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arXiv:1202.1795 · Philosophical Transactions of the Royal Society A Mathematical Physical and Engineering Sciences

On the quantumness of correlations in nuclear magnetic resonance

Diogo O. Soares-Pinto, R. Auccaise, Jonas Maziero, A. Gavini-Viana, R. M. Serra, Lucas C. Céleri

Published Sep 3, 2012• 25 citations
arXivHTMLPDF

Abstract

Nuclear magnetic resonance (NMR) was successfully employed to test several protocols and ideas in quantum information science. In most of these implementations, the existence of entanglement was ruled out. This fact introduced concerns and questions about the quantum nature of such bench tests. In this paper, we address some issues related to the non-classical aspects of NMR systems. We discuss some experiments where the quantum aspects of this system are supported by quantum correlations of separable states. Such quantumness, beyond the entanglement-separability paradigm, is revealed via a departure between the quantum and the classical versions of information theory. In this scenario, the concept of quantum discord seems to play an important role. We also present an experimental implementation of an analogue of the single-photon Mach-Zehnder interferometer employing two nuclear spins to encode the interferometric paths. This experiment illustrates how non-classical correlations of separable states may be used to simulate quantum dynamics. The results obtained are completely equivalent to the optical scenario, where entanglement (between two field modes) may be present.

DOI
10.1098/rsta.2011.0364

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Nuclear magnetic resonance (NMR) was successfully employed to test several protocols and ideas in quantum information science. In most of these implementations, the existence of entanglement was ruled out. This fact introduced concerns and questions about the quantum nature of such bench tests. In this paper, we address some issues related to the non-classical aspects of NMR systems. We discuss some experiments where the quantum aspects of this system are supported by quantum correlations of separable states. Such quantumness, beyond the entanglement-separability paradigm, is revealed via a departure between the quantum and the classical versions of information theory. In this scenario, the concept of quantum discord seems to play an important role. We also present an experimental implementation of an analogue of the single-photon Mach-Zehnder interferometer employing two nuclear spins to encode the interferometric paths. This experiment illustrates how non-classical correlations of separable states may be used to simulate quantum dynamics. The results obtained are completely equivalent to the optical scenario, where entanglement (between two field modes) may be present.
The existence of quantum correlation (as revealed by quantum discord), other than entanglement and its role in quantum-information processing (QIP), is a current subject for discussion. In particular, it has been suggested that this nonclassical correlation may provide computational speedup for some quantum algorithms. In this regard, bulk nuclear magnetic resonance (NMR) has been successfully used as a test bench for many QIP implementations, although it has also been continuously criticized for not presenting entanglement in most of the systems used so far. In this paper, we report a theoretical and experimental study on the dynamics of quantum and classical correlations in an NMR quadrupolar system. We present a method for computing the correlations from experimental NMR deviation-density matrices and show that, given the action of the nuclear-spin environment, the relaxation produces a monotonic time decay in the correlations. Although the experimental realizations were performed in a specific quadrupolar system, the main results presented here can be applied to whichever system uses a deviation-density matrix formalism.
This thesis focuses on the experimental creation and detection of a variety of quantum correlations using nuclear magnetic resonance hardware. Quantum entanglement, being most common and counter-intuitive, is one of the main type considered in this thesis. Quantum correlations play a major role in achieving, the much talked, computational speedup. Creation and detection of such correlations experimentally is a major thrust area in experimental quantum information processing field. Main goals of the studies undertaken in this thesis were to come up with strategies to detect the entanglement in a 'state-independent' way and with low experimental resources. The core of all the detection protocols is based on our own developed method which enables us to measure any observable with high accuracy. The experimental protocol has been successfully implemented to detect the entanglement of random two-qubit pure states. Further, the schemes for the experimental detection as well as classification of generic and general three-qubit pure states have also been devised and implemented successfully. Quantum correlation possessed by mixed and///or separable states e.g. non-classical, bound-entanglement and of non-local nature were also investigated. In all the investigations, the results were verified by one or more alternative ways e.g. full quantum state tomography.
"We review the theoretical and the experimental researches aimed at quantifying or identifying quantum correlations in liquid-state nuclear magnetic resonance (NMR) systems at room temperature. We first overview, at the formal level, a method to determine the quantum discord and its classical counterpart in systems described by a deviation matrix. Next, we describe an experimental implementation of that method. Previous theoretical analysis of quantum discord decoherence had predicted the time dependence of the discord to change suddenly under the influence of phase noise. The experiment attests to the robustness of the effect, sufficient to confirm the theoretical prediction even under the additional influence of a thermal environment. Finally, we discuss an observable witness for the quantumness of correlations in two-qubit systems and its first NMR implementation. Should the nature, not the amount, of the correlation be under scrutiny, the witness offers the most attractive alternative."
The project concerned the study of quantum correlations (QC) in compound systems, i.e. statistical correlations more general than entanglement which are predicted by quantum mechanics but not described in any classical scenario. I aimed to understand the technical and operational properties of the measures of QC, their interplay with entanglement quantifiers and the experimental accessibility.\nIn the first part of my research path, after having acquired the conceptual and technical rudiments of the project, I provided solutions for some computational issues: I developed analytical and numerical algorithms for calculating bipartite QC in finite dimensional systems. Then, I tackled the problem of the experimental detection of QC. There is no Hermitian operator associated with entanglement measures, nor with QC ones. However, the information encoded in a density matrix is redundant to quantify them, thus the full knowledge of the state is not required to accomplish the task. I reported the first protocol to measure the QC of an unknown state by means of a limited number of measurements, without performing the tomography of the state. My proposal has been implemented experimentally in a NMR (Nuclear Magnetic Resonance) setting.\nIn the final stage of the project, I explored the foundational and operational merits of QC. I showed that the QC shared by two subsystems yield a genuinely quantum kind of uncertainty on single local observables. The result is a promising evidence of the potential exploitability of separable (unentangled) states for quantum metrology in noisy conditions.
In this review we discuss intriguing properties of apparently classical optical fields, that go beyond purely classical context and allow us to speak about quantum characteristics of such fields and about their applications in quantum technologies. We briefly define the genuinely quantum concepts of entanglement and steering. We then move to the boarder line between classical and quantum world introducing quantum discord, a more general concept of quantum coherence, and finally a controversial notion of classical entanglement. To unveil the quantum aspects of often classically perceived systems, we focus more in detail on quantum discordant correlations between the light modes and on nonseparability properties of optical vector fields leading to entanglement between different degrees of freedom of a single beam. To illustrate the aptitude of different types of correlated systems to act as quantum or quantum-like resource, entanglement activation from discord, high-precision measurements with classical entanglement and quantum information tasks using intra-system correlations are discussed. The common themes behind the versatile quantum properties of seemingly classical light are coherence, polarization and inter and intra-mode quantum correlations.
The quantification of quantum correlations (other than entanglement) usually entails labored numerical optimization procedures also demanding quantum state tomographic methods. Thus it is interesting to have a laboratory friendly witness for the nature of correlations. In this Letter we report a direct experimental implementation of such a witness in a room temperature nuclear magnetic resonance system. In our experiment the nature of correlations is revealed by performing only few local magnetization measurements. We also compared the witness results with those for the symmetric quantum discord and we obtained a fairly good agreement.