The liquid and crystal phases of a single-component Fermi gas with dipolar interactions are investigated using quantum Monte Carlo methods in two spatial dimensions and at zero temperature. The dipoles are oriented by an external field perpendicular to the plane of motion, resulting in a purely repulsive 1/r(3) interaction. In the liquid phase we calculate the equation of state as a function of the interaction strength and other relevant properties characterizing the Fermi-liquid behavior: effective mass, discontinuity at the Fermi surface, and pair correlation function. In the high density regime we calculate the equation of state of the Wigner crystal phase and the critical density of the liquid to solid quantum phase transition. Close to the freezing density we also search for the existence of a stripe phase, but such a phase is never found to be energetically favorable.
The liquid and crystal phases of a single-component Fermi gas with dipolar interactions are investigated using quantum Monte Carlo methods in two spatial dimensions and at zero temperature. The dipoles are oriented by an external field perpendicular to the plane of motion, resulting in a purely repulsive 1/r(3) interaction. In the liquid phase we calculate the equation of state as a function of the interaction strength and other relevant properties characterizing the Fermi-liquid behavior: effective mass, discontinuity at the Fermi surface, and pair correlation function. In the high density regime we calculate the equation of state of the Wigner crystal phase and the critical density of the liquid to solid quantum phase transition. Close to the freezing density we also search for the existence of a stripe phase, but such a phase is never found to be energetically favorable.
Density-functional theory is utilized to investigate the zero-temperature transition from a Fermi liquid to an inhomogeneous stripe, or Wigner crystal phase, predicted to occur in a one-component, spin-polarized, two-dimensional dipolar Fermi gas. Correlations are treated semiexactly within the local-density approximation using an empirical fit to quantum Monte Carlo data. We find that the inclusion of the nonlocal contribution to the Hartree-Fock energy is crucial for the onset of an instability to an inhomogeneous density distribution. Our density-functional theory supports a transition to both a one-dimensional stripe phase and a triangular Wigner crystal. However, we find that there is an instability first to the stripe phase, followed by a transition to the Wigner crystal at higher coupling.
The liquid-to-ordered phase transition in a bilayer system of fermions is studied within the context of our recently proposed density-functional theory [B. P. van Zyl, W. Kirkby, and W. Ferguson, Phys. Rev. A 92, 023614 (2015)]. In each two-dimensional layer, the fermions interact via a repulsive, isotropic dipolar interaction. The presence of a second layer introduces an attractive interlayer interaction, thereby allowing the presence of inhomogeneous density phases which would otherwise be energetically unfavorable. For any fixed layer separation, we find an instability to a commensurate one-dimensional stripe phase in each layer, which always precedes the formation of a triangular Wigner crystal. However, at a certain fixed coupling, tuning the separation can lead to the system favoring a commensurate triangular Wigner crystal, or one-dimensional stripe phase, completely bypassing the Fermi liquid state. While other crystalline symmetries, with energies lower than the liquid phase can be found, they are never allowed to form owing to their high energetic cost relative to the triangular Wigner crystal and stripe phase.
We study a two-component mixture of fermionic dipoles in two dimensions at zero temperature, interacting via a purely repulsive 1/r3 potential. This model can be realized with ultracold atoms or molecules when their dipole moments are aligned in the confinement direction orthogonal to the plane. We characterize the unpolarized mixture by means of the diffusion Monte Carlo technique. Computing the equation of state, we identify the regime of validity for a mean-field theory based on a low-density expansion and compare our results with the hard-disk model of repulsive fermions. At high density, we address the possibility of itinerant ferromagnetism, namely, whether the ground state can be fully polarized in the fluid phase. Within the fixed-node approximation, we show that the accuracy of Jastrow-Slater trial wave functions, even with the typical two-body backflow correction, is not sufficient to resolve the relevant energy differences. By making use of the iterative-backflow improved trial wave functions, we observe no signature of a fully polarized ground state up to the freezing density.
The rapid progress in the production and cooling of molecular gases indicates that experimental studies of quantum gases with a strong dipolar interaction is soon within reach. Dipolar gases are predicted to exhibit very rich physics including quantum liquid crystal phases such as density waves as well as superfluid phases, both of which play an important role for our understanding of strongly correlated systems. Here, we investigate the zero temperature properties of the density-wave phase of a two-dimensional (2D) system of fermionic dipoles using a conserving Hartree-Fock theory. We calculate the amplitude of the density waves as a function of the dipole moment and orientation with respect to the 2D plane. The stripes give rise to a 1D Brillouin zone structure, and the corresponding quasiparticle spectrum is shown to have gapped as well as gapless regions around the Fermi surface. As a result, the system remains compressible in the density-wave phase, and it collapses for strong attraction. We show that the density waves have clear signatures in the momentum distribution and in the momentum correlations. Both can be measured in time-of-flight experiments. Finally, we discuss how the striped phase can be realized with experimentally available systems.
Motivated by the search for quantum liquid crystal phases in a gas of ultracold atoms and molecules, we study the density-wave and nematic instabilities of dipolar fermions on the two-dimensional square lattice (in the $x\text{\ensuremath{-}}y$ plane) with dipoles pointing to the z direction. We determine the phase diagram using two complementary methods, the Hartree-Fock mean-field theory and the linear-response analysis of compressibility. Both give consistent results. In addition to the staggered $(\ensuremath{\pi},\ensuremath{\pi})$ density wave, over a finite range of densities and hopping parameters, the ground state of the system first becomes nematic and then smectic, when the dipolar interaction strength is increased. Both phases are characterized by the same broken fourfold (C4) rotational symmetry. The difference is that the nematic phase has a closed Fermi surface but the smectic does not. The transition from the nematic to the smectic phase is associated with a jump in the nematic order parameter. This jump is closely related to the Van Hove singularities. We derive the kinetic equation for collective excitations in the normal isotropic phase and find that the zero sound mode is strongly Landau damped and thus is not a well-defined excitation. Experimental implications of our results are discussed.
We study Fermi-liquid properties of a weakly interacting two-dimensional gas of single-component fermionic polar molecules with dipole moments d oriented perpendicularly to the plane of their translational motion. This geometry allows the minimization of inelastic losses due to chemical reactions for reactive molecules and, at the same time, provides a possibility of a clear description of many-body (beyond mean-field) effects. The long-range character of the dipole-dipole repulsive interaction between the molecules, which scales as 1/r3 at large distances r, makes the problem drastically different from the well-known problem of the two-species Fermi gas with repulsive contact interspecies interaction. We solve the low-energy scattering problem and develop a many-body perturbation theory beyond the mean field. The theory relies on the presence of a small parameter kFr∗, where kF is the Fermi momentum and ${r}_{*}=m{d}^{2}/{\ensuremath{\hbar}}^{2}$ is the dipole-dipole length, with m being the molecule mass. We obtain thermodynamic quantities as a series of expansion up to the second order in kFr∗ and argue that many-body corrections to the ground-state energy can be identified in experiments with ultracold molecules, as it has been recently done for ultracold fermionic atoms. Moreover, we show that only many-body effects provide the existence of zero sound and calculate the sound velocity.