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arXiv:1202.5240 · Physical Review A

Guiding of Rydberg atoms in a high-gradient magnetic guide

Mallory Traxler, Rachel Sapiro, Cornelius Hempel, Karl P. Lundquist, E. Power, Georg A. Raithel

Published Aug 20, 2012• 3 citations
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Abstract

We study the guiding of ${}^{87}$Rb 59$D$${}_{5/2}$ Rydberg atoms in a linear, high-gradient, two-wire magnetic guide. Time-delayed microwave ionization and ion detection are used to probe the Rydberg atom motion. We observe guiding of Rydberg atoms over a period of 5 ms following excitation. The decay time of the guided-atom signal is about five times that of the initial state. We attribute the lifetime increase to an initial phase of $l$-changing collisions and thermally induced Rydberg-Rydberg transitions. Detailed simulations of Rydberg-atom guiding reproduce most experimental observations and offer insight into the internal-state evolution.

DOI
10.1103/physreva.86.023414

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We study the guiding of 87{}^{87}87Rb 59D$${}_{5/2} Rydberg atoms in a linear, high-gradient, two-wire magnetic guide. Time-delayed microwave ionization and ion detection are used to probe the Rydberg atom motion. We observe guiding of Rydberg atoms over a period of 5 ms following excitation. The decay time of the guided-atom signal is about five times that of the initial state. We attribute the lifetime increase to an initial phase of lll-changing collisions and thermally induced Rydberg-Rydberg transitions. Detailed simulations of Rydberg-atom guiding reproduce most experimental observations and offer insight into the internal-state evolution.
We study cold rubidium Rydberg atoms, initially prepared in state 59D5/259{D}_{5/2}59D5/2​, guided along a two-wire magnetic atom guide. The evolution of the atoms is driven by the combined effects of internal-state transitions and dipole forces acting on the center-of-mass degree of freedom. State-selective field ionization, applied at a variable delay time, is used to investigate the evolution of the internal-state distribution. We observe a broadening of the field ionization spectrum caused by population transfer between Rydberg states. At late times, the distribution of the remaining Rydberg atoms becomes biased toward states with high principal quantum numbers. The population transfer is attributed to thermal transitions and, to a lesser extent, initial state mixing due to Rydberg-Rydberg collisions. Characteristic components in spatially and temporally resolved distributions of the ion signal are interpreted in the context of the underlying physics. The system is simulated with a model in which the center-of-mass dynamics are treated classically, while the internal-state dynamics are treated quantum mechanically. The simulation qualitatively reproduces most experimental findings and provides experimentally inaccessible information.
In this thesis, I explore a variety of experiments within linear, two-wire, magnetic atom guides. Experiments include guiding of Rydberg atoms; transferring between states while keeping the atoms contained within the guide; and designing, constructing, and testing a new experimental apparatus. The ultimate goal of the atom guiding experiments is to develop a continuous atom laser. The guiding of Rydberg atoms is demonstrated. The evolution of the atoms is driven by the combined effects of dipole forces acting on the center-of-mass degree of freedom as well as internal-state transitions. Time delayed microwave and state-selective field ionization are used to investigate the evolution of the internal-state distribution as well as the Rydberg atom motion while traversing the guide. The observed decay time of the guided-atom signal is about five times that of the initial state. A population transfer between Rydberg states contributes to this lengthened lifetime, and also broadens the observed field ionization spectrum. Transfer from one guided ground state to another is studied. In our setup, before the atoms enter the guide, they are pumped into the ∣F=1,mF=−1rangle|F=1, m_F=-1rangle∣F=1,mF​=−1rangle state. Using two repumpers, one tuned to the F=1rightarrowF′=0F=1rightarrow F'=0F=1rightarrowF′=0 transition and the other tuned to the F=1rightarrowF′=2F=1rightarrow F'=2F=1rightarrowF′=2 transition, the atoms are pumped between these guided states. Magnetic reflections within the guide are also studied. Design and construction of a new linear magnetic atom guide is detailed. This guide~betabetabeta has many improvements over the original guide~alphaalphaalpha: a Zeeman slower, magnetic injection, a physical shutter, and surface adsorption evaporative cooling are some of the main changes. Testing of this new system is underway. It is hoped that the improvements to guide~betabetabeta will yield an atom density sufficient to reach degeneracy, thereby forming a continuous BEC at the end of the guide. The BEC, which will be continuously replenished by the atoms within the guide, will be outcoupled to form a continuous atom laser.
We report on the trapping of long-lived strongly magnetized Rydberg atoms. 85Rb atoms are laser cooled and collected in a superconducting magnetic trap with a strong bias field (2.9 T) and laser excited to Rydberg states. Collisions scatter a small fraction of the Rydberg atoms into long-lived high-angular momentum "guiding-center" Rydberg states, which are magnetically trapped. The Rydberg atomic cloud is examined using a time-delayed, position-sensitive probe. We observe magnetic trapping of these Rydberg atoms for times up to 200 ms. Oscillations of the Rydberg-atom cloud in the trap reveal an average magnetic moment of the trapped Rydberg atoms of approximately -8microB. These results provide guidance for other Rydberg-atom trapping schemes and illuminate a possible route for trapping antihydrogen.
Cold circular Rydberg atoms are produced and magnetically trapped. The trap is characterized by direct spatial imaging of ion distributions, ion counting, and state-selective field ionization. At room temperature, we observe about 70% of the trapped atoms remaining after 6 ms. We measure a trap oscillation frequency increase of the circular Rydberg atom trap relative to the ground-state atom trap due to the larger magnetic moment of the circular Rydberg atoms. Simulations of the center-of-mass and internal-state evolution of circular states in our magnetic trap are performed and results are in good agreement with experimental observations.
Pulsed supersonic beams of helium atoms in the high-field-seeking 52p52p52p Rydberg state have been guided while following helical trajectories in the electrostatic field of a charged wire suspended along the axis of a grounded cylindrical metallic tube. The operation of this electrostatic wire guide for samples in high-field-seeking Rydberg-Stark states has been investigated with dc and pulsed electric potentials applied to the wire while the guided atoms were detected by pulsed electric-field ionization. The acceptance of the guide has been determined through numerical particle trajectory simulations.
Summary form only given. Laser-cooled atoms can be excited into Rydberg states to study Rydberg gases at high densities and low atomic velocities. Dense clouds of such atoms undergo virtually complete ionization when their density exceeds a critical value dependent on the principal quantum number n. We report a new regime in which the excited Rydberg population spontaneously evolves into long-lived high-l states, the lifetimes of which exceed the natural lifetimes of the initially excited Rydberg levels by two orders of magnitude. /sup 87/Rb atoms are collected and cooled to 50 /spl mu/K in a magneto optical trap (MOT), which is periodically turned off for 50 ms. 1 ms after the shutdown of the MOT the Rydberg atoms are created via a two-step excitation process using a 5 /spl mu/s long diode laser pulse.