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arXiv:1206.3213 · Physical Review A

Superradiant phase transitions with three-level systems

Alexandre Baksic, Pierre Nataf, Cristiano Ciuti

Published Feb 13, 2013• 51 citations
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Abstract

We determine the phase diagram of $N$ identical three-level systems interacting with a single photonic mode in the thermodynamical limit ($N\ensuremath{\rightarrow}\ensuremath{\infty}$) by accounting for the so-called diamagnetic term and the inequalities imposed by the Thomas-Reich-Kuhn (TRK) oscillator strength sum rule. The key role of transitions between excited levels and the occurrence of first-order phase transitions is discussed. We show that, in contrast to two-level systems, in the three-level case the TRK inequalities do not always prevent a superradiant phase transition in the presence of a diamagnetic term.

DOI
10.1103/physreva.87.023813

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We determine the phase diagram of NNN identical three-level systems interacting with a single photonic mode in the thermodynamical limit (N\ensuremath→\ensuremath∞N\ensuremath{\rightarrow}\ensuremath{\infty}N\ensuremath→\ensuremath∞) by accounting for the so-called diamagnetic term and the inequalities imposed by the Thomas-Reich-Kuhn (TRK) oscillator strength sum rule. The key role of transitions between excited levels and the occurrence of first-order phase transitions is discussed. We show that, in contrast to two-level systems, in the three-level case the TRK inequalities do not always prevent a superradiant phase transition in the presence of a diamagnetic term.
We consider an ensemble of three-level particles in Lambda configuration interacting with two bosonic modes. The Hamiltonian has the form of a generalized Dicke model. We show that in the thermodynamic limit this model supports a superradiant quantum phase transition. Remarkably, this can be both a first- and a second-order phase transition. A connection of the phase diagram to the symmetries of the Hamiltonian is also given. In addition, we show that this model can describe atoms interacting with an electromagnetic field in which the microscopic Hamiltonian includes a diamagnetic contribution. Even though the parameters of the atomic system respect the Thomas-Reiche-Kuhn sum rule, the system still shows a superradiant phase transition.
In this doctoral thesis, the thermodynamic phases und phase transitions of a generalised Dicke model are studied and characterised. Both, finite and vanishing temperatures are considered. The Dicke model of quantum optics describes collective phenomena which occur when light interacts with a many-atom system. In the thermodynamic limit, a so-called Hepp–Lieb superradiant phase transition sets in. A superradiant phase develops for low temperatures or strong coupling between light and atoms, which is characterised by a macroscopic excitation of the light field and a spontaneous, collective polarisation of the atoms. This thesis discusses a generalised version of the Dicke model, which is described by a quantum mechanical system consisting of three-level atoms in Lambda-configuration and two modes of a resonator. By means of the Holstein–Primakoff transformation, the Hamiltonian of this system is written in terms of four interacting, non-linear oscillators, which can be linearised in the thermodynamic limit, yielding the ground-state energy as well as the low-energy excitations. The phase diagram consisting of two superradiant phases separated by continuous and first-order phase transitions is derived. In order to clarify the question whether or not the superradiant phase transition of this generalised Dicke model can be observed experimentally for real atoms, the significance of the diamagnetic term is discussed. In contrast to the original Dicke model, superradiant phase transitions are possible in principle. This is due to the first-order phase transitions. In addition, a no-go theorem for continuous superradiant phase transitions is presented. The argument is based on the Thomas–Reiche–Kuhn sum rule. Last, we study the superradiant phase transition of the generalised Dicke model at finite temperatures. Therefore, the partition sum is computed and analysed in the thermodynamic limit using Laplace’s method. At finite temperatures, the properties of the phase diagram and phases remain. However, here all phase transitions are of first order.
The controllability of current quantum technologies allows one to implement spin-boson models where two-photon couplings are the dominating terms of light-matter interaction. In this case, when the coupling strength becomes comparable with the characteristic frequencies, a spectral collapse can take place, i.e., the discrete system spectrum can collapse into a continuous band. Here, we analyze the thermodynamic limit of the two-photon Dicke model, which describes the interaction of an ensemble of qubits with a single bosonic mode. We find that there exists a parameter regime where two-photon interactions induce a superradiant phase transition, before the spectral collapse occurs. Furthermore, we extend the mean-field analysis by considering second-order quantum fluctuation terms, in order to analyze the low-energy spectrum and compare the critical behavior with the one-photon case.
Entanglement and quantum correlations between atoms are not usually considered key ingredients of the superradiant phase transition. Here we consider the Tavis-Cummings model, a solvable system of two-levels atoms, coupled with a single-mode quantized electromagnetic field. This system undergoes a superradiant phase transition, even in a finite-size framework, accompanied by a spontaneous symmetry breaking, and an infinite sequence of energy level crossings. We find approximated expressions for the ground state, its energy, and the position of the level crossings, valid in the limit of a very large number of photons with respect to that of the atoms. In that same limit, we find that the number of photons scales quadratically with the coupling strength, and linearly with the system size, providing a new insight into the superradiance phenomenon. Resorting to novel multipartite measures, we then demonstrate that this quantum phase transition is accompanied by a crossover in the quantum correlations and entanglement between the atoms (qubits). The latters therefore represent suited order parameters for this transition. Finally, we show that these properties of the quantum phase transition persist in the thermodynamic limit.
Entanglement and quantum correlations between atoms are not usually considered key ingredients of the superradiant phase transition. Here we consider the Tavis−Cummings model, a solvable system of two-levels atoms, coupled with a single-mode quantized electromagnetic field. This system undergoes a superradiant phase transition, even in a finite-size framework, accompanied by a spontaneous symmetry breaking, and an infinite sequence of energy level crossings. We find approximated expressions for the ground state, its energy, and the position of the level crossings, valid in the limit of a very large number of photons with respect to that of the atoms. In that same limit, we find that the number of photons scales quadratically with the coupling strength, and linearly with the system size, providing a new insight into the superradiance phenomenon. Resorting to novel multipartite measures, we then demonstrate that this quantum phase transition is accompanied by a crossover in the quantum correlations and entanglement between the atoms (qubits). The latters therefore represent suited order parameters for this transition. Finally, we show that these properties of the quantum phase transition persist in the thermodynamic limit.