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arXiv:1112.0338 · Journal of Physics B Atomic Molecular and Optical Physics

Atomic frequency comb storage as a slow-light effect

M Bonarota, J.-L. Le Gouët, Sergey A. Moiseev, T. Chanelière

Published Jun 8, 2012• 21 citations
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Abstract

Atomic Frequency Comb (AFC) protocol has been particularly successful recently to demonstrate the storage of quantum information in a solid medium (rare-earth doped crystals). The AFC is inspired by the photon-echo technique. We show in this paper that the AFC is actually closely related to the slow-light based storage protocols extensively used in atomic vapours. Experimental verifications are performed in thulium doped YAG (Tm3+:YAG). We clarify the interplay between absorption and dispersion and propose a classification of the existing protocols.

DOI
10.1088/0953-4075/45/12/124002

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Rare-earth-doped crystals are promising candidates for quantum storage, yet their performance in free-space configurations is fundamentally restricted by low optical depth. Here, we demonstrate high-efficiency quantum storage in a stoichiometric EuCl3⋅_3 \cdot3​⋅ 6D2_22​O crystal, which intrinsically provides high optical density without the complexity of cavity implementation. We show that in this high-density regime, the system exhibits significant slow-light-like effects, including dispersion-induced echo delays and finesse-dependent echo intensity modulation. We develop a unified theoretical framework showing how absorption and dispersion work in concert to mediate echo generation. We achieve storage efficiencies of 42.9% for classical light and 34.4% for weak coherent pulses, alongside 90% efficiency for slow-light storage. These findings validate EuCl3⋅_3 \cdot3​⋅ 6D2_22​O as a robust platform, establishing a viable pathway for scalable solid-state quantum memory.
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Photon echoes in rare-earth-doped crystals are studied to understand the challenges of making broadband quantum memories using the atomic frequency comb (AFC) protocol in systems with hyperfine structure. The hyperfine structure of Pr 3+ poses an obstacle to this goal because frequencies associated with the hyperfine transitions change the simple picture of modulation at an externally imposed frequency. The current work focuses on the intermediate case where the hyperfine spacing is comparable to the comb spacing, a challenging regime that has recently been considered. Operating in this regime may facilitate storing quantum information over a larger spectral range in such systems. In this work, we prepare broadband AFCs using optical combs with tooth spacings ranging from 1 MHz to 16 MHz in fine steps, and measure transmission spectra and photon echoes for each. We predict the spectra and echoes theoretically using the optical combs as input to either a rate equation code or a density matrix code, which calculates the redistribution of populations. We then use the redistributed populations as input to a semiclassical theory using the frequency-dependent dielectric function. The two sets of predictions each give a good, but different account of the photon echoes.
This thesis describes experiments aimed at developing a key component in applications such as quantum networks and long-distance quantum communication systems: quantum memories. Quantum memories for light using photon-echo and coherent rephrasing techniques have been developed. The work is carried out on rare-earth-ion-doped inorganic crystals. Several properties are associated with these crystals such as long coherence times and long-lived ground state sublevels that are particularly interesting in connection applications in the area of quantum information science. It is demonstrated the preparation of optical inhomogeneous absorption profiles such that the light only interacts with a specific transition at a selected frequency. Narrow absorbing structures with widths of <100 kHz have been prepared with no absorption in the surrounding spectral interval. Most of the experiments were carried out using Pr3+:Y2SiO5. However, in our search for suitable a Λ-system in the material under consideration, we also performed spectral hole-burning spectroscopy in Nd:Y2SiVO4. As part of the search for host materials for Pr, Pr:La2(WO4)3 crystal was characterized using a variety of methods, such as, hole burning and photon-echoes. Electromagnetically induced transparency was also observed in this crystal. The most important criteria for evaluating quantum memory performance and the most important physical requirements are discussed. After investigating the standard photon echo techniques and controlled reversible inhomogeneous broadening (CRIB) for quantum state storage, we considered an efficient multimode quantum memory protocol; the atomic frequency comb (AFC) protocol. Combs with peaks of widths 100-300 kHz and an optical depth of~ 10 were created by optical pumping inside an emptied region of the inhomogeneous profile of Pr3+:Y2SiO5, allowing us to improve the efficiency of light storage. Light storage combining a photon-echo technique based on an AFC and spin-wave storage have been demonstrated, and an experimental AFC scheme for the storage of weak coherent light pulses in Pr3+:Y2SiO5 is presented. Finally, we have investigated superradiance and slow light effects. Both these effects occur in the high optical depth regime and can influence the memory performance. Under certain conditions superradiance results in the immediate re-emission of the stored light in a single burst of coherent radiation, and inside spectrally structured materials, slow light effects may result when storage is performed.