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arXiv:1109.0146 · Physical Review A

Control of inhomogeneous atomic ensembles of hyperfine qudits

Brian Mischuck, Seth Merkel, Ivan Deutsch

Published Feb 3, 2012• 37 citations
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Abstract

We study the ability to control $d$-dimensional quantum systems (qudits) encoded in the hyperfine spin of alkali-metal atoms through the application of radio- and microwave-frequency magnetic fields in the presence of inhomogeneities in amplitude and detuning. Such a capability is essential to the design of robust pulses that mitigate the effects of experimental uncertainty and also for application to tomographic addressing of particular members of an extended ensemble. We study the problem of preparing an arbitrary state in the Hilbert space from an initial fiducial state. We prove that inhomogeneous control of qudit ensembles is possible based on a semianalytic protocol that synthesizes the target through a sequence of alternating rf and microwave-driven SU(2) rotations in overlapping irreducible subspaces. Several examples of robust control are studied, and the semianalytic protocol is compared to a brute-force, full numerical search. For small inhomogeneities, $<$$1%$, both approaches achieve average fidelities greater than 0.99, but the brute-force approach performs superiorly, reaching high fidelities in shorter times and capable of handling inhomogeneities well beyond experimental uncertainty. The full numerical search is also applied to tomographic addressing whereby two different nonclassical states of the spin are produced in two halves of the ensemble.

DOI
10.1103/physreva.85.022302

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We study the ability to control ddd-dimensional quantum systems (qudits) encoded in the hyperfine spin of alkali-metal atoms through the application of radio- and microwave-frequency magnetic fields in the presence of inhomogeneities in amplitude and detuning. Such a capability is essential to the design of robust pulses that mitigate the effects of experimental uncertainty and also for application to tomographic addressing of particular members of an extended ensemble. We study the problem of preparing an arbitrary state in the Hilbert space from an initial fiducial state. We prove that inhomogeneous control of qudit ensembles is possible based on a semianalytic protocol that synthesizes the target through a sequence of alternating rf and microwave-driven SU(2) rotations in overlapping irreducible subspaces. Several examples of robust control are studied, and the semianalytic protocol is compared to a brute-force, full numerical search. For small inhomogeneities, <$$1%, both approaches achieve average fidelities greater than 0.99, but the brute-force approach performs superiorly, reaching high fidelities in shorter times and capable of handling inhomogeneities well beyond experimental uncertainty. The full numerical search is also applied to tomographic addressing whereby two different nonclassical states of the spin are produced in two halves of the ensemble.
We study quantum control of the full hyperfine manifold in the ground-electronic state of alkali-metal atoms based on applied radio frequency and microwave fields. Such interactions should allow essentially decoherence-free dynamics and the application of techniques for robust control developed for NMR spectroscopy. We establish the conditions under which the system is controllable in the sense that one can generate an arbitrary unitary map on the system. We apply this to the case of 133Cs^{133}\mathrm{Cs}133Cs with its d=16d=16d=16 dimensional Hilbert space of magnetic sublevels in the 6S1∕26{S}_{1∕2}6S1∕2​ state, and design control wave forms that generate an arbitrary target state from an initial fiducial state. We develop a generalized Wigner function representation for this space consisting of the direct sum of two irreducible representations of SU(2), allowing us to visualize these states. The performance of different control scenarios is evaluated based on the ability to generate a high-fidelity operation in an allotted time with the available resources. We find good operating points commensurate with modest laboratory requirements.
We study the ability to implement unitary maps on states of the I=9/2I=9/2I=9/2 nuclear spin in 87Sr^{87}\mathrm{Sr}87Sr, a d=10d=10d=10 dimensional (qudecimal) Hilbert space, using quantum optimal control. Through a combination of nuclear spin resonance and a tensor ac Stark shift, by solely modulating the phase of a radio-frequency magnetic field, the system is quantum controllable. Alkaline-earth-metal atoms, such as 87Sr^{87}\mathrm{Sr}87Sr, have a very favorable figure of merit for such control due to narrow intercombination lines and the large hyperfine splitting in the excited states. We numerically study the quantum speed limit, optimal parameters, and the fidelity of arbitrary state preparation and full SU(10) maps, including the presence of decoherence due to optical pumping induced by the light-shifting laser. We also study the use of robust control to mitigate some dephasing due to inhomogeneities in the light shift. We find that with an rf Rabi frequency of ${\mathrm{\ensuremath{\Omega}}}_{\text{rf}}$ and 0.5% inhomogeneity in the the light shift we can prepare an arbitrary Haar-random state in a time $T=4.5\ensuremath{\pi}/{\mathrm{\ensuremath{\Omega}}}_{\text{rf}}$ with average fidelity $\ensuremath{\langle}{\mathcal{F}}_{\ensuremath{\psi}}\ensuremath{\rangle}=0.9992$, and an arbitrary Haar-random SU(10) map in a time $T=24\ensuremath{\pi}/{\mathrm{\ensuremath{\Omega}}}_{\text{rf}}$ with average fidelity $\ensuremath{\langle}{\mathcal{F}}_{U}\ensuremath{\rangle}=0.9923$.
Quantum state reconstruction based on weak continuous measurement has the advantage of being fast, accurate and almost non-perturbative. In this work we present a pedagogical review of the protocol proposed by Silberfarb et al (2005 Phys. Rev. Lett. 95 030402), whereby an ensemble of identically prepared systems is collectively probed and controlled in a time-dependent manner so as to create an informationally complete continuous measurement record. The measurement history is then inverted to determine the state at the initial time through a maximum-likelihood estimate. The general formalism is applied to the case of reconstruction of the quantum state encoded in the magnetic sublevels of a large-spin alkali atom, 133 Cs. We detail two different protocols for control. Using magnetic interactions and a quadratic ac Stark shift, we can reconstruct a chosen hyperfine manifold F , e.g. the seven-dimensional F = 3 manifold in the electronic ground state of Cs. We review the procedure as implemented in experiments (Smith et al 2006 Phys. Rev. Lett. 97 180403). We extend the protocol to the more ambitious case of reconstruction of states in the full 16-dimensional electronic ground subspace ( F = 3⊕ F = 4), controlled by microwaves and radio-frequency (RF) magnetic fields. We give detailed derivations of all physical interactions, approximations, numerical methods and fitting procedures, tailored to the realistic experimental setting. For the case of light-shift and magnetic control, reconstruction fidelities of ∼0.95 have been achieved, limited primarily by inhomogeneities in the light-shift. For the case of microwave/RF-control we simulate fidelity >0.97, limited primarily by signal-to-noise.
Neutral atoms are promising candidates to store and manipulate quantum information. In this thesis we examine several problems related to the control of neutral atoms for quantum computation and simulation. In the first problem we show how the transport of atoms in an optical lattice can be controlled through variation of the polarization of the optical lattice and the application of global microwave pulses. This type of control control is a first step in many of the schemes for quantum computation and quantum simulation. We show that with the available tools for global control, the synthesis of any unitary transformation, consistent with translational invariance, may be performed and provide an explicit method for carrying this out. In the second problem, we study a spectroscopic method for probing atomic interactions that may form the basis for two-qudit quantum logic gates. The confinement of atoms required to perform quantum computation can strongly affect how they interact. Probing the nature of those confinement-induced effects is a first step towards quantum computing with neutral atoms. Transport of the atoms to overlapping wells is achieved through microwave pulses that drive population between hyperfine levels in a lin-perp-lin polarization-gradient lattice. By measuring the amount of population transferred into certain excited states, we can detect changes in the spectrum of the two-atom system induced by the interaction. In the third problem, we consider a cloud of cold atoms driven by both microwave and radio-frequency magnetic fields. The large number of spin sublevels available in individual atoms makes them candidates for a qudit-based quantum computer. Because the applied fields that drive the system may be inhomogeneous, the collection of atoms forms an ensemble of different qudits. Borrowing ideas developed for NMR control, we show how to drive the ensemble through a given evolution. We show that even in the presence of large experimental errors, state preparation may be achieved with high fidelities. We also show that intentionally applied variations in spatial magnetic fields can be used to synthesize different states in different regions of space.
Quantum systems with Hilbert space dimension greater than two (qudits) provide an alternative to qubits as carriers of quantum information, and may prove advantageous for quantum information tasks if good laboratory tools for qudit manipulation and readout can be developed. We have implemented a protocol for arbitrary unitary transformations in the 16 dimensional hyperfine ground manifold of Cesium 133 atoms, using phase modulated rf and microwave magnetic fields to drive the atomic evolution. Our phase modulation waveforms are designed numerically using a variant of the highly efficient GRAPE algorithm. The fidelity of the resulting transformations is verified experimentally through randomized benchmarking, which indicates an average fidelity better than 97% across a sample of random unitaries.
Quantum control in large dimensional Hilbert spaces is essential for realizing the power of quantum information processing. For closed quantum systems the relevant input/output maps are unitary transformations, and the fundamental challenge becomes how to implement these with high fidelity in the presence of experimental imperfections and decoherence. For two-level systems (qubits) most aspects of unitary control are well understood, but for systems with Hilbert space dimension d>2 (qudits), many questions remain regarding the optimal design of control Hamiltonians and the feasibility of robust implementation. Here we show that arbitrary, randomly chosen unitary transformations can be efficiently designed and implemented in a large dimensional Hilbert space (d=16) associated with the electronic ground state of atomic 133Cs, achieving fidelities above 0.98 as measured by randomized benchmarking. Generalizing the concepts of inhomogeneous control and dynamical decoupling to d>2 systems, we further demonstrate that these qudit unitary maps can be made robust to both static and dynamic perturbations. Potential applications include improved fault-tolerance in universal quantum computation, nonclassical state preparation for high-precision metrology, implementation of quantum simulations, and the study of fundamental physics related to open quantum systems and quantum chaos.