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arXiv:1112.3524 · Physical Review A

NMR implementation of a quantum delayed-choice experiment

Soumya S. Roy, Abhishek Shukla, T. S. Mahesh

Published Feb 7, 2012• 77 citations
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Abstract

We report an experimental demonstration of a quantum delayed-choice experiment via nuclear magnetic resonance techniques. Two spin-1/2 nuclei from each molecule of a liquid ensemble are used as target and ancilla qubits. The circuit corresponding to the recently proposed quantum delayed-choice setup has been implemented with different states of an ancilla qubit. As expected theoretically, our experiments clearly demonstrate continuous morphing of the target qubit between particle-like and wave-like behaviors. The experimental visibility of the interference patterns shows good agreement with theory.

DOI
10.1103/physreva.85.022109

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We report an experimental demonstration of a quantum delayed-choice experiment via nuclear magnetic resonance techniques. Two spin-1/2 nuclei from each molecule of a liquid ensemble are used as target and ancilla qubits. The circuit corresponding to the recently proposed quantum delayed-choice setup has been implemented with different states of an ancilla qubit. As expected theoretically, our experiments clearly demonstrate continuous morphing of the target qubit between particle-like and wave-like behaviors. The experimental visibility of the interference patterns shows good agreement with theory.
The puzzling properties of quantum mechanics, i.e., wave-particle duality, entanglement, and superposition, have been dissected experimentally over the past decades. However, hidden-variable (HV) models based on three classical assumptions of wave-particle objectivity, determinism, and independence strive to explain the same experiments or even defeat quantum mechanics. Meanwhile, the steady development of quantum technologies continues to enable us to test experimentally the predictions of quantum mechanics and HV theories. We report an experimental demonstration of an entanglement-assisted quantum delayed-choice scheme using a liquid nuclear magnetic resonance quantum-information processor. This experiment is based on the recently proposed scheme [R. Ionicioiu et al., Nat. Commun. 5. 3997 (2014)], which predicted different results for quantum mechanics and HV theories. In our experiments, the intensities and the visibilities of the interference are consistent with the theoretical predictions of quantum mechanics. The results show that a contradiction with the experiments is indeed appearing when all three assumptions of the HV models are combined, though any two of those assumptions are compatible with the experiments.
Nuclear Magnetic Resonance (NMR) forms a natural test-bed to perform quantum information processing (QIP) and has so far proven to be one of the most successful quantum information processors. The nuclear spins in a molecule treated as quantum bits or qubits which are the basic building blocks of a quantum computer. The development of NMR over half a century puts it in a platform where we can utilize its excellent control techniques over an ensemble of spin systems and perform quantum computation in a highly controlled way. Apart from a successful quantum information processor, NMR is also a highly powerful quantum platform where many of the potentially challenging quantum mechanical experiments can be performed.
Wave-particle duality of quantum objects is one of the most striking features of quantum physics and has been widely studied in past decades. Developments of quantum technologies enable us to experimentally realize several quantum phenomena. Observation of wave-particle morphing behavior in the context of the quantum delayed-choice experiment (QDCE) is one of them. Adopting the scheme of QDCE, we demonstrate how the coexistence of wave and particle nature emerges as a consequence of the uncertainty in the quantum controlled experimental setup, using a five-qubit cloud-based quantum processor. We also show that an entanglement-assisted scheme of the same reproduces the predictions of quantum mechanics. We put evidence that a local hidden variable theory is incompatible with quantum mechanical predictions by comparing the variation of intensities obtained from our experiment with hidden variable predictions.
Nuclear magnetic resonance (NMR) is a direct macroscopic manifestation of the quantum mechanics of the intrinsic angular momentum of atomic nuclei. It is best known for its extraordinary range of applications, which include molecular structure determination, medical imaging, and measurements of flow and diffusion rates. Most recently, liquid-state NMR spectroscopy has been found to provide a powerful experimental tool for the development and evaluation of the coherent control techniques needed for quantum information processing. This burgeoning new interdisciplinary field has the potential to achieve cryptographic, communications, and computational feats far beyond what is possible with known classical physics. Indeed, NMR has made the demonstration of many of these feats sufficiently simple to be carried out by high school summer interns working in our laboratory (see the last two authors). In this paper the basic principles of quantum information processing by NMR spectroscopy are described, along with several illustrative experiments suitable for incorporation into the undergraduate physics curriculum. These experiments are spin–spin interferometry, an implementation of the quantum Fourier transform, and the quantum simulation of a harmonic oscillator.
We propose and experimentally demonstrate an efficient framework for the quantum simulation of quantum channels in nuclear magnetic resonance (NMR). Our approach relies on the suitable decomposition of nonunitary operators in a linear combination of ddd unitary ones, which can be then experimentally implemented with the assistance of a number of ancillary qubits that grows logarithmically in ddd. As a proof-of-principle demonstration, we realize the quantum simulation of three quantum channels for a single-qubit: phase damping, amplitude damping, and depolarizing channels. For these paradigmatic cases, we measure key features, such as the fidelity of the initial state and the associated von Neumann entropy for a qubit evolving through these channels. Our experiments are carried out using nuclear spins in a liquid sample and NMR control techniques.