Observation of Correlated Particle-Hole Pairs and String Order in Low-Dimensional Mott Insulators
Manuel Endres, Marc Cheneau, Takeshi Fukuhara, Christof Weitenberg, Peter Schauß, C. Gross, Leonardo Mazza, Mari Carmen Bañuls, Lode Pollet, Immanuel Bloch, Stefan Kuhr
Quantum phases of matter are characterized by the underlying correlations of the many-body system. Although this is typically captured by a local order parameter, it has been shown that a broad class of many-body systems possesses a hidden nonlocal order. In the case of bosonic Mott insulators, the ground state properties are governed by quantum fluctuations in the form of correlated particle-hole pairs that lead to the emergence of a nonlocal string order in one dimension. By using high-resolution imaging of low-dimensional quantum gases in an optical lattice, we directly detect these pairs with single-site and single-particle sensitivity and observe string order in the one-dimensional case.
Quantum phases of matter are characterized by the underlying correlations of the many-body system. Although this is typically captured by a local order parameter, it has been shown that a broad class of many-body systems possesses a hidden nonlocal order. In the case of bosonic Mott insulators, the ground state properties are governed by quantum fluctuations in the form of correlated particle-hole pairs that lead to the emergence of a nonlocal string order in one dimension. By using high-resolution imaging of low-dimensional quantum gases in an optical lattice, we directly detect these pairs with single-site and single-particle sensitivity and observe string order in the one-dimensional case.
Exotic quantum many-body states, such as Haldane and spin liquid phases, can exhibit remarkable features like fractional excitations and non-Abelian statistics and offer new understandings of quantum entanglement in many-body quantum systems. These phases are classified by nonlocal correlators that can be directly measured in atomic analog quantum simulating platforms, such as optical lattices and Rydberg atom arrays. However, characterizing these phases in large systems is experimentally challenging because they are sensitive to local errors like atom loss, which suppress its signals exponentially. Additionally, protocols for systematically identifying and mitigating uncorrelated errors in analog quantum simulators are lacking. Here, we address these challenges by developing an error-correction method for large-scale neutral atom quantum simulators using optical lattices. Our error-correction method can distinguish correlated particle-hole pairs from uncorrelated holes in the Mott insulator. After removing the uncorrelated errors, we observe a dramatic improvement in the nonlocal parity correlator and find the perimeter scaling law. Furthermore, the error model provides a statistical estimation of fluctuations in site occupation, from which we measure the generalized brane correlator and confirm that it can be an order parameter for Mott insulators in two dimensions. Our work provides a promising avenue for investigating and characterizing exotic phases of matters in large-scale quantum simulators. Published by the American Physical Society 2024
Nonlocal order parameters capture the presence of correlated fluctuations between specific degrees of freedom, in otherwise disordered quantum matter. Here, we provide a further example of their fundamental role, deriving the ground state phase diagram of the filling one extended Bose-Hubbard model, exclusively in terms of their ordering. By means of a density matrix renormalization group numerical analysis, we show that in addition to the (even) parity order characteristic of the Mott insulating phase and the string order nonvanishing in the Haldane insulator, the recently proposed odd parity order completes the picture, becoming nonvanishing at the transition from the normal superfluid to the paired superfluid phase. The above three nonlocal parameters capture all the distinct phases, including the density wave phase, in which the local order is seen as the simultaneous presence of correlated fluctuations in different channels. They provide a unique tool for the experimental observation of the full phase diagram of strongly correlated quantum matter, by means of local density measurements.
The Mott-insulating phase of the two-dimensional (2D) Bose-Hubbard model is expected to be characterized by a nonlocal brane parity order.Parity order captures the presence of microscopic particlehole fluctuations and entanglement, whose properties depend on the underlying lattice geometry.We realize 2D Bose-Hubbard models in dynamically tunable lattice geometries, using neutral atoms in a passively phase-stable tunable optical lattice in combination with programmable site-blocking potentials.We benchmark the performance of our system by single-particle quantum walks in the square, triangular, kagome, and Lieb lattices.In the strongly correlated regime, we microscopically characterize the geometry dependence of the quantum fluctuations and experimentally validate brane parity as a proxy for the nonlocal order parameter signaling the superfluid-to-Mott-insulating phase transition.
We investigate the ground-state properties of a newly discovered phase of one-dimensional lattice bosons with extended interactions [E. G. Dalla Torre et al., Phys. Rev. Lett. 97, 260401 (2006)]. The new phase, termed the Haldane insulator in analogy with the gapped phase of spin-1 chains, is characterized by a nonlocal order parameter, which can only be written as an infinite string in terms of the bosonic densities. We show that the string order can nevertheless be probed with physical fields that couple locally, via the effect those fields have on the quantum phase transitions separating the exotic phase from the conventional Mott and density wave phases. Using a field theoretical analysis, we show that a perturbation that breaks lattice inversion symmetry gaps the critical point separating the Mott and Haldane phases and eliminates the sharp distinction between them. This is remarkable given that neither of these phases involves broken inversion symmetry. We also investigate the evolution of the phase diagram with the tunable coupling between parallel chains in an optical lattice setup. We find that interchain tunneling destroys the direct phase transition between the Mott and Haldane insulators by establishing an intermediate superfluid phase. On the other hand, coupling the chains only by weak repulsive interactions does not modify the structure of the phase diagram. The theoretical predictions are confirmed with numerical calculations using the density matrix renormalization group.
Correlation functions play an important role for the theoretical and experimental characterization of many-body systems. In solid-state systems, they are usually determined through scattering experiments, whereas in cold gases systems, time-of-flight, and in situ absorption imaging are the standard observation techniques. However, none of these methods allow the in situ detection of spatially resolved correlation functions at the single-particle level. Here, we give a more detailed account of recent advances in the detection of correlation functions using in situ fluorescence imaging of ultracold bosonic atoms in an optical lattice. This method yields single-site- and single-atom-resolved images of the lattice gas in a single experimental run, thus gaining direct access to fluctuations in the many-body system. As a consequence, the detection of correlation functions between an arbitrary set of lattice sites is possible. This enables not only the detection of two-site correlation functions but also the evaluation of non-local correlations, which originate from an extended region of the system and are used for the characterization of quantum phases that do not possess (quasi-)long-range order in the traditional sense.
Ultracold atoms in optical lattices provide an extremely clean and controllable setting to explore quantum many-body phases of matter. Here we give a brief review of the strong-correlation physics that has been realized using such ultracold atoms in optical lattices ranging from the realization of Hubbard models to studies of quantum magnetism and the detection of single atoms with lattice site resolution. All this has opened up fundamentally new opportunities for the investigation of quantum many-body systems. Introduction Over the past years, ultracold atoms in optical lattices have emerged as versatile new systems to explore the physics of quantum many-body systems. On the one hand, they can be helpful in gaining a better understanding of known phases of matter and their dynamical behavior; on the other hand, they allow one to realize completely novel quantum systems that have not been studied before in nature [1, 2, 3]. Commonly, the approach of exploring quantum many-body systems in such a way is referred to as “quantum simulations.” Examples of some of the first strongly interacting many-body phases that have been realized both in lattices and in the continuum include the quantum phase transition from a superfluid to a Mott insulator [4, 5, 6], fermionic Mott insulators [7, 8], the achievement of a Tonks- Girardeau gas [9, 10], and the realization of the Bose-Einsten condensate (BEC)– Bardeen-Cooper-Schrieffer (BCS) crossover (see also Chapter 12) in Fermi gas mixture [11] using Feshbach resonances [12]. In almost all of these experiments, detection was limited to time-of-flight imaging or more refined derived techniques that mainly characterized the momentum distribution of the quantum gas [2]. For several years, researchers in the field have therefore aspired to employ in situ single-particle detection methods for the analysis of ultracold quantum gases. Only recently has it become possible to implement such imaging techniques, marking a milestone for the characterization and manipulation of ultracold quantum gases [13, 14, 15, 16, 17]. In our discussion, we will focus on one of the most successful of these techniques based on high-resolution fluorescence imaging. Despite being a rather new technique, such quantum gas microscopy has already proven to be an enabling technology for probing and manipulating quantum many-body systems. For the first time, controllable and strongly interacting many-body systems, as realized with ultracold atoms, could be observed on a local scale [17, 16].