We report on controlled doping of an ultracold Rb gas with single neutral Cs impurity atoms. Elastic two-body collisions lead to a rapid thermalization of the impurity inside the Rb gas, representing the first realization of an ultracold gas doped with a precisely known number of impurity atoms interacting via s-wave collisions. Inelastic interactions are restricted to a single three-body recombination channel in a highly controlled and pure setting, which allows us to determine the Rb-Rb-Cs three-body loss rate with unprecedented precision. Our results pave the way for a coherently interacting hybrid system of individually controllable impurities in a quantum many-body system.
We report on controlled doping of an ultracold Rb gas with single neutral Cs impurity atoms. Elastic two-body collisions lead to a rapid thermalization of the impurity inside the Rb gas, representing the first realization of an ultracold gas doped with a precisely known number of impurity atoms interacting via s-wave collisions. Inelastic interactions are restricted to a single three-body recombination channel in a highly controlled and pure setting, which allows us to determine the Rb-Rb-Cs three-body loss rate with unprecedented precision. Our results pave the way for a coherently interacting hybrid system of individually controllable impurities in a quantum many-body system.
Abstract We report on the experimental doping of a 87 Rubidium (Rb) Bose–Einstein condensate (BEC) with individual neutral 133 Cesium (Cs) atoms. We discuss the experimental tools and procedures to facilitate Cs-Rb interaction. First, we use degenerate Raman side-band cooling of the impurities to enhance the immersion efficiency for the impurity in the quantum gas. We identify the immersed fraction of Cs impurities from the thermalization of Cs atoms upon impinging on a BEC, where elastic collisions lead to a localization of Cs atoms in the Rb cloud. Second, further enhancement of the immersion probability is obtained by localizing the Cs atoms in a species-selective optical lattice and a subsequent transport into the Rb cloud. Here, impurity-BEC interaction is monitored by position and time-resolved three-body loss of Cs impurities immersed into the BEC. This combination of experimental methods allows for the controlled doping of a BEC with neutral impurity atoms, paving the way to impurity aided probing and coherent impurity-quantum bath interaction.
Recent studies on the dynamics of single, neutral impurities immersed in an ultracold gas are reviewed. This paradigmatic model system is realized by the controlled doping of single Caesium atoms into an ultracold Rubidium gas. Interaction between the impurity and the gas in both the motional and internal degrees of freedom is studied for a broad range of bath temperatures in the thermal and quantum‐degenerate regime. Tracing single‐atom diffusion it is found that, even for a granular bath, where the assumption of a continuous medium is not fulfilled, a modified Langevin equation yields excellent predictions for tracer diffusion. Numerical modeling of impurity dynamics in a three‐dimensional superfluid bath shows the emergence of a prethermalized state for intermediate times due to the existence of a superfluid critical momentum, while for lower dimensions the effect of thermal phonons dominates and obstructs the formation of such nonthermal states. Finally, unleashing the quasi‐spin degree of freedom, the authors observe and control spin‐exchange dynamics between individual impurities and the bath. Moreover, a regime of sympathetic impurity cooling is realized, where the internal‐state coherence of the impurity is preserved. In the future, control over the motional and spin‐degree of freedom will enable using individual impurities as thermalized, localized, minimally invasive quantum probes for a quantum fluid.
We report on spin dynamics of individual, localized neutral impurities immersed in a Bose-Einstein condensate. Single cesium atoms are transported into a cloud of rubidium atoms and thermalize with the bath, and the ensuing spin exchange between localized impurities with quasispin F_{i}=3 and bath atoms with F_{b}=1 is resolved. Comparing our data to numerical simulations of spin dynamics, we find that, for gas densities in the Bose-Einstein condensate regime, the dynamics is dominated by the condensed fraction of the cloud. We spatially resolve the density overlap of impurities and gas by the spin population of impurities. Finally, we trace the coherence of impurities prepared in a coherent superposition of internal states when coupled to a gas of different densities. For our choice of states, we show that, despite high bath densities and, thus, fast thermalization rates, the impurity coherence is not affected by the bath, realizing a regime of sympathetic cooling while maintaining internal state coherence. Our work paves the way toward the nondestructive probing of quantum many-body systems via localized impurities.
We employ collisions of individual atomic cesium (Cs) impurities with an ultracold rubidium (Rb) gas to probe atomic interaction with hyperfine- and Zeeman-state sensitivity. Controlling the Rb bath's internal state yields access to novel phenomena observed in interatomic spin exchange. These can be tailored at ultralow energies, owing to the excellent experimental control over all relevant energy scales. First, detecting spin-exchange dynamics in the Cs hyperfine-state manifold, we resolve a series of previously unreported Feshbach resonances at magnetic fields below 300 mG, separated by energies as low as h×15 kHz. The series originates from a coupling to molecular states with binding energies below h×1 kHz and wave function extensions in the micrometer range. Second, at magnetic fields below ≈100 mG, we observe the emergence of a new reaction path for alkali atoms, where in a single, direct collision between two atoms two quanta of angular momentum can be transferred. This path originates from the hyperfine analog of dipolar spin-spin relaxation. Our work yields control of subtle ultralow-energy features of atomic collision dynamics, opening new routes for advanced state-to-state chemistry, for controlling spin exchange in quantum many-body systems for solid-state simulations, or for determination of high-precision molecular potentials.
We analyze reactive collisions of a single Ba+ ion in contact with an ultracold gas of Rb atoms at low three-body collision energies of 2.2(9) $\mathrm{mK}\ifmmode\times\else\texttimes\fi{}{k}_{\mathrm{B}}$. Mapping out the Ba+ loss rate dependence on the Rb atom density we can discern two-body reactive collisions from three-body ones and determine both rate coefficients, which are ${k}_{2}=3.1(6)(6)\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}13}\phantom{\rule{0.28em}{0ex}}{\mathrm{cm}}^{3}\phantom{\rule{0.16em}{0ex}}{\mathrm{s}}^{\ensuremath{-}1}$ and ${k}_{3}=1.04(4)(45)\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}24}\phantom{\rule{0.28em}{0ex}}{\mathrm{cm}}^{6}\phantom{\rule{0.16em}{0ex}}{\mathrm{s}}^{\ensuremath{-}1}$, respectively (statistical and systematic errors in parentheses). Thus, the measured ternary recombination dominates over binary reactions even at moderate atom densities of $n\ensuremath{\approx}{10}^{12}\phantom{\rule{0.28em}{0ex}}{\mathrm{cm}}^{\ensuremath{-}3}$. The results for Ba+ and Rb are representative for a wide range of cold ion-atom systems and can serve as guidance for the future development of the field of hybrid atom-ion research.
Over the recent years a new research field emerged that combines technologies for cooling and trapping of neutral atoms and charged ions in one experimental apparatus. These atom-ion hybrid traps enable the investigation of atom-ion interactions at unprecedentedly low collision energies targeting the ultracold s-wave regime. In this thesis I report on experiments performed in an hybrid atom-ion apparatus combining single Ba^+ or Rb^+ ions with ultracold neutral Rb atoms. The main focus of this work is studying the emerging three-body reaction dynamics in a cold charged gas. First, I will present measurements investigating cold reactions in the hetero-nuclear Ba^+ - Rb system. So far, most theoretical and experimental studies have been dealing with reactions between two particles. However, we find that three-body reactions already dominate over two-body ones at atomic densities down to 10^{−11} cm^{−3} once collision energies are in the low mK regime. We then investigate the energy scaling of inelastic ternary collisions between an ion and two atoms. A power-law scaling of the three-body rate coefficient is predicted by theory. We find agreement with the experiment if we include the ion’s kinetic energy distribution that we access numerically. The next study elaborates on the very first observation of ternary reactions in a hybrid cold atom-ion setup. For this we immerse a single Rb^+ ion into ultracold Rb atoms with sufficiently reduced excess micromotion. Occurring reactions are signaled by the creation of highly energetic Rb^+ ions. I will also showcase novel techniques to investigate the atom and the ion system by using the respective other one which were developed by us over the course of the last years. In order to reduce the total ion kinetic energy in a Paul trap one has to compensate the ion’s excess micromotion. This is routinely being done by analyzing the ion’s fluorescence. By observing collision energy dependent elastic atom-ion collisions in an ultracold atom cloud we directly infer the ion’s micromotion energy. This way we can perform atom-ion experiments with optically dark Rb^+ ions and good excess micromotion. Without the need of visible laser light for micromotion compensation we are able to investigate the evolution of quasi-static stray electric fields in a Paul trap over a period of several months. The last study I will present is targeted at neutral Rb only. There, we spectroscopically access the molecular state distribution of Rb_2 molecules formed in neutral three-body recombination by state-selective ionization of these molecules. Trapping and subsequent detection of these ions is being done with our Paul trap, which has the role of a very sensitive single ion detector in these measurements.