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arXiv:1202.6286 · New Journal of Physics

Phase-space tomography of matter-wave diffraction in the Talbot regime

Sun Kyung Lee, M S Kim, Carola Szewc, Hendrik Ulbricht

Published Apr 2, 2012• 5 citations
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Abstract

We report on the theoretical investigation of Wigner distribution function (WDF) reconstruction of the motional quantum state of large molecules in de Broglie interference. De Broglie interference of fullerenes and as the like already proves the wavelike behaviour of these heavy particles, while we aim to extract more quantitative information about the superposition quantum state in motion. We simulate the reconstruction of the WDF numerically based on an analytic probability distribution and investigate its properties by variation of parameters, which are relevant for the experiment. Even though the WDF described in the near-field experiment cannot be reconstructed completely, we observe negativity even in the partially reconstructed WDF. We further consider incoherent factors to simulate the experimental situation such as a finite number of slits, collimation, and particle-slit van der Waals interaction. From this we find experimental conditions to reconstruct the WDF from Talbot interference fringes in molecule Talbot-Lau interferometry.

DOI
10.1088/1367-2630/14/4/045001

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We report on the theoretical investigation of Wigner distribution function (WDF) reconstruction of the motional quantum state of large molecules in de Broglie interference. De Broglie interference of fullerenes and as the like already proves the wavelike behaviour of these heavy particles, while we aim to extract more quantitative information about the superposition quantum state in motion. We simulate the reconstruction of the WDF numerically based on an analytic probability distribution and investigate its properties by variation of parameters, which are relevant for the experiment. Even though the WDF described in the near-field experiment cannot be reconstructed completely, we observe negativity even in the partially reconstructed WDF. We further consider incoherent factors to simulate the experimental situation such as a finite number of slits, collimation, and particle-slit van der Waals interaction. From this we find experimental conditions to reconstruct the WDF from Talbot interference fringes in molecule Talbot-Lau interferometry.
We show our progress in setting up a three grating near-field Talbot-Lau interferometer (TLI) for large molecules such as C60. The TLI is the preferred tool for showing the wave nature of large particles, as it accepts beams of poor spatial coherence and because of its scaling properties with increasing mass of the particles. The spatial coherence is prepared by the first grating, it can be seen as an array of many collimation slits. Our setup is highly flexible in terms of the possibility of changing most of the parameters (such as distances between the gratings and grating angles) from the outside of the UHV-chamber. As the interferometer and the molecular beam source are place in separate vacuum chambers, refilling the oven and adjusting the setup parameters to different molecules is possible without opening the interferometer chamber. This is necessary, as the pressure in the interferometer chamber has to be lower than 5.10-7 mbar in order to observe high interference contrast. The TLI is highly sensitive to vibrations, especially in the range of 1 kHz (the inverse time-of-flight of the molecules through the interferometer), which makes vibration damping crucial for the success of observing interference. We observed vibration amplitudes of up to 75 nm at low frequencies (158 Hz). Compared to the inverse time-of-flight of the molecules, these vibrations are not 'seen' by the molecules and are non-critical. We observed interference of C60 with a contrast of 27 %, by scanning the self-image of the diffraction grating. In the present setup, an interference contrast of 60 % should be observed with perfect alignment of the gratings. Time-of-flight measurements showed small modulations of the velocity distribution at for interference expected distances of 2.5 ms. We also show the possibility of reconstructing the Wigner distribution function out of measurements for the case of Talbot interference under experimental conditions.
Paths of particles, emitted from distributed sources and passing out through slits of two gratings, G0G_{0}G0​ and G1G_{1}G1​, up to detectors, have been computed in details by the path integral method. The slits are represented by Gaussian functions that simulate fuzzy edges of the slits. Waves of matter be computed by this method show perfect interference patterns both between the gratings and behind the second grating. Coherent and noncoherent the distributed particle sources reproducing the interference patterns are discussed in details. Paraxial approximation stems from the wave function when removing the distributed sources onto infinity. The more hard-edged slits of the grating G1G_{1}G1​ are examined by simulating those slits by a superposition of more hard the Gaussian functions. As for the particles here we consider fullerene molecules. De Broglie wavelength of the molecules is adopted equal to 5 pm.
Particle paths, emitted from distributed sources and passing out through slits of two gratings, G0 and G1, up to detectors, have been computed in detail by the path integral method. The particles under consideration are fullerene molecules with a De Broglie wavelength equal to 5 pm. The slits are Gaussian functions that simulate fuzzy edges of the slits. Waves of the matter computed by this method show perfect interference patterns both between the gratings and behind the second grating. Coherent and non-coherent distributed particle sources reproducing the interference patterns are discussed in detail. Paraxial approximation results from removing the distributed sources onto innity. This approximation gives a wave function reproducing an exact copy of the Talbot carpet. PACS numbers: 03.75.-b, 03.75.Dg, 42.25.Hz
We demonstrate a near-field Talbot-Lau interferometer for C70 fullerene molecules. Such interferometers are particularly suitable for larger masses. Using three free-standing gold gratings of 1 microm period and a transversally incoherent but velocity-selected molecular beam, we achieve an interference fringe visibility of 40% with high count rate. Both the high visibility and its velocity dependence are in good agreement with a quantum simulation that takes into account the van der Waals interaction of the molecules with the gratings and are in striking contrast to a classical moiré model.
For various experiments to investigate quantum effects, matter-wave diffraction is an apparent example. Particle diffractions have been measured even at the large molecular level, such as the C 60 molecules. In order to describe the matter-wave diffraction of C 60 beam, we assume the initial wave functions behind a grating in form of the Fourier series with a Gaussian distribution function. By applying the Feynman path integral, the exact wave functions of the molecule diffraction in the near-field regime can be derived analytically. The obtained probability density distributions are corresponding to interference fringes as found in the Fresnel diffraction. The probability of finding C 60 molecules, behind the grating at the Talbot length, consistency with the mentioned experimental data of C 60 diffractions.
We discuss new de Broglie coherence experiments in a near-field molecule interferometer with a variety of large organic molecules. While de Broglie coherence is to first order only associated with the center-of-mass motion of the diffracted particle, we here investigate the question as to which extent the internal molecular property is relevant for, compatible with or detrimental for maintaining coherence in the translational degree of freedom. External perturbations, such as inhomogeneous external electric fields, may influence the delocalized molecules inside the matter wave interferometer and they allow us to access the molecular polarizabilities, permanent or even fluctuating electric dipole moments. We extract information about the molecular states from the interference phase shifts as well as from the observed dephasing in a Kapitza-Dirac Talbot-Lau-Stark-deflectometer. We discuss the relevance of our experiments with regard to both molecule metrology and the foundations of quantum mechanics, i.e. the preservation of coherence for highly complex particles in external fields.