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arXiv:1201.1985 · Physical Review A

Laser-phase and frequency stabilization using atomic coherence

Yoshio Torii, Hideyasu Tashiro, Nozomi Ohtsubo, T. Aoki

Published Sep 4, 2012• 23 citations
arXivHTMLPDF

Abstract

We present a simple method of stabilizing the laser phase and frequency by polarization spectroscopy of an atomic vapor. In analogy to the Pound-Drever-Hall method, which uses a cavity as a memory of the laser phase, this method uses atomic coherence (dipole oscillations) as a phase memory of the transmitting laser field. A preliminary experiment using a distributed feedback laser diode and a rubidium vapor cell demonstrates a shot-noise-limited laser linewidth reduction (from 2 MHz to 20 kHz). This method would improve the performance of gas-cell-based optical atomic clocks and magnetometers and facilitate laser-cooling experiments using narrow transitions.

DOI
10.1103/physreva.86.033805

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We present a simple method of stabilizing the laser phase and frequency by polarization spectroscopy of an atomic vapor. In analogy to the Pound-Drever-Hall method, which uses a cavity as a memory of the laser phase, this method uses atomic coherence (dipole oscillations) as a phase memory of the transmitting laser field. A preliminary experiment using a distributed feedback laser diode and a rubidium vapor cell demonstrates a shot-noise-limited laser linewidth reduction (from 2 MHz to 20 kHz). This method would improve the performance of gas-cell-based optical atomic clocks and magnetometers and facilitate laser-cooling experiments using narrow transitions.
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We present a simple modulation-free technique to stabilize a laser frequency to the Doppler-free spectra of an atomic vapor. Polarization spectroscopy with use of a balanced polarimeter allows us to obtain a background-free dispersion signal suitable for high-speed and robust frequency stabilization. We employed the method to the 5S(1/2) F = 2 --> 5P(3/2) F' = 3 transition of 87Rb atoms. The achieved feedback bandwidth was approximately 100 kHz, and an efficient suppression of the frequency noise in a laboratory environment was attained.
The utilization of atomic or molecular spectroscopy for frequency locking of single-frequency laser to improve laser frequency stability plays an important role in the experimental investigation of optically pumped atomic magnetometers, atomic clocks, laser cooling and trapping of atoms, etc. We have experimentally demonstrated a technique for frequency stabilization of a single-frequency laser employing the bright state spectroscopy (BSS) with a rubidium atomic vapor cell. By utilizing the counter-propagating dual-frequency 795 nm laser beams with mutually orthogonal linear polarization and a frequency difference of 6.834 GHz, which is equal to the hyperfine splitting of rubidium-87 ground state 5S1/2, an absorption-enhanced signal with narrow linewidth at the center of Doppler-broadened transmission spectroscopy is observed when continuous scanning the laser frequency over rubidium-87 D1 transition. This is the so-called BSS. Amplitude of the absorption-enhanced signal in the BSS is much larger compared with the conventional saturation absorption spectroscopy (SAS). The relationship between linewidth and amplitude of the BSS signal and laser beam intensity has been investigated. This high-contrast absorption-enhanced BSS signal has been employed for the laser frequency stabilization. The experimental results show that the frequency stability is 4.4×10−11 with an integration time of 40 s, near one order of magnitude better than that for using the SAS.
Lasers with high spectral purity are indispensable for optical clocks and coherent manipulation of atomic and molecular qubits for applications such as quantum computing and quantum simulation. Stabilisation of the laser to a reference can provide a narrow linewidth and high spectral purity. However, widely-used diode lasers exhibit fast phase noise that prevents high fidelity qubit manipulation. Here we demonstrate a self-injection locked diode laser system utilizing a medium finesse cavity. The cavity not only provides a stable resonance frequency, but at the same time acts as a low-pass filter for phase noise beyond the cavity linewidth of around 100 kHz, resulting in low phase noise from dc to the injection lock limit. We model the expected laser performance and benchmark it using a single trapped 40^{40}40Ca+^{+}+-ion as a spectrum analyser. We show that the fast phase noise of the laser at relevant Fourier frequencies of 100 kHz to >2 MHz is suppressed to a noise floor of between -110 dBc/Hz and -120 dBc/Hz, an improvement of 20 to 30 dB over state-of-the-art Pound-Drever-Hall-stabilized extended-cavity diode lasers. This strong suppression avoids incoherent (spurious) spin flips during manipulation of optical qubits and improves laser-driven gates in using diode lasers with applications in quantum logic spectroscopy, quantum simulation and quantum computation.
Lasers with high spectral purity are indispensable for optical clocks and for the coherent manipulation of atomic and molecular qubits in applications such as quantum computing and quantum simulation. While the stabilization of such lasers to a reference can provide a narrow linewidth, the widely used diode lasers exhibit fast phase noise that prevents high-fidelity qubit manipulation. In this paper, we demonstrate a self-injection locked diode laser system that utilizes a high-finesse cavity. This cavity not only provides a stable resonance frequency, it also acts as a low-pass filter for phase noise beyond the cavity linewidth of around 100 kHz, resulting in low phase noise from dc to the injection lock limit. We model the expected laser performance and benchmark it using a single trapped 40 Ca + -ion as a spectrum analyzer. We show that the fast phase noise of the laser at relevant Fourier frequencies of 100 kHz to >2 MHz is suppressed to a noise floor of between −110 dBc/Hz and −120 dBc/Hz, an improvement of 20 to 30 dB over state-of-the-art Pound-Drever-Hall-stabilized extended-cavity diode lasers. This strong suppression avoids incoherent (spurious) spin flips during manipulation of optical qubits and improves laser-driven gates when using diode lasers in applications involving quantum logic spectroscopy, quantum simulation, and quantum computation.
Precise laser stabilization is a fundamental aspect of modern metrology, directly influencing the accuracy of fundamental measurements in fields such as high-precision metrology, atomic sensor applications, and quantum technologies. Saturation absorption spectroscopy (SAS) is one of the most effective techniques for achieving high spectral stability, as it enables laser frequencies to be locked to atomic resonances. This technique exploits the nonlinear interaction between a weaker probe beam and a stronger pump beam within a rubidium (Rb) atomic vapor cell. By eliminating Doppler broadening, SAS allows well-defined hyperfine transitions to be resolved, providing a reliable optical frequency reference. This study aims to optimize laser frequency stabilization using the SAS technique by investigating the effects of laser light polarization, atomic vapor cell temperature, and pump-probe power adjustments. Polarization-dependent selection rules influence transition probabilities, thereby affecting spectral contrast and frequency stability. Additionally, atomic density variations, which depend on the vapor cell temperature, influence signal strength and linewidth, necessitating precise temperature control for optimal performance. Furthermore, the pump power must be sufficient to induce saturation without excessive power broadening, while the probe power must remain low enough to prevent spectral line distortion. By optimizing polarization, temperature, and power parameters, the stabilization of the Rb atomic laser can be enhanced, leading to improved reproducibility and consistency in high-precision measurements. SAS-based laser stabilization is particularly crucial for atomic sensor applications and quantum technologies, where highly stable, narrow-linewidth lasers are essential for precision measurements. Applications such as atomic magnetometers, gyroscopes, and inertial navigation systems depend on precisely stabilized lasers for optimal performance. By enhancing the reliability of laser frequency stabilization, this work contributes to the advancement of next-generation atomic sensors with improved sensitivity and stability.