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arXiv:1206.7054 · Physical Review A

Electric-field sensing near the surface microstructure of an atom chip using cold Rydberg atoms

J. D. Carter, Owen Cherry, J. D. D. Martin

Published Nov 1, 2012• 59 citations
arXivHTMLPDF

Abstract

The electric fields near the heterogeneous metal-dielectric surface of an atom chip were measured using cold atoms. The atomic sensitivity to electric fields was enhanced by exciting the atoms to Rydberg states that are 10${}^{8}$ times more polarizable than the ground state. We attribute the measured fields to charging of the insulators between the atom chip wires. Surprisingly, it is found that although the chip wire currents were turned off before Rydberg excitation, the measured fields were strongly influenced by how the wire currents had been applied. These fields may be dramatically lowered with appropriate voltage biasing, suggesting configurations for the future development of hybrid quantum systems.

DOI
10.1103/physreva.86.053401

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The electric fields near the heterogeneous metal-dielectric surface of an atom chip were measured using cold atoms. The atomic sensitivity to electric fields was enhanced by exciting the atoms to Rydberg states that are 108{}^{8}8 times more polarizable than the ground state. We attribute the measured fields to charging of the insulators between the atom chip wires. Surprisingly, it is found that although the chip wire currents were turned off before Rydberg excitation, the measured fields were strongly influenced by how the wire currents had been applied. These fields may be dramatically lowered with appropriate voltage biasing, suggesting configurations for the future development of hybrid quantum systems.
On one side, atom-chip experiments have demonstrated to be a versatile tool to study quantum physics in cold atoms systems. On the other side, Rydberg atoms have exaggerated properties that makes them good candidates to study quantum information and quantum simulations protocols. In this thesis both system are put together with the aim to study Rydberg physics (in particular atom-atom interaction) in an atom-chip experiment. Due to the exaggerated properties of Rydberg atoms they are very sensitive to electric fields. Thus, the combination of Rydberg atoms with surfaces can be challenging. Therefore a detailed characterization of the mentioned stray electric fields via the analysis of Stark-Zeeman maps is crucial. We employ two-photon Rydberg Stark spectroscopy of a micron-sized cloud of magnetically trapped ultracold rubidium atoms to characterize the electric fields near our atom-chip. Once we characterized the local electric fields we were able to study in more detail the effect of Rydberg excitation in the ultracold cloud of atoms. For instance we observed the formation of ultralong-range Rydberg molecules in our system. In these molecules a ground state atom is weakly bound to the Rydberg electron. We also attempted to observe the effect of Rydberg blockade in the system by looking at the characteristics of Rydberg spectra. Finally we studied the possibility of inducing rf transitions within a Rydberg state manifold in order to enhance our detection method and populate states that are not accessible directly with a two-photon laser transition.
We use the sensitive response to electric fields of Rydberg atoms to characterize all three vector components of the local electric field close to an atom-chip surface. We measured Stark-Zeeman maps of SSS and DDD Rydberg states using an elongated cloud of ultracold rubidium atoms (temperature $T\ensuremath{\sim}2.5\phantom{\rule{4pt}{0ex}}\ensuremath{\mu}\mathrm{K}$) trapped magnetically $100\phantom{\rule{4pt}{0ex}}\ensuremath{\mu}\mathrm{m}$ from the chip surface. The spectroscopy of SSS states yields a calibration for the generated local electric field at the position of the atoms. The values for different components of the field are extracted from the more complex response of DDD states to the combined electric and magnetic fields. From the analysis we find residual fields in the two uncompensated directions of $0.0\ifmmode\pm\else\textpm\fi{}0.2$ and $1.98\ifmmode\pm\else\textpm\fi{}0.09$ V/cm. This method also allows us to extract a value for the relevant field gradient along the long axis of the cloud. The manipulation of electric fields and the magnetic trapping are both done using on-chip wires, making this setup a promising candidate to observe Rydberg-mediated interactions on a chip.
An atom chip has been fabricated for the study of interactions between 87^{87}87Rb Rydberg atoms and a Au surface. The chip tightly confines cold atoms by generating high magnetic field gradients using microfabricated current-carrying wires. These trapped atoms may be excited to Rydberg states at well-defined atom-surface distances. For the purpose of Rydberg atom-surface interaction studies, the chip has a thermally evaporated Au surface layer, separated from the underlying trapping wires by a planarizing polyimide dielectric. Special attention was paid to the edge roughness of the trapping wires, the planarization of the polyimide, and the grain structure of the Au surface.
Hybrid quantum platforms based on highly excited Rydberg atoms coupled to nanophotonics devices offer a promising route toward scalable quantum networks and integrated quantum technologies. However, the close proximity of Rydberg atoms to dielectric nanostructures makes these systems particularly susceptible to uncontrolled surface electric fields that can lead to a degradation of the excitation process. Here, we experimentally investigate Rydberg excitation of laser-cooled 87^{87}87Rb atoms via the evanescent field of an optical nanofiber in the presence of fiber-guided red- and blue-detuned light fields as used to trap ground state atoms in fiber-based dipole traps. We observe a time evolution of the Rydberg excitation spectrum when both the dipole trapping fields are on and the additional spectral features that appear can be suppressed by applying an external oscillating electric field to the system, strongly indicating that surface charge accumulation is responsible for the observed spectral feature. The experimental results are reproduced qualitatively by a model that incorporates DC energy level shifts arising from electric fields generated by charges deposited on the nanofiber surface. We identify Rydberg-ground state collisional ionization, which is enhanced by the dipole trapping fields, as the dominant mechanism for charge generation. These results provide new insight into charge dynamics at dielectric nanophotonic interfaces and establish practical guidelines for mitigating surface charge-induced electric fields in fiber-integrated Rydberg quantum systems.
The ionization of xenon Rydberg atoms at metallic surfaces is examined. The data show that, when the effects of stray electric "patch" fields present on the surface are taken into account, ionization is well described by a simple over-the-barrier model. The patch fields are determined from direct measurements of the potential variations across the target surfaces using Kelvin probe force microscopy. Monte Carlo techniques are used to model the atom-surface interaction. The results confirm the important role that patch fields can play during Rydberg atom-surface interactions and suggest that such interactions can provide a sensitive probe of stray fields at surfaces. To demonstrate this, measurements of the threshold conditions required to observe ions resulting from surface ionization are used to estimate how large such stray fields can be. The data show that the stray fields can be sizable, as large as ∼ 10 3 V · cm -1 100 nm from the surface and ∼ 10 V · cm -1 500 nm from the surface, and illustrate the potential of Rydberg atoms for detecting and characterizing surface electric fields. Methods to enhance the surface ionization signal using electrode arrays patterned on a surface are investigated. Simulations show that bias voltages applied to a series of parallel wires comprised of two interleaved comb-shaped electrodes can have a dramatic impact on ion collection efficiency. It is suggested that such a surface can be used to efficiently collect low- n Rydberg atoms ( n [Special characters omitted.] 10). Significant progress towards fabrication of a functioning surface of 1 μm wide wires with 1 μm spacing is documented.
Experiments handling Rydberg atoms near surfaces must necessarily deal with the high sensitivity of Rydberg atoms to (stray) electric fields that typically emanate from adsorbates on the surface. We demonstrate a method to modify and reduce the stray electric field by changing the adsorbate distribution. We use one of the Rydberg excitation lasers to locally affect the adsorbed dipole distribution. By adjusting the averaged exposure time we change the strength (with the minimal value less than 0.2V/cm0.2\phantom{\rule{0.28em}{0ex}}\mathrm{V}/\mathrm{cm}0.2V/cm at $78\phantom{\rule{0.28em}{0ex}}\ensuremath{\mu}\mathrm{m}$ from the chip) and even the sign of the perpendicular field component. This technique is a useful tool for experiments handling Rydberg atoms near surfaces, including atom chips.