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arXiv:1202.6361 · Physical Review Letters

Experimental Realization of Plaquette Resonating Valence-Bond States with Ultracold Atoms in Optical Superlattices

Sylvain Nascimbène, Y.-A. Chen, M. Atala, Monika Aidelsburger, Stefan Trotzky, B. Paredes, Immanuel Bloch

Published May 14, 2012• 101 citations
arXivHTMLPDF

Abstract

The concept of valence-bond resonance plays a fundamental role in the theory of the chemical bond and is believed to lie at the heart of many-body quantum physical phenomena. Here we show direct experimental evidence of a time-resolved valence-bond quantum resonance with ultracold bosonic atoms in an optical lattice. By means of a superlattice structure we create a three-dimensional array of independent four-site plaquettes, which we can fully control and manipulate in parallel. Moreover, we show how small-scale plaquette resonating valence-bond (RVB) states with s- and d-wave symmetry can be created and characterized. We anticipate our findings to open the path towards the creation and analysis of many-body RVB states in ultracold atomic gases.

DOI
10.1103/physrevlett.108.205301

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The concept of valence-bond resonance plays a fundamental role in the theory of the chemical bond and is believed to lie at the heart of many-body quantum physical phenomena. Here we show direct experimental evidence of a time-resolved valence-bond quantum resonance with ultracold bosonic atoms in an optical lattice. By means of a superlattice structure we create a three-dimensional array of independent four-site plaquettes, which we can fully control and manipulate in parallel. Moreover, we show how small-scale plaquette resonating valence-bond (RVB) states with s- and d-wave symmetry can be created and characterized. We anticipate our findings to open the path towards the creation and analysis of many-body RVB states in ultracold atomic gases.
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This dissertation summarizes my recent work regarding systems of strongly interacting fermionic atoms in optical lattices. This work addresses the combination of two experimental techniques that have been the subject of much recent research in ultracold atom physics. One is the use of optical lattices, which provide a means to realize diverse interaction configurations within a clean, controllable system. The other is the use of magnetically tunable Feshbach resonances to control the strength of the interatomic interaction. Together, these techniques offer the possibility of an experimental realization of many important model Hamiltonians of condensed matter physics, and may also lead to the discovery of new physics. Recent study of this system has shown that strong interactions near Feshbach resonance will lead to the population of multiple lattice bands, and that collisions between atoms on neighboring sites cannot be neglected. These effects lead to a complicated Hamiltonian, but one which can be simplified to an effective single-band model equivalent to the generalized Hubbard model (GHM), which is an extension of the Hubbard model that includes correlated hopping terms. My main results concern the study of this model. The strong correlations between the particles make it difficult to definitively determine the many body physics of the GHM. As a first approach to understanding the GHM in optical lattices, I focus mainly on cases where the problem is greatly simplified by allowing interactions among only small groups of lattice sites. This restriction can be implemented in experiments using an optical superlattice potential. Our results include a proposed scheme (based on double-well superlattices) to empirically verify that the GHM describes this system and to directly measure the various parameters of this model. Other results include exact solutions on four-site square plaquettes, which demonstrate that d-wave excitations can occur in the low-energy states. By using a superlattice to give an array of weakly coupled plaquettes, one can thus produce a d-wave superfluid state. This is of relevance to the study of high-Tc superconductors, although I note certain key differences between the sort of d-wave superfluid described here and that of the superconductors.
We study small systems of strongly interacting ultracold atoms under the influence of gauge potentials and spin-orbit couplings. We use second-order perturbation theory in tunneling, derive an effective theory for the strongly correlated insulating states with one atom per site, and solve it exactly. We find dramatic changes in the level structure and in the amount of degeneracies expected. We also demonstrate the dynamical behavior as the barriers between plaquettes are gradually removed and find potentially high overlap with the resonating valence bond (RVB) state of the larger system.
Ultracold atoms in optical lattices provide a versatile platform for studying many-body physics in a defect-free system with tunable parameters. For the analog quantum simulation of the Fermi-Hubbard model, fermionic atoms take on the role of the valence electrons and optical lattices provide the periodic potential in place of the solid-state crystal. The dynamics in the system are described by the tunneling amplitude t between neighboring lattice sites and the interaction energy U of two particles occupying the same lattice site. With the depth of the optical lattices and an external magnetic field, both parameters can be tuned to access a wide range of regimes. Two superimposed lattices with different lattice periods form an optical superlattice, where the most common configuration is a bichromatic superlattice with lattice periods different by a factor of two. Depending on the lattice depths and the relative phase of the lattices, the bichromatic superlattice potential ranges from an array of weakly-coupled double wells to a continuous lattice potential with a staggered energy offset. We developed a calibration technique for measuring the depth of an optical lattice with local resolution. The band structure of the optical lattice is probed by modulating the lattice depth and exciting the atoms to higher bands. However, compared to resolving the band occupations in a time-of-flight measurement, we further excite the atoms to an untrapped band to deplete the optical lattice along equipotential lines where the modulation frequency is resonant with the local band transitions. From the profile of the lattice depth, we obtain the calibration factor for the power regulation, the waist of the underlying lattice beams and the position of the lattice axis. This technique combines several calibration measurements, thereby reducing the measurement time and enabling an automation of the lattice alignment. For the bichromatic superlattice we realized an active stabilization of the superlattice phase that enables long-term measurements with a precise control over the superlattice phase. The instability of the superlattice phase is a result of the different refractive indices for the two lattices in air and the optical elements along the optical path. Using environmental sensors, we monitor the temperature, the pressure, and the relative humidity to apply the expected correction to the superlattice phase. The stabilized superlattice phase enabled the investigation of Floquet-driven double wells by modulating the energy offset through the superlattice phase. We used a near-resonant driving frequency with respect to the interaction energy to enhance the pair-tunneling amplitude in doubly-occupied double wells compared to static double wells and compared to the tunneling amplitude in singly-occupied double wells.
We report on the controlled creation of a valence bond state of delocalized effective-spin singlet and triplet dimers by means of a bichromatic optical superlattice. We demonstrate a coherent coupling between the singlet and triplet states and show how the superlattice can be employed to measure the singlet-fraction employing a spin-blockade effect. Our method provides a reliable way to detect and control nearest-neighbor spin correlations in many-body systems of ultracold atoms. Being able to measure these correlations is an important ingredient in studying quantum magnetism in optical lattices. We furthermore employ a SWAP operation between atoms which are part of different triplets, thus effectively increasing their bond-length. Such a SWAP operation provides an important step towards the massively parallel creation of a multiparticle entangled state in the lattice.