Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

arXiv:1201.6295 · Physical Review Letters

Nonequilibrium Kondo model: Crossover from weak to strong coupling

Mikhail Pletyukhov, Herbert Schoeller

Published Jun 26, 2012• 89 citations
arXivHTMLPDF

Abstract

We analyze the nonequilibrium Kondo model at finite voltage and temperature by using a new formulation of the real-time renormalization group method with the Laplace variable as the flow parameter. We evaluate the energy-dependent spin relaxation rate and nonlinear conductance, and derive an approximate form for the universal line shape for the latter in the whole crossover regime from weak to strong coupling. The results are shown to agree well with exact methods in equilibrium, Fermi-liquid theory, weak-coupling expansions, and recent experiments. For the transient spin dynamics we find a universal exponential decay in the long-time limit along with a truncation-dependent pre-exponential power law. For multichannel models a pure power-law decay typical for non-Fermi-liquid behavior is predicted.

DOI
10.1103/physrevlett.108.260601

Related papers

Transport properties of fully screened Kondo models

Christoph B. M. Hörig, Christophe Mora, Dirk Schuricht

We study the nonequilibrium transport properties of fully (exactly) screened Kondo quantum dots subject to a finite bias voltage or a finite temperature. First, we calculate the Fermi-liquid coefficients of the conductance for models with arbitrary spin, i.e., its leading behavior for small bias voltages or temperatures. Second, we determine the low-temperature behavior of the static susceptibility from the exactly known Bethe ansatz results for the magnetization. Third, we study the crossover from strong to weak coupling in the spin-1/2 and the spin-1 models coupled to one or two screening channels, respectively. Using a real-time renormalization group method we calculate the static and dynamical spin-spin correlation functions for the spin-1/2 model as well as the linear and differential conductance and the static susceptibility for the spin-1 model. We define various Kondo scales and discuss their relations. We assess the validity of the renormalization-group treatment by comparing with known results for the temperature dependence of the linear conductance and static susceptibility as well as the Fermi-liquid behavior at low energies.

arXiv:1402.0479•Physical Review B•Apr 11, 2014•11 citations

Relaxation versus Decoherence: Spin and Current Dynamics in the Anisotropic Kondo Model at Finite Bias and Magnetic Field

Mikhail Pletyukhov, Dirk Schuricht, Herbert Schoeller

Using a nonequilibrium renormalization group method we study the real-time evolution of spin and current in the anisotropic Kondo model (both antiferromagnetic and ferromagnetic) at a finite magnetic field h(0) and bias voltage V. We derive analytic expressions for all times in the weak-coupling regime max{V, h(0),1/t} >> T(c) (T(c) is the strong-coupling scale). We find that all observables decay both with the spin relaxation and decoherence rates Gamma(1/2). Various V-dependent logarithmic, oscillatory, and power-law contributions are predicted. The low-energy cutoff of logarithmic terms is generically identified by the difference of transport decay rates. For small times t << max{V, h(0)}(-1), we obtain universal dynamics for spin and current.

arXiv:0910.0119•Physical Review Letters•Mar 8, 2010•78 citations

Real-time renormalization group in frequency space: A two-loop analysis of the nonequilibrium anisotropic Kondo model at finite magnetic field

Herbert Schoeller, Frank Reininghaus

We apply a recently developed nonequilibrium real-time renormalization group (RG) method in frequency space to describe nonlinear quantum transport through a small fermionic quantum system coupled weakly to several reservoirs via spin and/or orbital fluctuations. Within a weak-coupling two-loop analysis, we derive analytic formulas for the nonlinear conductance and the kernel determining the time evolution of the reduced density matrix. A consistent formalism is presented how the RG flow is cut off by relaxation and dephasing rates. We apply the general formalism to the nonequilibrium anisotropic Kondo model at finite magnetic field. We consider the weak-coupling regime, where the maximum of voltage and bare magnetic field is larger than the Kondo temperature. In this regime, we calculate the nonlinear conductance, the magnetic susceptibility, the renormalized spin relaxation and dephasing rates, and the renormalized $g$ factor. All quantities are considered up to the first logarithmic correction beyond leading order at resonance. Up to a redefinition of the Kondo temperature, we confirm previous results for the conductance and the magnetic susceptibility in the isotropic case. In addition, we present a consistent calculation of the resonant line shapes, including the determination whether the spin relaxation or dephasing rate cuts off the logarithmic divergence. Furthermore, we calculate quantities characterizing the exponential decay of the time evolution of the magnetization. In contrast to the conductance, we find that the derivative of the spin relaxation (dephasing) rate with respect to the magnetic field is logarithmically enhanced (suppressed) for voltages smaller (larger) than the renormalized magnetic field, and that the logarithmic divergence is cut off by the opposite rate. The renormalized $g$ factor is predicted to show a symmetric logarithmic suppression at resonance, which is cut off by the spin relaxation rate. We propose a three-terminal setup to measure the suppression at resonance. For all quantities, we analyze also the anisotropic case and find additional nonequilibrium effects at resonance.

arXiv:0902.1446•Physical Review B•Jul 22, 2009•55 citations

Spin precession and real-time dynamics in the Kondo model: Time-dependent numerical renormalization-group study

Frithjof B. Anders, Avraham Schiller

A detailed derivation of the recently proposed time-dependent numerical renormalization-group (TD-NRG) approach to nonequilibrium dynamics in quantum-impurity systems is presented. We demonstrate that the method is suitable for fermionic as well as bosonic baths. Comparisons with exact analytical results for the charge relaxation in the resonant-level model and for dephasing in the spin-boson model establish the accuracy of the method. The real-time dynamics of a single spin coupled to each type of bath is investigated. We use the TD-NRG to calculate the spin relaxation and spin precession of a single Kondo impurity. The short- and long-time dynamics are studied as a function of temperature in the ferromagnetic and antiferromagnetic regimes. The short-time dynamics agrees very well with analytical results obtained at second order in the exchange coupling $J$. In the ferromagnetic regime, the transient spin decay is described by the scaling variable $x=2{\ensuremath{\rho}}_{F}\ensuremath{\mid}J(T)\ensuremath{\mid}Tt$. In the antiferromagnetic regime, the long-time decay is governed for $T<{T}_{K}$ by the Kondo time scale $1∕{T}_{K}$. Here ${\ensuremath{\rho}}_{F}$ is the conduction-electron density of states, ${T}_{K}$ is the Kondo temperature, and $J(T)$ is the effective exchange coupling at temperature $T$. Results for spin precession are obtained by rotating the external magnetic field from the $x$ axis to the $z$ axis.

arXiv:cond-mat/0604517•Physical Review B•Dec 18, 2006•250 citations

Crossover from nonequilibrium to equilibrium behavior in the time-dependent Kondo model

Dmitry Lobaskin, Stefan K. Kehrein

We investigate the equilibration of a Kondo model that is initially prepared in a nonequilibrium state towards its equilibrium behavior. Such initial nonequilibrium states can, e.g., be realized in quantum-dot experiments with time-dependent gate voltages. We evaluate the nonequilibrium spin-spin correlation function at the Toulouse point of the Kondo model exactly and analyze the crossover between nonequilibrium and equilibrium behavior as the nonequilibrium initial state evolves as a function of the waiting time for the first spin measurement. Using the flow equation method, we extend these results to the experimentally relevant limit of small Kondo couplings.

arXiv:cond-mat/0405193•Physical Review B•May 18, 2005•65 citations

Kondo effect out of equilibrium

Thomas Korb, Herbert Schoeller

Correlations are a central ingredient of modern condensed matter physics. With the advent of mesoscopic physics, it became possible to study correlated systems in non-equilibrium situations, which can be reached by e.g. driving a constant current through a quantum dot. A basic question is how correlations on the one hand and a non-equilibrium current on the other hand influence each other. Here this interplay is studied for the model system of a quantum dot in the Kondo regime using the real time renormalization group (RTRG) method. This method is a functional renormalization group (RG) method allowing a non-perturbative description of correlated systems in non-equilibrium. For the Kondo quantum dot the method is generalized to the case of double vertices. The RTRG method not only provides equations for the calculation of the renormalized coupling between the quantum dot spin and the reservoir electrons, but also equations for the calculation of the non-equilibrium decoherence rate and the non-equilibrium current.The RG equations are derived to second order. This approximation is expected to be valid as long as the quantum dot does not enter the strong coupling regime, i.e. the effective coupling strength between the quantum dot spin and the electrons does not become too large. It is found that this is the case if the bias voltage applied to the dot or the temperature is much larger than the Kondo temperature.It is shown that the RG equations lead to coupling functions depending on the energy of the incident and the scattered electron. This dependence is simplified to the dependence on the average energy of the incident and the scattered electron in the weak coupling regime.A closer inspection of the RG equations for the couplings shows that they not only contain terms leading to a logarithmic increase of the coupling strength but also subleading terms which are unimportant in the weak coupling regime. The RG equations are solved analytically for the case where the subleading terms are neglected. It is found that the coupling functions develop resonances at energies associated with the chemical potentials of the reservoirs. The height of these resonances is determined by the decoherence rate. However, for bias voltages much larger than the Kondo temperature these resonances do not affect the conductance for a two terminal setup, so the conductance does not provide a measure for the decoherence rate in this case. It is found that the conductance for the two terminal setup is a universal function of voltage/Kondo temperature and temperature/Kondo temperature in the weak coupling regime. This function is calculated analytically in the limits of vanishing voltage or temperature. Furthermore, it is found that for zero temperature the decoherence rate is proportional to the non-equilibrium current flowing through the system. This supports the physical picture that a non-equilibrium current is associated with a decoherence rate, which cuts the logarithmic scaling of the coupling strength.Finally, the RG equations are solved numerically for zero temperature including the subleading corrections found before. As expected, the subleading corrections have no impact on the decoherence rate and the conductance in the weak coupling regime. On the other hand, it is found that they lead to strong deviations from the results of the analytic leading logarithmic approximation if the bias voltage approaches the Kondo temperature. Generally, it is found that the subleading corrections lead to a saturation of the decoherence rate and the conductance to some finite value. However, for the numerical solution a numerical regularization parameter has to be introduced. It turns out that the saturation value found depends on its value, so no statements on the precise value of the decoherence rate and the current can be made in this regime.

•Jan 1, 2006•0 citations
We analyze the nonequilibrium Kondo model at finite voltage and temperature by using a new formulation of the real-time renormalization group method with the Laplace variable as the flow parameter. We evaluate the energy-dependent spin relaxation rate and nonlinear conductance, and derive an approximate form for the universal line shape for the latter in the whole crossover regime from weak to strong coupling. The results are shown to agree well with exact methods in equilibrium, Fermi-liquid theory, weak-coupling expansions, and recent experiments. For the transient spin dynamics we find a universal exponential decay in the long-time limit along with a truncation-dependent pre-exponential power law. For multichannel models a pure power-law decay typical for non-Fermi-liquid behavior is predicted.
We study the nonequilibrium transport properties of fully (exactly) screened Kondo quantum dots subject to a finite bias voltage or a finite temperature. First, we calculate the Fermi-liquid coefficients of the conductance for models with arbitrary spin, i.e., its leading behavior for small bias voltages or temperatures. Second, we determine the low-temperature behavior of the static susceptibility from the exactly known Bethe ansatz results for the magnetization. Third, we study the crossover from strong to weak coupling in the spin-1/2 and the spin-1 models coupled to one or two screening channels, respectively. Using a real-time renormalization group method we calculate the static and dynamical spin-spin correlation functions for the spin-1/2 model as well as the linear and differential conductance and the static susceptibility for the spin-1 model. We define various Kondo scales and discuss their relations. We assess the validity of the renormalization-group treatment by comparing with known results for the temperature dependence of the linear conductance and static susceptibility as well as the Fermi-liquid behavior at low energies.
Using a nonequilibrium renormalization group method we study the real-time evolution of spin and current in the anisotropic Kondo model (both antiferromagnetic and ferromagnetic) at a finite magnetic field h(0) and bias voltage V. We derive analytic expressions for all times in the weak-coupling regime max{V, h(0),1/t} >> T(c) (T(c) is the strong-coupling scale). We find that all observables decay both with the spin relaxation and decoherence rates Gamma(1/2). Various V-dependent logarithmic, oscillatory, and power-law contributions are predicted. The low-energy cutoff of logarithmic terms is generically identified by the difference of transport decay rates. For small times t << max{V, h(0)}(-1), we obtain universal dynamics for spin and current.
We apply a recently developed nonequilibrium real-time renormalization group (RG) method in frequency space to describe nonlinear quantum transport through a small fermionic quantum system coupled weakly to several reservoirs via spin and/or orbital fluctuations. Within a weak-coupling two-loop analysis, we derive analytic formulas for the nonlinear conductance and the kernel determining the time evolution of the reduced density matrix. A consistent formalism is presented how the RG flow is cut off by relaxation and dephasing rates. We apply the general formalism to the nonequilibrium anisotropic Kondo model at finite magnetic field. We consider the weak-coupling regime, where the maximum of voltage and bare magnetic field is larger than the Kondo temperature. In this regime, we calculate the nonlinear conductance, the magnetic susceptibility, the renormalized spin relaxation and dephasing rates, and the renormalized ggg factor. All quantities are considered up to the first logarithmic correction beyond leading order at resonance. Up to a redefinition of the Kondo temperature, we confirm previous results for the conductance and the magnetic susceptibility in the isotropic case. In addition, we present a consistent calculation of the resonant line shapes, including the determination whether the spin relaxation or dephasing rate cuts off the logarithmic divergence. Furthermore, we calculate quantities characterizing the exponential decay of the time evolution of the magnetization. In contrast to the conductance, we find that the derivative of the spin relaxation (dephasing) rate with respect to the magnetic field is logarithmically enhanced (suppressed) for voltages smaller (larger) than the renormalized magnetic field, and that the logarithmic divergence is cut off by the opposite rate. The renormalized ggg factor is predicted to show a symmetric logarithmic suppression at resonance, which is cut off by the spin relaxation rate. We propose a three-terminal setup to measure the suppression at resonance. For all quantities, we analyze also the anisotropic case and find additional nonequilibrium effects at resonance.
A detailed derivation of the recently proposed time-dependent numerical renormalization-group (TD-NRG) approach to nonequilibrium dynamics in quantum-impurity systems is presented. We demonstrate that the method is suitable for fermionic as well as bosonic baths. Comparisons with exact analytical results for the charge relaxation in the resonant-level model and for dephasing in the spin-boson model establish the accuracy of the method. The real-time dynamics of a single spin coupled to each type of bath is investigated. We use the TD-NRG to calculate the spin relaxation and spin precession of a single Kondo impurity. The short- and long-time dynamics are studied as a function of temperature in the ferromagnetic and antiferromagnetic regimes. The short-time dynamics agrees very well with analytical results obtained at second order in the exchange coupling JJJ. In the ferromagnetic regime, the transient spin decay is described by the scaling variable $x=2{\ensuremath{\rho}}_{F}\ensuremath{\mid}J(T)\ensuremath{\mid}Tt$. In the antiferromagnetic regime, the long-time decay is governed for T<TKT<{T}_{K}T<TK​ by the Kondo time scale 1∕TK1∕{T}_{K}1∕TK​. Here ${\ensuremath{\rho}}_{F}$ is the conduction-electron density of states, TK{T}_{K}TK​ is the Kondo temperature, and J(T)J(T)J(T) is the effective exchange coupling at temperature TTT. Results for spin precession are obtained by rotating the external magnetic field from the xxx axis to the zzz axis.
We investigate the equilibration of a Kondo model that is initially prepared in a nonequilibrium state towards its equilibrium behavior. Such initial nonequilibrium states can, e.g., be realized in quantum-dot experiments with time-dependent gate voltages. We evaluate the nonequilibrium spin-spin correlation function at the Toulouse point of the Kondo model exactly and analyze the crossover between nonequilibrium and equilibrium behavior as the nonequilibrium initial state evolves as a function of the waiting time for the first spin measurement. Using the flow equation method, we extend these results to the experimentally relevant limit of small Kondo couplings.
Correlations are a central ingredient of modern condensed matter physics. With the advent of mesoscopic physics, it became possible to study correlated systems in non-equilibrium situations, which can be reached by e.g. driving a constant current through a quantum dot. A basic question is how correlations on the one hand and a non-equilibrium current on the other hand influence each other. Here this interplay is studied for the model system of a quantum dot in the Kondo regime using the real time renormalization group (RTRG) method. This method is a functional renormalization group (RG) method allowing a non-perturbative description of correlated systems in non-equilibrium. For the Kondo quantum dot the method is generalized to the case of double vertices. The RTRG method not only provides equations for the calculation of the renormalized coupling between the quantum dot spin and the reservoir electrons, but also equations for the calculation of the non-equilibrium decoherence rate and the non-equilibrium current.The RG equations are derived to second order. This approximation is expected to be valid as long as the quantum dot does not enter the strong coupling regime, i.e. the effective coupling strength between the quantum dot spin and the electrons does not become too large. It is found that this is the case if the bias voltage applied to the dot or the temperature is much larger than the Kondo temperature.It is shown that the RG equations lead to coupling functions depending on the energy of the incident and the scattered electron. This dependence is simplified to the dependence on the average energy of the incident and the scattered electron in the weak coupling regime.A closer inspection of the RG equations for the couplings shows that they not only contain terms leading to a logarithmic increase of the coupling strength but also subleading terms which are unimportant in the weak coupling regime. The RG equations are solved analytically for the case where the subleading terms are neglected. It is found that the coupling functions develop resonances at energies associated with the chemical potentials of the reservoirs. The height of these resonances is determined by the decoherence rate. However, for bias voltages much larger than the Kondo temperature these resonances do not affect the conductance for a two terminal setup, so the conductance does not provide a measure for the decoherence rate in this case. It is found that the conductance for the two terminal setup is a universal function of voltage/Kondo temperature and temperature/Kondo temperature in the weak coupling regime. This function is calculated analytically in the limits of vanishing voltage or temperature. Furthermore, it is found that for zero temperature the decoherence rate is proportional to the non-equilibrium current flowing through the system. This supports the physical picture that a non-equilibrium current is associated with a decoherence rate, which cuts the logarithmic scaling of the coupling strength.Finally, the RG equations are solved numerically for zero temperature including the subleading corrections found before. As expected, the subleading corrections have no impact on the decoherence rate and the conductance in the weak coupling regime. On the other hand, it is found that they lead to strong deviations from the results of the analytic leading logarithmic approximation if the bias voltage approaches the Kondo temperature. Generally, it is found that the subleading corrections lead to a saturation of the decoherence rate and the conductance to some finite value. However, for the numerical solution a numerical regularization parameter has to be introduced. It turns out that the saturation value found depends on its value, so no statements on the precise value of the decoherence rate and the current can be made in this regime.