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arXiv:1206.4956 · Journal of Mathematical Physics

Large deviations, central limit, and dynamical phase transitions in the atom maser

Federico Girotti, Merlijn van Horssen, Raffaella Carbone, Mădălin Guţǎ

Published Jun 1, 2022• 7 citations
arXivHTMLPDF

Abstract

The theory of quantum jump trajectories provides a new framework for understanding dynamical phase transitions in open systems. A candidate for such transitions is the atom maser, which for certain parameters exhibits strong intermittency in the atom detection counts and has a bistable stationary state. Although previous numerical results suggested that the “free energy” may not be a smooth function, we show that the atom detection counts satisfy a large deviations principle and, therefore, we deal with a phase crossover rather than a genuine phase transition. We argue, however, that the latter occurs in the limit of an infinite pumping rate. As a corollary, we obtain the central limit theorem for the counting process. The proof relies on the analysis of a certain deformed generator whose spectral bound is the limiting cumulant generating function. The latter is shown to be smooth so that a large deviations principle holds by the Gärtner–Ellis theorem. One of the main ingredients is the Krein–Rutman theory, which extends the Perron–Frobenius theorem to a general class of positive compact semigroups.

DOI
10.1063/5.0078916

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The theory of quantum jump trajectories provides a new framework for understanding dynamical phase transitions in open systems. A candidate for such transitions is the atom maser, which for certain parameters exhibits strong intermittency in the atom detection counts and has a bistable stationary state. Although previous numerical results suggested that the “free energy” may not be a smooth function, we show that the atom detection counts satisfy a large deviations principle and, therefore, we deal with a phase crossover rather than a genuine phase transition. We argue, however, that the latter occurs in the limit of an infinite pumping rate. As a corollary, we obtain the central limit theorem for the counting process. The proof relies on the analysis of a certain deformed generator whose spectral bound is the limiting cumulant generating function. The latter is shown to be smooth so that a large deviations principle holds by the Gärtner–Ellis theorem. One of the main ingredients is the Krein–Rutman theory, which extends the Perron–Frobenius theorem to a general class of positive compact semigroups.
Quantum Markov processes are widely used models of the dynamics open quantum systems, a fundamental topic in theoretical and mathematical physics with important applications in experimental realisations of quantum systems such as ultracold atomic gases and new quantum information technologies such as quantum metrology and quantum control. In this thesis we present a mathematical framework which effectively characterises dynamical phase transitions in quantum Markov processes, using the theory of large deviations, by combining insights developed in non-equilibrium dynamics with techniques from quantum information and probability. We provide a natural decomposition for quantum Markov chains into phases, paving the way for the rigorous treatment of critical features of such systems such as phase transitions and phase purification. A full characterisation of dynamical phase transitions beyond properties of the steady state is described in terms of a dynamical perspective through critical behaviour of the quantum jump trajectories. We extend a fundamental result from large deviations for classical Markov chains, the Sanov theorem, to a quantum setting; we prove this Sanov theorem for the output of quantum Markov chains, a result which could be extended to a quantum Donsker-Varadhan theory. We perform an in-depth analysis of the atom maser, an infinite-dimensional quantum Markov process exhibiting various types of critical behaviour: for certain parameters it exhibits strong intermittency in the atom detection counts, and has a bistable stationary state. We show that the atom detection counts satisfy a large deviations principle, and therefore we deal with a phase cross-over rather than a genuine phase transition, although the latter occurs in the limit of infinite pumping rate. As a corollary, we obtain the Central Limit Theorem for the counting process.
We use high-order cumulants to investigate the Lee-Yang zeros of generating functions of dynamical observables in open quantum systems. At long times the generating functions take on a large-deviation form with singularities of the associated cumulant generating functions-or dynamical free energies-signifying phase transitions in the ensemble of dynamical trajectories. We consider a driven three-level system as well as the dissipative Ising model. Both systems exhibit dynamical intermittency in the statistics of quantum jumps. From the short-time behavior of the dynamical Lee-Yang zeros, we identify critical values of the counting field which we attribute to the observed intermittency and dynamical phase coexistence. Furthermore, for the dissipative Ising model we construct a trajectory phase diagram and estimate the value of the transverse field where the stationary state changes from being ferromagnetic (inactive) to paramagnetic (active).
In this paper, we consider the statistics of repeated measurements on the output of a quantum Markov chain. We establish a large deviations result analogous to Sanov’s theorem for the multi-site empirical measure associated to finite sequences of consecutive outcomes of a classical stochastic process. Our result relies on the construction of an extended quantum transition operator (which keeps track of previous outcomes) in terms of which we compute moment generating functions, and whose spectral radius is related to the large deviations rate function. As a corollary to this, we obtain a central limit theorem for the empirical measure. Such higher level statistics may be used to uncover critical behaviour such as dynamical phase transitions, which are not captured by lower level statistics such as the sample mean. As a step in this direction, we give an example of a finite system whose level-1 (empirical mean) rate function is independent of a model parameter while the level-2 (empirical measure) rate is not.
We study the dynamics of the single-atom maser, or micromaser, by means of the recently introduced method of thermodynamics of quantum jump trajectories. We find that the dynamics of the micromaser displays multiple space-time phase transitions, i.e., phase transitions in ensembles of quantum jump trajectories. This rich dynamical phase structure becomes apparent when trajectories are classified by dynamical observables that quantify dynamical activity, such as the number of atoms that have changed state while traversing the cavity. The space-time transitions can be either first order or continuous, and are controlled not just by standard parameters of the micromaser but also by nonequilibrium "counting" fields. We discuss how the dynamical phase behavior relates to the better known stationary-state properties of the micromaser.
We apply the large-deviation method to study trajectories in dissipative quantum systems. We show that in the long time limit the statistics of quantum jumps can be understood from thermodynamic arguments in terms of dynamical phases and transitions between them in trajectory space. We illustrate our approach with three simple examples: a driven 2-level system where we find a particular scale invariance point in the ensemble of trajectories of emitted photons; a blinking 3-level system, where we argue that intermittency in the photon count is related to a crossover between distinct dynamical phases; and a micromaser, where we find an actual first-order phase transition in the ensemble of trajectories.
We describe how to characterize dynamical phase transitions in open quantum systems from a purely dynamical perspective, namely, through the statistical behavior of quantum jump trajectories. This approach goes beyond considering only properties of the steady state. While in small quantum systems dynamical transitions can only occur trivially at limiting values of the controlling parameters, in many-body systems they arise as collective phenomena and within this perspective they are reminiscent of thermodynamic phase transitions. We illustrate this in open models of increasing complexity: a three-level system, the micromaser, and a dissipative version of the quantum Ising model. In these examples dynamical transitions are accompanied by clear changes in static behavior. This is however not always the case, and, in general, dynamical phases need to be uncovered by observables which are strictly dynamical, e.g., dynamical counting fields. We demonstrate this via the example of a class of models of dissipative quantum glasses, whose dynamics can vary widely despite having identical (and trivial) stationary states.