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arXiv:1203.4629 · Physical Review E

Temperature crossover of decoherence rates in chaotic and regular bath dynamics

Ángel S. Sanz, Yossi Elran, Paul W. Brumer

Published Mar 30, 2012• 6 citations
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Abstract

The effect of chaotic bath dynamics on the decoherence of a quantum system is examined for the vibrational degrees of freedom of a diatomic molecule in a realistic, constant temperature collisional bath. As an example, the specific case of I(2) in liquid xenon is examined as a function of temperature, and the results compared with an integrable xenon bath. A crossover in behavior is found: The integrable bath induces more decoherence at low bath temperatures than does the chaotic bath, whereas the opposite is the case at the higher bath temperatures. These results, verifying a conjecture due to Wilkie, shed light on the differing views of the effect of chaotic dynamics on system decoherence.

DOI
10.1103/physreve.85.036218

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The effect of chaotic bath dynamics on the decoherence of a quantum system is examined for the vibrational degrees of freedom of a diatomic molecule in a realistic, constant temperature collisional bath. As an example, the specific case of I(2) in liquid xenon is examined as a function of temperature, and the results compared with an integrable xenon bath. A crossover in behavior is found: The integrable bath induces more decoherence at low bath temperatures than does the chaotic bath, whereas the opposite is the case at the higher bath temperatures. These results, verifying a conjecture due to Wilkie, shed light on the differing views of the effect of chaotic dynamics on system decoherence.
We study the effects of dissipation and decoherence induced on a harmonic oscillator by the coupling to a chaotic system with two degrees of freedom. Using the Feynman-Vernon approach and treating the chaotic system semiclassically, we show that the effects of the low-dimensional chaotic environment are in many ways similar to those produced by thermal baths. The classical correlation and response functions play important roles in both classical and quantum formulations. Our results are qualitatively similar to the high-temperature regime of the Caldeira-Leggett model.
We numerically investigate decoherence of a two-spin system (central system) by a bath of many spins 1/2. By carefully adjusting parameters, the dynamical regime of the bath has been varied from quantum chaos to regular, while all other dynamical characteristics have been kept practically intact. We explicitly demonstrate that for a many-body quantum bath, the onset of quantum chaos leads to significantly faster and stronger decoherence compared to an equivalent non-chaotic bath. Moreover, the non-diagonal elements of the system's density matrix, the linear entropy, and the fidelity of the central system decay differently for chaotic and non-chaotic baths. Therefore, knowledge of the basic parameters of the bath (strength of the system-bath interaction, and the bath's spectral density of states) is not always sufficient, and much finer details of the bath's dynamics can strongly affect the decoherence process.
Effective descriptions accounting for the evolution of quantum systems that are acted on by a bath are desirable. As the number of bath degrees of freedom increases and full quantum simulations turn out computationally prohibitive, simpler models become essential to understand and gain an insight into the main physical mechanisms involved in the system dynamics. In this regard, vibrational decoherence of an I2 diatomics is tackled here within the framework of Markovian quantum state diffusion. The I2 dynamics are analyzed in terms of an effective decoherence rate, Λ, and the specific choice of the initial state, in particular, Gaussian wave packets and two-state superpositions. It is found that, for Markovian baths, the relevant quantity regarding decoherence is the product of friction (η) and temperature (T); there is no distinction between varying one or the other. It is also observed that decoherence becomes faster as the energy levels involved in the system state correspond to higher eigenvalues. This effect is due to a population redistribution during the dynamical process and an eventual irreversible loss of the initial coherence. These results have been compared with those available in the literature from more detailed semiclassical IVR simulations, finding a good agreement.
We investigate the decoherence properties of a central system composed of two spins 12 in contact with a spin bath. The dynamical regime of the bath ranges from a fully integrable limit to complete chaoticity. We show that the dynamical regime of the bath determines the efficiency of the decoherence process. For perturbative regimes, the integrable limit provides stronger decoherence, while in the strong coupling regime the chaotic limit becomes more efficient. We also show that the decoherence time behaves in a similar way. On the contrary, the rate of decay of magnitudes like linear entropy or fidelity does not depend on the dynamical regime of the bath. We interpret the latter results as due to a comparable complexity of the Hamiltonian for both the integrable and the fully chaotic limits.
Vibrational decoherence of a "breathing sphere" oscillator in a thermal Lennard-Jones bath is examined using a classical analog approach. The equivalence between this approach and the linearized semiclassical initial value representation (IVR) is established and the method is exploited to produce a useful computational strategy that can efficiently evaluate the time dependence of the decoherence in these systems. A comparison between Harmonic and Morse "breathing sphere" models is presented and the rate of decoherence is found to depend on the choice of model, the initial state of the oscillator, the initial conditions of the bath (temperature, density), and the choice of quantity measuring the decoherence rate. The results are used to examine the utility of the Caldeira-Leggett model in this realistic system.
The well-known increase of the decoherence rate with the temperature, for a quantum system coupled to a linear thermal bath, no longer holds for a different bath dynamics. This is shown by means of a simple classical nonlinear bath, as well as a quantum spin-boson model. The anomalous effect is due to the temperature dependence of the bath spectral profile. In the case of the second model, a link with the quantum Zeno effect is provided. The decoherence reduction via the temperature increase can be relevant for the design of quantum computers.