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arXiv:1205.6985 · Physical Review A

Spin squeezing and Schrödinger-cat-state generation in atomic samples with Rydberg blockade

Tomáš Opatrný, Klaus Mølmer

Published Aug 27, 2012• 33 citations
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Abstract

A scheme is proposed to prepare squeezed states and Schr\"odinger-cat-like states of the collective spin degrees of freedom associated with a pair of ground states in an atomic ensemble. The scheme uses an effective Jaynes-Cummings interaction which can be provided by excitation of the atoms to Rydberg states and an effective ${J}_{x}$ interaction implemented by a resonant Raman coupling between the atomic ground states. Dynamical evolution both with a constant Hamiltonian and with adiabatic variation of the two interaction terms is studied. We show that by the application of further resonant laser fields, we can suppress nonadiabatic transfer under the time-varying Hamiltonian and significantly speed up the evolution towards a maximally squeezed, ${J}_{z}=0$, collective spin state.

DOI
10.1103/physreva.86.023845

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A scheme is proposed to prepare squeezed states and Schr"odinger-cat-like states of the collective spin degrees of freedom associated with a pair of ground states in an atomic ensemble. The scheme uses an effective Jaynes-Cummings interaction which can be provided by excitation of the atoms to Rydberg states and an effective Jx{J}_{x}Jx​ interaction implemented by a resonant Raman coupling between the atomic ground states. Dynamical evolution both with a constant Hamiltonian and with adiabatic variation of the two interaction terms is studied. We show that by the application of further resonant laser fields, we can suppress nonadiabatic transfer under the time-varying Hamiltonian and significantly speed up the evolution towards a maximally squeezed, Jz=0{J}_{z}=0Jz​=0, collective spin state.
We show that the interaction between Rydberg atomic states can provide continuous spin squeezing of atoms with two ground states. The interaction prevents the simultaneous excitation of more than a single atom in the sample to the Rydberg state, and we propose to utilize this blockade effect to realize an effective collective spin Hamiltonian ${J}_{x}^{2}\ensuremath{-}{J}_{y}^{2}.$ With this Hamiltonian the quantum-mechanical uncertainty of the spin variable ${J}_{x}\ensuremath{-}{J}_{y}$ can be significantly reduced.
The realization of a Jaynes-Cummings model in the optical domain is proposed for an atomic ensemble. The scheme exploits the collective coupling of the atoms to a quantized cavity mode and the nonlinearity introduced by coupling to high-lying Rydberg states. A two-photon transition resonantly couples the single-atom ground state $|g\ensuremath{\rangle}$ to a Rydberg state $|e\ensuremath{\rangle}$ via a nonresonant intermediate state $|i\ensuremath{\rangle}$, but due to the interaction between Rydberg atoms only a single atom can be resonantly excited in the ensemble. This restricts the state space of the ensemble to the collective ground state $|G\ensuremath{\rangle}$ and the collectively excited state $|E\ensuremath{\rangle}$ with a single Rydberg excitation distributed evenly on all atoms. The collectively enhanced coupling of all atoms to the cavity field with coherent coupling strengths which are much larger than the decay rates in the system leads to the strong coupling regime of the resulting effective Jaynes-Cummings model. We use numerical simulations to show that the cavity transmission can be used to reveal detailed properties of the Jaynes-Cummings ladder of excited states and that the atomic nonlinearity gives rise to highly nontrivial photon emission from the cavity. Finally, we suggest that the absence of interactions between remote Rydberg atoms may, due to a combinatorial effect, induce a cavity-assisted excitation blockade whose range is larger than the typical Rydberg dipole-dipole interaction length.
We propose to apply stimulated adiabatic passage to transfer atoms from their ground state into Rydberg excited states. Atoms a few micrometers apart experience a dipole-dipole interaction among Rydberg states that is strong enough to shift the atomic resonance and inhibit excitation of more than a single atom. We show that the adiabatic passage in the presence of this interaction between two atoms leads to robust creation of maximally entangled states and to two-bit quantum gates. For many atoms, the excitation blockade leads to an effective implementation of collective-spin and Jaynes-Cummings-like Hamiltonians, and we show that the adiabatic passage can be used to generate collective J_{x}=0 eigenstates and Greenberger-Horne-Zeilinger states of tens of atoms.
We generate spin squeezed ground states in an atomic spin-1 Bose-Einstein condensate tuned near the quantum-critical point separating the different spin phases of the interacting ensemble using a novel nonadiabatic technique. In contrast to typical nonequilibrium methods for preparing atomic squeezed states by quenching through a quantum phase transition, squeezed ground states are time stationary with a constant quadrature squeezing angle. A squeezed ground state with 6-8 dB of squeezing and a constant squeezing angle is demonstrated. The long-term evolution of the squeezed ground state is measured and shows gradual decrease in the degree of squeezing over 2 s that is well modeled by a slow tuning of the Hamiltonian due to the loss of atomic density. Interestingly, modeling the gradual decrease does not require additional spin decoherence models despite a loss of 75% of the atoms.
The generation of entanglement in atomic systems plays a central topic in the fields of quantum information storage and processing. Moreover, a special category of entangled states of multi-atom ensembles, spin squeezed states, have been proven to lead to considerable improvement in the sensitivity of precision measurements compared to systems involving uncorrelated atoms. A treatment of entanglement in open systems is, however, incomplete without a precise description of the process of decoherence which necessarily accompanies it. The theory of entanglement and decoherence are the two main topics of this thesis. Methods are described for the generation of strong correlations in large atomic ensembles using either cavity quantum electrodynamics or measurement outcome conditioned quantum dynamics. Moreover, the description of loss of entanglement resulting from the coupling to a noise reservoir (electromagnetic vacuum) is explored. A spin squeezing parameter is used throughout this thesis as both a measure of entanglement strength and as an indication of the sensitivity improvement above the so-called standard quantum limit (sensitivity obtained with uncorrelated particles) in metrology. The first scheme considered consists of a single mode cavity field interacting with a collection of atoms for which spin squeezing is produced in both resonant and off-resonant regimes. In the resonant case, transfer of squeezing from a field state to the atoms is analyzed, while in the off-resonant regime squeezing is produced via an effective nonlinear interaction (one-axis twisting Hamiltonian). A second, more experimentally realistic case, is one involving the interaction of free space atoms with laser pulses; a projective measurement of a source field originating from atomic fluctuations provides a means of preparing atomic collective states such as spin squeezed and Schrodinger cat states. A new unravelling is proposed, that employs the detection of photon number in a single output channel and is capable of producing mesoscopic Schrodinger cat states in a single step. As a first step to understanding the role of cooperative decoherence, of importance in the case of dense pencil-shaped atomic ensembles, the collective spin decoherence of a two multilevel atom system is derived. This calculation is also relevant to entanglement loss for two qubits manipulated using with reading/writing pulses. Finally, a scheme is proposed in which arbitrarily strong entanglement can be produced in a four-wave mixing setup, where the preparation of the atoms in a dark state limits the decoherence to negligible values.