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arXiv:1106.1013 · Physical Review B

Thermodynamics of the one-dimensional frustrated Heisenberg ferromagnet with arbitrary spin

M. Härtel, Johannes Richter, Dieter Ihle, Jürgen Schnack, S.‐L. Drechsler

Published Sep 6, 2011• 25 citations
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Abstract

The thermodynamic quantities (spin-spin correlation functions $\ensuremath{\langle}{\mathbf{S}}_{0}{\mathbf{S}}_{n}\ensuremath{\rangle}$, correlation length $\ensuremath{\xi}$, spin susceptibility $\ensuremath{\chi}$, and specific heat ${C}_{V}$) of the frustrated one-dimensional ${J}_{1}$-${J}_{2}$ Heisenberg ferromagnet with arbitrary spin quantum number $S$ below the quantum critical point, i.e., for ${J}_{2}<|{J}_{1}|/4$, are calculated using a rotation-invariant Green-function formalism and full diagonalization as well as a finite-temperature Lanczos technique for finite chains of up to $N=20$ sites. The low-temperature behavior of the susceptibility $\ensuremath{\chi}$ and the correlation length $\ensuremath{\xi}$ are well described by $\ensuremath{\chi}=\frac{2}{3}{S}^{4}\left(|{J}_{1}|\ensuremath{-}4{J}_{2}\right){T}^{\ensuremath{-}2}+A{S}^{5/2}{\left(|{J}_{1}|\ensuremath{-}4{J}_{2}\right)}^{1/2}{T}^{\ensuremath{-}3/2}$ and $\ensuremath{\xi}={S}^{2}\left(|{J}_{1}|\ensuremath{-}4{J}_{2}\right){T}^{\ensuremath{-}1}+B{S}^{1/2}{\left(|{J}_{1}|\ensuremath{-}4{J}_{2}\right)}^{1/2}{T}^{\ensuremath{-}1/2}$ with $A\ensuremath{\approx}1.1\ensuremath{\cdots}1.2$ and $B\ensuremath{\approx}0.84\ensuremath{\cdots}0.89$. The vanishing of the factors in front of the temperature at ${J}_{2}=|{J}_{1}|/4$ indicates a change of the critical behavior of $\ensuremath{\chi}$ and $\ensuremath{\xi}$ at $T\ensuremath{\rightarrow}0$. The specific heat may exhibit an additional frustration-induced low-temperature maximum when approaching the quantum critical point. Such a maximum appears for $S=1/2$ and $S=1$, but was not found for $S>1$.

DOI
10.1103/physrevb.84.104411

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