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arXiv:1104.4134 · Physical Review A

Photon-echo quantum memories in inhomogeneously broadened two-level atoms

D. L. McAuslan, Patrick M. Ledingham, William R. Naylor, Sarah E. Beavan, Morgan P. Hedges, Matthew J. Sellars, Jevon J. Longdell

Published Aug 5, 2011• 75 citations
arXivHTMLPDF

Abstract

Here, we propose a solid-state quantum memory that does not require spectral holeburning, instead using strong rephasing pulses like traditional photon-echo techniques. The memory uses external broadening fields to reduce the optical depth and so switch off the collective atom-light interaction when desired. The proposed memory should allow operation with reasonable efficiency in a much broader range of material systems, for instance Er${}^{3+}$ doped crystals which have a transition at 1.5 $\ensuremath{\mu}\text{m}$. We present analytic theory supported by numerical calculations and initial experiments.

DOI
10.1103/physreva.84.022309

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Here, we propose a solid-state quantum memory that does not require spectral holeburning, instead using strong rephasing pulses like traditional photon-echo techniques. The memory uses external broadening fields to reduce the optical depth and so switch off the collective atom-light interaction when desired. The proposed memory should allow operation with reasonable efficiency in a much broader range of material systems, for instance Er3+{}^{3+}3+ doped crystals which have a transition at 1.5 \ensuremathμm\ensuremath{\mu}\text{m}\ensuremathμm. We present analytic theory supported by numerical calculations and initial experiments.
The photon-echo quantum memory is based on a controlled rephasing of the atomic coherence excited by a signal light field in the inhomogeneously broadened resonant line. Here, we demonstrate an active mechanism of the atomic rephasing that provides a perfect retrieval of the stored light field in the photon-echo quantum memory based on the use of arbitrary initial inhomogeneous broadening of the resonant line. We show that the rephasing mechanism can exploit all resonant atoms, thereby maximally increasing an optical depth of the resonant transition, which is one of the critical parameters for the realization of highly efficient quantum memory. We also demonstrate that the rephasing mechanism can be used for various realizations of the photon-echo quantum memory, thereby creating many possibilities for its practical realization.
We propose a method to implement a quantum memory for light based on ensembles of two-level atoms. Our protocol is based on controlled reversible inhomogeneous broadening (CRIB), where an external field first dephases the atomic polarization and thereby stores an incoming light pulse into collective states of the atomic ensemble, and later a reversal of the applied field leads to a rephasing of the atomic polarization and a reemission of the light. As opposed to previous proposals for CRIB-based quantum memories, we propose only applying the broadening for a short period after most of the pulse has already been absorbed by the ensemble. We show that with this procedure there exist certain modes of the incoming light field that can be stored with an efficiency approaching 100% in the limit of high optical depth and long coherence time of the atoms. These results demonstrate that it is possible to operate an efficient quantum memory without any optical control fields.
We present a simple quantum memory scheme that allows for the storage of a light field in an ensemble of two-level atoms. The technique is analogous to the NMR gradient echo for which the imprinting and recalling of the input field are performed by controlling a linearly varying broadening. Our protocol is perfectly efficient in the limit of high optical depths and the output pulse is emitted in the forward direction. We provide a numerical analysis of the protocol together with an experiment performed in a solid state system. In close agreement with our model, the experiment shows a total efficiency of up to 15%, and a recall efficiency of 26%. We suggest simple realizable improvements for the experiment to surpass the no-cloning limit.
It has recently been discovered that the optical analog of a gradient echo, in an optically thick material, could form the basis of an optical memory that is both completely efficient and noise-free. Here we present analytical calculations showing that this is the case. There is close analogy between the operation of the memory and an optical system with two beam splitters. We can use this analogy to calculate efficiencies as a function of optical depth for a number of quantum memory schemes based on controlled inhomogeneous broadening. In particular, we show that multiple switching leads to a net 100% retrieval efficiency for the optical gradient echo even in the optically thin case.
Photon-echo-based quantum memories use inhomogeneously broadened, optically thick ensembles of absorbers to store a weak optical signal and employ various protocols to rephase the atomic coherences for information retrieval. We study the application of two consecutive, frequency-chirped control pulses for coherence rephasing in an ensemble with a ``natural'' inhomogeneous broadening. Although propagation effects distort the two control pulses differently, chirped pulses that drive adiabatic passage can rephase atomic coherences in an optically thick storage medium. Combined with spatial phase-mismatching techniques to prevent primary echo emission, coherences can be rephased around the ground state to achieve secondary echo emission with close to unit efficiency. Potential advantages over similar schemes working with $\ensuremath{\pi}$ pulses include greater potential signal fidelity, reduced noise due to spontaneous emission, and better capability for the storage of multiple memory channels.
We demonstrate experimentally the storage and retrieval of weak coherent light fields at telecommunication wavelengths in a solid. Light pulses at the single photon level are stored for a time up to 600 ns in an erbium-doped Y2SiO5 crystal at 2.6 K and retrieved on demand. The memory is based on photon echoes with controlled reversible inhomogeneous broadening, which is realized here for the first time at the single photon level. This is implemented with an external field gradient using the linear Stark effect. This experiment demonstrates the feasibility of a solid-state quantum memory for single photons at telecommunication wavelengths, which would represent an important resource in quantum information science.