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arXiv:1109.2464 · Physical Review Letters

Density Instabilities in a Two-Dimensional Dipolar Fermi Gas

Meera M. Parish, Francesca Maria Marchetti

Published Apr 5, 2012• 63 citations
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Abstract

We study the density instabilities of a two-dimensional gas of dipolar fermions with aligned dipole moments. The random phase approximation (RPA) for the density-density response function is never accurate for the dipolar gas, and so we incorporate correlations beyond RPA via an improved version of the Singwi-Tosi-Land-Sjölander scheme. In addition to density-wave instabilities, our formalism captures the collapse instability that is expected from Hartree-Fock calculations but is absent from RPA. Crucially, we find that when the dipoles are perpendicular to the layer, the system spontaneously breaks rotational symmetry and forms a stripe phase, in defiance of conventional wisdom.

DOI
10.1103/physrevlett.108.145304

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We study the density instabilities of a two-dimensional gas of dipolar fermions with aligned dipole moments. The random phase approximation (RPA) for the density-density response function is never accurate for the dipolar gas, and so we incorporate correlations beyond RPA via an improved version of the Singwi-Tosi-Land-Sjölander scheme. In addition to density-wave instabilities, our formalism captures the collapse instability that is expected from Hartree-Fock calculations but is absent from RPA. Crucially, we find that when the dipoles are perpendicular to the layer, the system spontaneously breaks rotational symmetry and forms a stripe phase, in defiance of conventional wisdom.
We investigate the phase diagram of dipolar fermions with aligned dipole moments in a two-dimensional (2D) bilayer. Using a version of the Singwi-Tosi-Land-Sj\"olander scheme recently adapted to dipolar fermions in a single layer [M. M. Parish and F. M. Marchetti, Phys. Rev. Lett. 108, 145304 (2012)], we determine the density-wave instabilities of the bilayer system within linear response theory. We find that the bilayer geometry can stabilize the collapse of the 2D dipolar Fermi gas with intralayer attraction to form a new density wave phase that has an orientation perpendicular to the density wave expected for strong intralayer repulsion. We thus obtain a quantum phase transition between stripe phases that is driven by the interplay between strong correlations and the architecture of the low-dimensional system.
We consider a uniform dipolar Fermi gas in two dimensions (2D) where the dipole moments of fermions are aligned by an orientable external field. We obtain the ground state of the gas in the Hartree-Fock approximation and investigate random-phase-approximation stability against density fluctuations of finite momentum. It is shown that the density-wave instability takes place in a broad region where the system is stable against collapse. We also find that the critical temperature can be a significant fraction of Fermi temperature for a realistic system of polar molecules.
We investigate the behavior of identical dipolar fermions with aligned dipole moments in two-dimensional multilayers at zero temperature. We consider density instabilities that are driven by the attractive part of the dipolar interaction and, for the case of bilayers, we elucidate the properties of the stripe phase recently predicted to exist in this interaction regime. When the number of layers is increased, we find that this ``attractive'' stripe phase exists for an increasingly larger range of dipole angles, and if the interlayer distance is sufficiently small, the stripe phase eventually spans the full range of angles, including the situation where the dipole moments are aligned perpendicular to the planes. However, in this regime, we expect the behavior to be strongly modified by the binding of dipoles between layers. In the limit of an infinite number of layers, we derive an analytic expression for the mean-field interlayer effects in the density-density response function and, using this result, we find that the stripe phase is replaced by a collapse of the dipolar system.
The rapid progress in the production and cooling of molecular gases indicates that experimental studies of quantum gases with a strong dipolar interaction is soon within reach. Dipolar gases are predicted to exhibit very rich physics including quantum liquid crystal phases such as density waves as well as superfluid phases, both of which play an important role for our understanding of strongly correlated systems. Here, we investigate the zero temperature properties of the density-wave phase of a two-dimensional (2D) system of fermionic dipoles using a conserving Hartree-Fock theory. We calculate the amplitude of the density waves as a function of the dipole moment and orientation with respect to the 2D plane. The stripes give rise to a 1D Brillouin zone structure, and the corresponding quasiparticle spectrum is shown to have gapped as well as gapless regions around the Fermi surface. As a result, the system remains compressible in the density-wave phase, and it collapses for strong attraction. We show that the density waves have clear signatures in the momentum distribution and in the momentum correlations. Both can be measured in time-of-flight experiments. Finally, we discuss how the striped phase can be realized with experimentally available systems.
Density-functional theory is utilized to investigate the zero-temperature transition from a Fermi liquid to an inhomogeneous stripe, or Wigner crystal phase, predicted to occur in a one-component, spin-polarized, two-dimensional dipolar Fermi gas. Correlations are treated semiexactly within the local-density approximation using an empirical fit to quantum Monte Carlo data. We find that the inclusion of the nonlocal contribution to the Hartree-Fock energy is crucial for the onset of an instability to an inhomogeneous density distribution. Our density-functional theory supports a transition to both a one-dimensional stripe phase and a triangular Wigner crystal. However, we find that there is an instability first to the stripe phase, followed by a transition to the Wigner crystal at higher coupling.
We study the in-plane and out-of-plane density ordering instabilities of quasi-two-dimensional fermionic polar molecules in single-layer and multilayer configurations. We locate the soft modes by evaluating linear response functions within the conserving time-dependent Hartree-Fock (TDHF) approximation. The short-range exchange effects are taken into account by solving the Bethe-Salpeter integral equation numerically. An instability phase diagram is calculated for both single-layer and multilayer systems and the unstable wave vector is indicated. In all cases, the in-plane density wave instability is found to precede the out-of-plane instability. The unstable wave vector is found to be approximately twice the Fermi wave vector of one of the subbands at a time and can change discontinuously as a function of density and dipolar interaction strength. In multilayer configurations, we find a large enhancement of density-wave instability driven by dilute quasiparticles in the first excited subband. Finally, we provide a simple qualitative description of the phase diagrams using an RPA-like approach. Compared to previous works done within the RPA approximation, we find that inclusion of exchange interactions stabilize the normal liquid phase further and increase the critical dipolar interaction strength corresponding to the onset of density-wave instability by over a factor of two.