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arXiv:1111.4607

Inversion-free, noiseless Raman echoes

Byoung Seung HAM

Published Nov 20, 2011• 0 citations
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Abstract

Using double optical Raman rephasing, an inversion-free resonant Raman echo is studied in an inhomogeneously broadened spin ensemble of a solid medium, where the Raman optical field-excited spin coherence has a frozen propagation vector. Unlike photon echoes whose quantum memory application is strictly limited due to πrephasing pulse-induced population inversion causing quantum noises, the optical Raman field-excited spin echo is inherently silent owing to the frozen propagation vector. Thus, the doubly rephased Raman echo can be directly applied for quantum interface in a population inversion-free environment.

DOI
10.48550/arxiv.1111.4607

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Using double optical Raman rephasing, an inversion-free resonant Raman echo is studied in an inhomogeneously broadened spin ensemble of a solid medium, where the Raman optical field-excited spin coherence has a frozen propagation vector. Unlike photon echoes whose quantum memory application is strictly limited due to πrephasing pulse-induced population inversion causing quantum noises, the optical Raman field-excited spin echo is inherently silent owing to the frozen propagation vector. Thus, the doubly rephased Raman echo can be directly applied for quantum interface in a population inversion-free environment.
Rephasing in photon echoes is a fundamental mechanism of retrieving optical information stored in a collective ensemble of atoms or ions. With an extremely weak quantum optical data, population inversion by the rephasing process is inevitable resulting in serious quantum noise. Here, an inversion-free rephasing method in photon echoes is presented by using deshelving-based atom phase control. The present method makes photon echoes directly applicable to quantum memories with benefits of extended photon storage time and nearly perfect retrieval efficiency. In this revised version only the rephasing pulse propagation direction is corrected to make a silent echo of E1 in Fig. 1.
We investigate the use of resonant optical Raman pulses to excite and rephase ground state spin coherences via the partial storage or shelving of atoms. Unlike direct-rf-excited spin echoes or off-resonant Raman echoes, the resonant Raman optical field efficiently excites and rephases the spin coherence using \ensuremath{\pi} and 2\ensuremath{\pi} pulses, respectively. In a crystal of Pr3+{\mathrm{Pr}}^{3+}Pr3+ doped Y2SiO5,{\mathrm{Y}}_{2}{\mathrm{SiO}}_{5},Y2​SiO5​, we experimentally observe spin echo efficiency as high as 46% of the free induction decay signal.
Unlike slow-light-based quantum memories, photon echoes offer the benefit of high speed and wide bandwidth. Over the last decade, the rephasing mechanism of photon echoes has been studied for quantum memories to overcome fundamental limitations in photon echoes, such as population inversion and low retrieval efficiency. Although these limitations have been overcome in modified photon echo schemes, photon storage time is still too short to apply it to long-distance quantum communications. For long-distance quantum communications, ultralong photon storage time of the order of seconds is needed to implement quantum repeaters. In this review article, challenging techniques for ultralong photon storage are presented, where ultralong storage is obtained via a coherence conversion process between optical and spin states by using an optical locking technique. To remove population-inversion-caused quantum noise, a double rephasing scheme is addressed, where rephasing-pulse-caused population inversion hinders photon echoes for quantum memory applications.
Quantum coherence control is reinvestigated for a new physical insight in quantum nonlinear optics and applied for a wavelength-convertible quantum memory in a solid ensemble whose spin states are inhomogeneously broadened. Unlike typical atomic media whose spin decays are homogeneous, a spin inhomogeneously broadened solid ensemble requires a counter-intuitive quantum coherence control to avoid spontaneous emission-caused quantum noises. Such a quantum coherence control in a solid ensemble satisfying both near perfect retrieval efficiency and ultralong photon storage offers a solid framework to quantum repeaters, scalable qubit generations, quantum cryptography, and highly sensitive magnetometry. Here, the basic physics of the counter-intuitive quantum coherence control is presented not only for a fundamental understanding of collective ensemble phase control but also for a coherence conversion mechanism between optical and spin states involving Raman rephasing.