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arXiv:1110.5330 · Physical Review A

d -wave superfluidity in optical lattices of ultracold polar molecules

Kevin A. Kuns, Ana María Rey, Alexey Vyacheslavovich Gorshkov

Published Dec 29, 2011• 27 citations
arXivHTMLPDF

Abstract

Recent work on ultracold polar molecules, governed by a generalization of the $t$-$J$ Hamiltonian, suggests that molecules may be better suited than atoms for studying $d$-wave superfluidity due to stronger interactions and larger tunability of the system. We compute the phase diagram for polar molecules in a checkerboard lattice consisting of weakly coupled square plaquettes. In the simplest experimentally realizable case where there is only tunneling and an $XX$-type spin-spin interaction, we identify the parameter regime where $d$-wave superfluidity occurs. We also find that the inclusion of a density-density interaction destroys the superfluid phase and that the inclusion of a spin-density or an Ising-type spin-spin interaction can enhance the superfluid phase. We also propose schemes for experimentally realizing the perturbative calculations exhibiting enhanced $d$-wave superfluidity.

DOI
10.1103/physreva.84.063639

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Recent work on ultracold polar molecules, governed by a generalization of the ttt-JJJ Hamiltonian, suggests that molecules may be better suited than atoms for studying ddd-wave superfluidity due to stronger interactions and larger tunability of the system. We compute the phase diagram for polar molecules in a checkerboard lattice consisting of weakly coupled square plaquettes. In the simplest experimentally realizable case where there is only tunneling and an XXXXXX-type spin-spin interaction, we identify the parameter regime where ddd-wave superfluidity occurs. We also find that the inclusion of a density-density interaction destroys the superfluid phase and that the inclusion of a spin-density or an Ising-type spin-spin interaction can enhance the superfluid phase. We also propose schemes for experimentally realizing the perturbative calculations exhibiting enhanced ddd-wave superfluidity.
By selecting two dressed rotational states of ultracold polar molecules in an optical lattice, we obtain a highly tunable generalization of the $t\mathrm{\text{\ensuremath{-}}}J$ model, which we refer to as the $t\mathrm{\text{\ensuremath{-}}}J\mathrm{\text{\ensuremath{-}}}V\mathrm{\text{\ensuremath{-}}}W$ model. In addition to XXZXXZXXZ spin exchange, the model features density-density interactions and density-spin interactions; all interactions are dipolar. We show that full control of all interaction parameters in both magnitude and sign can be achieved independently of each other and of the tunneling. As a first step towards demonstrating the potential of the system, we apply the density matrix renormalization group method to obtain the 1D phase diagram of the simplest experimentally realizable case. Specifically, we show that the tunability and the long-range nature of the interactions in the $t\mathrm{\text{\ensuremath{-}}}J\mathrm{\text{\ensuremath{-}}}V\mathrm{\text{\ensuremath{-}}}W$ model enable enhanced superfluidity. Finally, we show that Bloch oscillations in a tilted lattice can be used to probe the phase diagram experimentally.
We compute physical properties across the phase diagram of the $t\ensuremath{-}{J}_{\ensuremath{\perp}}$ chain with long-range dipolar interactions, which describe ultracold polar molecules on optical lattices. Our results obtained by the density-matrix renormalization group indicate that superconductivity is enhanced when the Ising component Jz{J}_{z}Jz​ of the spin-spin interaction and the charge component VVV are tuned to zero and even further by the long-range dipolar interactions. At low densities, a substantially larger spin gap is obtained. We provide evidence that long-range interactions lead to algebraically decaying correlation functions despite the presence of a gap. Although this has recently been observed in other long-range interacting spin and fermion models, the correlations in our case have the peculiar property of having a small and continuously varying exponent. We construct simple analytic models and arguments to understand the most salient features.
We study a system of ultracold fermionic polar molecules in a two-dimensional square lattice interacting via both the long-range dipole-dipole interaction and a short-range on-site attractive interaction. Singlet-superfluid, change density wave, and supersolid phases are found to exist in the system. We map out the zero-temperature phase diagram and find that the supersolid phase is considerably stabilized by the dipole-dipole interaction and thus can exist over a large region of filling factors. We study the melting of the supersolid phase with increasing temperature, map out a finite-temperature phase diagram of the system at fixed filling, and determine the parameter region where the supersolid phase can possibly be observed in experiments.
This dissertation summarizes my recent work regarding systems of strongly interacting fermionic atoms in optical lattices. This work addresses the combination of two experimental techniques that have been the subject of much recent research in ultracold atom physics. One is the use of optical lattices, which provide a means to realize diverse interaction configurations within a clean, controllable system. The other is the use of magnetically tunable Feshbach resonances to control the strength of the interatomic interaction. Together, these techniques offer the possibility of an experimental realization of many important model Hamiltonians of condensed matter physics, and may also lead to the discovery of new physics. Recent study of this system has shown that strong interactions near Feshbach resonance will lead to the population of multiple lattice bands, and that collisions between atoms on neighboring sites cannot be neglected. These effects lead to a complicated Hamiltonian, but one which can be simplified to an effective single-band model equivalent to the generalized Hubbard model (GHM), which is an extension of the Hubbard model that includes correlated hopping terms. My main results concern the study of this model. The strong correlations between the particles make it difficult to definitively determine the many body physics of the GHM. As a first approach to understanding the GHM in optical lattices, I focus mainly on cases where the problem is greatly simplified by allowing interactions among only small groups of lattice sites. This restriction can be implemented in experiments using an optical superlattice potential. Our results include a proposed scheme (based on double-well superlattices) to empirically verify that the GHM describes this system and to directly measure the various parameters of this model. Other results include exact solutions on four-site square plaquettes, which demonstrate that d-wave excitations can occur in the low-energy states. By using a superlattice to give an array of weakly coupled plaquettes, one can thus produce a d-wave superfluid state. This is of relevance to the study of high-Tc superconductors, although I note certain key differences between the sort of d-wave superfluid described here and that of the superconductors.
We investigate many-body phase diagrams of atomic boson-fermion mixtures loaded in the two-dimensional optical lattice. Bosons mediate an attractive, finite-range interaction between fermions, leading to fermion pairing phases of different orbital symmetries. Specifically, we show that by properly tuning atomic and lattice parameters it is possible to create superfluids with sss-, ppp-, and ddd-wave pairing symmetry as well as spin and charge density wave phases. These phases and their stability are analyzed within the mean-field approximation for systems of $^{40}\mathrm{K}\text{\ensuremath{-}}^{87}\mathrm{Rb}$ and $^{40}\mathrm{K}\text{\ensuremath{-}}^{23}\mathrm{Na}$ mixtures. For the experimentally accessible regime of parameters, superfluids with unconventional fermion pairing have transition temperature around a percent of the Fermi energy.
The molecular Hubbard Hamiltonian (MHH) naturally arises for ultracold ground-state polar alkali-metal dimer molecules in optical lattices. We show that, unlike ultracold atoms, different molecules display different many-body phases due to intrinsic variances in molecular structure even when the molecular symmetry is the same. We also demonstrate a wide variety of experimental controls on ${}^{1}\ensuremath{\Sigma}$ molecules via external fields, including applied static electric and magnetic fields, an ac microwave field, and the polarization and strength of optical lattice beams. We provide explicit numerical calculations of the parameters of the MHH, including tunneling and direct and exchange dipole-dipole interaction energies, for the molecules 6{}^{6}6Li133{}^{133}133Cs, 23{}^{23}23Na40{}^{40}40K, 87{}^{87}87Rb133{}^{133}133Cs, 40{}^{40}40K87{}^{87}87Rb, and 6{}^{6}6Li23{}^{23}23Na in weak and strong applied electric fields. As case studies of many-body physics, we use infinite-size matrix product state methods to explore the quantum phase transitions from the superfluid phase to half-filled and third-filled crystalline phases in one dimension.