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arXiv:1204.1510 · Physical Review A

Effects of magnetic dipole-dipole interactions in atomic Bose-Einstein condensates with tunable s -wave interactions

Abraham J. Olson, Daniel Whitenack, Yong P. Chen

Published Oct 8, 2013• 28 citations
arXivHTMLPDF

Abstract

The $s$-wave interaction is usually the dominant form of interactions in atomic Bose-Einstein condensates (BECs). Recently, Feshbach resonances have been employed to reduce the strength of the $s$-wave interaction in many atomic species. This opens the possibilities to study magnetic dipole-dipole interactions (MDDIs) in BECs, where the novel physics resulting from long-range and anisotropic dipolar interactions can be explored. Using a variational method, we study the effect of MDDIs on the statics and dynamics of atomic BECs with tunable $s$-wave interactions for a variety of species, including both nonalkali metals with large magnetic dipole moments (${}^{52}$Cr, ${}^{164}$Dy, ${}^{168}$Er) and alkali metals (with much smaller magnetic dipole moments). A parameter of magnetic Feshbach resonances, ${\ensuremath{\epsilon}}_{dd,\text{max}}$, is used to quantitatively indicate the feasibility of experimentally observing MDDI effects in different atomic species. We find that strong MDDI effects should be observable in both in-trap and time-of-flight behaviors, not only for the strongly magnetic dipolar species but also for the alkali-metal BECs of ${}^{7}$Li, ${}^{39}$K, and ${}^{133}$Cs. In addition, we predict several effects which should be experimentally observable. Our results provide a helpful guide for experimentalists to realize and study atomic dipolar quantum gases.

DOI
10.1103/physreva.88.043609

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The sss-wave interaction is usually the dominant form of interactions in atomic Bose-Einstein condensates (BECs). Recently, Feshbach resonances have been employed to reduce the strength of the sss-wave interaction in many atomic species. This opens the possibilities to study magnetic dipole-dipole interactions (MDDIs) in BECs, where the novel physics resulting from long-range and anisotropic dipolar interactions can be explored. Using a variational method, we study the effect of MDDIs on the statics and dynamics of atomic BECs with tunable sss-wave interactions for a variety of species, including both nonalkali metals with large magnetic dipole moments (52{}^{52}52Cr, 164{}^{164}164Dy, 168{}^{168}168Er) and alkali metals (with much smaller magnetic dipole moments). A parameter of magnetic Feshbach resonances, \ensuremathϵdd,max{\ensuremath{\epsilon}}_{dd,\text{max}}\ensuremathϵdd,max​, is used to quantitatively indicate the feasibility of experimentally observing MDDI effects in different atomic species. We find that strong MDDI effects should be observable in both in-trap and time-of-flight behaviors, not only for the strongly magnetic dipolar species but also for the alkali-metal BECs of 7{}^{7}7Li, 39{}^{39}39K, and 133{}^{133}133Cs. In addition, we predict several effects which should be experimentally observable. Our results provide a helpful guide for experimentalists to realize and study atomic dipolar quantum gases.
We report on experiments exploring the physics of dipolar quantum gases using a 52 Cr Bose-Einstein condensate (BEC). By means of a Feshbach resonance, it is possible to reduce the effects of short range interactions and reach a regime where the physics is governed by the long-range, anisotropic dipole-dipole interaction between the large (6 µB) magnetic moments of Chromium atoms. Several dramatic effects of the dipolar interaction are observed: the usual inversion of ellipticity of the condensate during time-of flight is inhibited, the stability of the dipolar gas depends strongly on the trap geometry, and the explosion following the collapse of an unstable dipolar condensate displays d-wave like features.
We report on experiments exploring the physics of dipolar quantum gases using a Chromium Bose-Einstein condensate (BEC). By means of a Feshbach resonance, it is possible to reduce the effects of short range interactions and reach a regime where the physics is governed by the long-range, anisotropic dipole-dipole interaction between the large (6μB6 μ_{\rm B}6μB​) magnetic moments of Chromium atoms. Several dramatic effects of the dipolar interaction are observed: the usual inversion of ellipticity of the condensate during time-of flight is inhibited, the stability of the dipolar gas depends strongly on the trap geometry, and the explosion following the collapse of an unstable dipolar condensate displays d-wave like features.
This tutorial presents a detailed discussion of the generation of a Bose–Einstein condensate (BEC) of chromium atoms. This constitutes the first realization of a Bose–Einstein condensate of atoms with strong dipole–dipole interaction. Due to the special electronic and magnetic properties of chromium atoms, standard methods cannot be applied to generate a chromium BEC. The tutorial contains a detailed discussion of the techniques that we use to create the chromium BEC. Compared to all other BECs that have been created so far, chromium atoms have an extraordinarily large magnetic dipole moment and therefore underlie strong magnetic dipole–dipole interaction which is in contrast to the contact interaction that stems from s-wave scattering of the atoms, long-range and anisotropic. A steadily growing number of theoretical publications show that many interesting new phenomena are expected to occur in a 'dipolar' BEC. An experimental investigation of the expansion dynamics of the chromium BEC provides the first experimental proof of a mechanical effect of dipole–dipole interaction in a gas. We describe the condensate by a hydrodynamic model of a superfluid that takes dipole–dipole interaction into account. Our experimental results are in excellent agreement with this theory. We are able to determine the relative strength parameter of the dipole–dipole interaction and deduce the s-wave scattering length of chromium atoms. These two quantities allow us to completely describe the interaction of the atoms in the condensate. The experimental results presented here make the chromium BEC the most promising system for further investigations of dipolar effects in degenerate quantum gases.
Weak dipolar effects in atomic Bose-Einstein condensates (BECs) have recently been predicted to develop spin textures. However, observation of the spin textures requires us to decrease the magnetic field down to approximately 10 microG for spin-1 alkali BECs, so that they are not washed out by the Zeeman effect. We present a scheme to observe the magnetic dipole-dipole interaction in alkali BECs under a realistic magnetic field of approximately 100 mG. Our scheme enables us to extract genuine dipolar effects and should apply also to (52)Cr BECs.
We report on experiments with ultracold chromium atoms. Preparing a cloud of 52Cr atoms in a crossed optical dipole trap (CODT) and applying magnetic fields between 4 and 600 G, we observe 14 Feshbach resonances by the occurrence of increased atom loss at distinct magnetic field values. A comparison with theory taking only dipole–dipole coupling into account shows very good agreement between experimental and theoretical resonance positions and allows us to extract the s-wave scattering lengths a 6=112(14) a 0, a 4= 58(6) a 0, a 2=−7(20) a 0 of the involved molecular potentials as well as the dispersion coefficients C 6= 733(70) au and au. The strongest resonance at 589 G has a calculated width of 1.7 G and reveals a three-body loss coefficient below L 3, max∼3×10−36 m6 s−1. Further evaporative cooling within the CODT leads to the formation of a Bose–Einstein condensate (BEC) with up to 100 000 condensed atoms. The magnetic dipole–dipole interaction between the Cr atoms is so strong that, as a first mechanical manifestation of dipole–dipole interaction, we observe a modification of the condensate expansion which depends on the alignment of the atomic magnetic dipoles with respect to the axis of the CODT. This magnetostrictive effect is in very good agreement with the theory of dipolar quantum gases and shows that a Cr-BEC is an excellent model system to study dipole–dipole interactions in degenerate quantum gases.
We have observed Bose-Einstein condensation of chromium atoms [1], whose large magnetic dipole moment is unique among all species that have been Bose-condensed so far. The arising magnetic forces are of anisotropic and long-range character and therefore introduce a novel type of interaction in the physics of ultracold quantum gases. In addition, it is expected that the character of the interaction present in a chromium BEC can be varied from mainly contact to purely dipolar utilizing one of the recently observed Feshbach resonances in 52Cr-collisions.