionic holons form Fermi surfaces and its superconductivity are studied. We show fluctuations of local SDW order orientation lead to d-wave superconductivity, and its quantum critical pairing mechanisms are investigated. Also, a theory of bound states between spinons and holons is studied. We show that the fractionalization induces a doubling electron-like quasiparticles, which naturally induces the fractionalized Fermi liquid. The bound state theory describes exotic properties of the underdoped Cuprates such as “nodal-antinodal dichotomy” at a mean field level description. At last, we study superfluidity of fermions in optical lattices near the Feshbach resonance. Due to divergence of scattering length at the resonance, universality is observed and characteristics of superfluidity has been studied. We extend such universal properties by considering superfluid-insulator transition with an even integer number of fermions per unit cell. The resulting insulator interpolates between a band insulator of fermions and a Mott insulator of fermion pairs.
Antiferromagnetic fluctuations in two dimensions cause a decrease in spectral weight at so-called hot spots associated with the pseudogap in electron-doped cuprates. In the 2D2\text{D}2D Hubbard model, these hot spots occur when the Vilk criterion is satisfied, namely, when the spin correlation length exceeds the thermal de Broglie wavelength. Using the two-particle self-consistent approach, here we show that this criterion may be violated near the antiferromagnetic quantum critical point when sufficient disorder is added to the model. Static disorder decreases inelastic scattering, in contradiction with Matthiessen's rule, leading to a shift in the position of the quantum critical point and a modification of the conditions for the appearance of hot spots. This opens the road to a study of the interplay between disorder, antiferromagnetic fluctuations, and superconductivity in electron-doped cuprates.
Qualitative changes in thermodynamic and single-particle properties characterize the transition between the pseudogapped electronic liquid and the Fermi liquid. Recent cold-atom experiments on a simulator of the Hubbard model with nearest-neighbor hoppings [L. H. Kendrick , .] showed that the isothermal compressibility κ ( δ ) has a maximum as a function of doping δ . Here, we use the two-particle self-consistent plus approach to explain these experiments and connect the maximum in κ ( δ ) to the transformation of the single-particle spectrum from the pseudogapped to the metallic regime. This elucidates the nature of the pseudogap. Specifically, the maximum in κ ( δ ) practically coincides with the doping at which the precursor of the lower ( π , π ) spin-density-wave (SDW) band at the antinodal point crosses the zero-frequency ω = 0 . The Knight shift χ sp ( 0 , 0 ) ( δ ) , as a function of doping, should also have a maximum. In addition, we demonstrate that two-particle self-consistent plus correctly predicts a maximum in the temperature dependence of the Knight shift χ sp ( 0 , 0 ) ( T ) , consistent with recent ultracold-atom experiments [T. Chalopin , .]. The maxima in both quantities should exist, at sufficiently low temperatures ( T ), in both the intermediate U ≈ U Mott and weak U < U Mott interaction limits. In both limits, the mechanism is critical thermal SDW fluctuations. At the antinodal pseudogap, the correlation length at δ max ( T ) can be small, controlled not by static but by dynamic critical thermal fluctuations. We also find that the SDW fluctuations are incommensurate at δ = δ max . We predict that, at low T , the multiple peaks in the spin susceptibility in the incommensurate case lead to more than two SDW precursor peaks in the spectral function and density of states. By allowing access to parameter regimes relevant to cuprates—including further-neighbor hopping ( t ′ , t ′′ ) and low temperatures, our work provides a high-impact tool for further studies by the broader community.