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arXiv:1201.3240 · Journal of Modern Optics

Atom and photon measurement in cooperative scattering by cold atoms

Tom Bienaimé, M. Petruzzo, D. Bigerni, N. Piovella, Robin Kaiser

Published Jul 12, 2011• 68 citations
arXivHTMLPDF

Abstract

In this paper, we study cooperative scattering of low intensity light by a cloud of N two-level systems. We include the incident laser field driving these two-level systems and compute the radiation pressure force on the center of mass of the cloud. This signature is of particular interest for experiments with laser cooled atoms. Including the complex coupling between dipoles in a scalar model for dilute clouds of two-level systems, we obtain expression for cooperative scattering forces taking into account the collective Lamb shift. We also derive the expression of the radiation pressure force on a large cloud of two-level systems from an heuristic approach and show that at lowest driving intensities this force is identical for a product and an entangled state.

DOI
10.1080/09500340.2011.594911

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In this paper, we study cooperative scattering of low intensity light by a cloud of N two-level systems. We include the incident laser field driving these two-level systems and compute the radiation pressure force on the center of mass of the cloud. This signature is of particular interest for experiments with laser cooled atoms. Including the complex coupling between dipoles in a scalar model for dilute clouds of two-level systems, we obtain expression for cooperative scattering forces taking into account the collective Lamb shift. We also derive the expression of the radiation pressure force on a large cloud of two-level systems from an heuristic approach and show that at lowest driving intensities this force is identical for a product and an entangled state.
Abstract A cloud of cold N two‐level atoms driven by a resonant laser beam shows cooperative effects both in the scattered radiation field and in the radiation pressure force acting on the cloud center‐of‐mass. The induced dipoles synchronize and the scattered light presents superradiant and/or subradiant features. We present a quantum description of the process in terms of a master equation for the atomic density matrix in the scalar, Born‐Markov approximations, reduced to the single‐excitation limit. From a perturbative approach for weak incident field, we derive from the master equation the effective Hamiltonian, valid in the linear regime. We discuss the validity of the driven timed Dicke ansatz and of a partial wave expansion for different optical thicknesses and we give analytical expressions for the scattered intensity and the radiation pressure force on the center of mass. We also derive an expression for collective suppression of the atomic excitation and the scattered light by these correlated dipoles.
We discuss the role of diffuse, Mie, and cooperative scattering on the radiation pressure force acting on the center of mass of a cloud of cold atoms. Even though a mean-field ansatz (the ``timed Dicke state''), previously derived from a cooperative scattering approach, has been shown to agree satisfactorily with experiments, diffuse scattering also describes very well most features of the radiation pressure force on large atomic clouds. We compare in detail an incoherent, random walk model for photons and a diffraction approach to the more complete description based on coherently coupled dipoles. We show that a cooperative scattering approach, although it provides a quite complete description of the scattering process, is not necessary to explain the previous experiments on the radiation pressure force.
Cooperative scattering in cold atoms has gained renewed interest, in particular in the context of single-photon superradiance, with the recent experimental observation of super- and subradiance in dilute atomic clouds. Numerical simulations to support experimental signatures of cooperative scattering are often limited by the number of dipoles which can be treated, well below the number of atoms in the experiments. In this paper, we provide systematic numerical studies aimed at matching the regime of dilute atomic clouds. We use a scalar coupled-dipole model in the low excitation limit and an exclusion volume to avoid density-related effects. Scaling laws for super- and subradiance are obtained and the limits of numerical studies are pointed out. We also illustrate the cooperative nature of light scattering by considering an incident laser field, where half of the beam has a π phase shift. The enhanced subradiance obtained under such condition provides an additional signature of the role of coherence in the detected signal.
Abstract When a cold atomic gas is illuminated by a quasi-resonant laser beam, light-induced dipole–dipole correlations make the scattering of light a cooperative process. Once a fluid description is adopted for the atoms, many scattering properties are captured by the definition of a complex refractive index. The solution of the scattering problem is here presented for spherical atomic clouds of arbitrary density profiles, such as parabolic densities characteristic of ultra-cold clouds. A new solution for clouds with infinite boundaries is derived, which is particularly useful for the Gaussian densities of thermal atomic clouds. The presence of Mie resonances, a signature of the cloud acting as a cavity for the light, is discussed. These resonances leave their fingerprint in various observables such as the scattered intensity or in the radiation pressure force, and can be observed by tuning the frequency of the incident laser field or the atom number.
The problem of the interaction of N atoms with a laser beam and vacuum modes can give rise to many interesting phenomena concerning the spontaneous emission of light and its propagation in the medium. The cooperative effects, for example, such as superadiance and subradiance, are effects related to the coherence created between the atoms when a photon is emitted spontaneously by a single excited atom. Superradiance can be defined as the enhancement of the spontaneous emission due to constructive interference of the scattered light. Its counterpart, subradiance, is the trapping of some remaining light due to destructive interference. In cold atoms, some previous theoretical works predict and characterize these two cooperative effects in a large and diluted atomic cloud, in the regime of low intensities and large detunings of the incident laser. The theoretical model is a coupled-dipole model for two-level atoms driven by a low-intensity field and in the scalar approach. The experiment consists in measuring the super- and subradiant decay rates from the temporal emitted intensity after the switch off of the incident laser in the steady state. Our experimental setup consists in a magneto-optical trap of rubidium 87 atoms at large resonant optical thicknesses. A probe beam excites the atoms close to the D2 line. The intensity emitted is detected by a single photon detector with no afterpulsing and a calibration procedure allows us to determine the resonant optical thickness of the cloud and its temperature. In this work, we report the experimental observation of super- and subradiance in a large cloud of cold atoms. For subradiance, the main result is the linear evolution of the characteristic time with the resonant optical thickness of the cloud and its independence of the detuning. For superradiance, we observe superradiance out of the forward direction. We verify the validity of our interpretations with the predictions of the coupled-dipole model. Finally, we discuss the interplay of subradiance and radiation trapping, as well as theoretical predictions for: a setup of a phased cloud, to control the subradiant amplitude emission; and temperature effects, where subradiance is shown to be robust in a large range of temperatures.