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arXiv:1103.1638 · Physical Review B

Quantum phase transitions around the staggered valence-bond solid

Cenke Xu, Leon Balents

Published Jul 15, 2011• 41 citations
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Abstract

Motivated by recent numerical results, we study the quantum phase transitions between ${Z}_{2}$ spin-liquid, N\'eel-ordered, and various valence-bond solid (VBS) states on the honeycomb and square lattices, with emphasis on the staggered VBS. In contrast to the well-understood columnar VBS order, the staggered VBS is not described by an $\mathit{XY}$-order parameter with ${Z}_{N}$ anisotropy close to these quantum phase transitions. Instead, we demonstrate that on the honeycomb lattice, the staggered VBS is more appropriately described as an O(3)- or CP(2)-order parameter with cubic anisotropy, while on the square lattice it is described by an O(4)- or CP(3)-order parameter.

DOI
10.1103/physrevb.84.014402

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We study a spin-1/2 SU(2) model on the honeycomb lattice with nearest-neighbor antiferromagnetic exchange J that favors Néel order and competing six-spin interactions Q that favor a valence-bond-solid (VBS) state in which the bond energies order at the "columnar" wave vector K=(2π/3,-2π/3). We present quantum Monte Carlo evidence for a direct continuous quantum phase transition between Néel and VBS states, with exponents and logarithmic violations of scaling consistent with those at analogous deconfined critical points on the square lattice. Although this strongly suggests a description in terms of deconfined criticality, the measured threefold anisotropy of the phase of the VBS order parameter shows unusual near-marginal behavior at the critical point.
We consider the S=1/2S=1/2S=1/2 Heisenberg model with nearest-neighbor interaction JJJ and an additional multispin interaction Q3{Q}_{3}Q3​ on the square lattice. The Q3{Q}_{3}Q3​ term consists of three bond-singlet projectors and is chosen to favor the formation of a valence-bond solid (VBS) where the valence bonds (singlet pairs) form a staggered pattern. The model exhibits a quantum phase transition from the N\'eel state to the VBS as a function of Q3/J{Q}_{3}/JQ3​/J. We study the model using quantum Monte Carlo (stochastic series expansion) simulations. The N\'eel-VBS transition in this case is strongly first order in nature, in contrast to similar previously studied models with continuous transitions into columnar VBS states. The qualitatively different transitions illustrate the important role of an emerging U(1)U(1)U(1) symmetry in the latter case, which is not possible in the present model due to the staggered VBS pattern (which does not allow local fluctuations necessary to rotate the local VBS order parameter).
We study the N\'eel to fourfold columnar valence bond solid (cVBS) quantum phase transition in a sign-free S=1S=1S=1 square-lattice model. This is the same kind of transition that for S=1/2S=1/2S=1/2 has been argued to realize the prototypical deconfined critical point. Extensive numerical simulations of the square-lattice S=1/2S=1/2S=1/2 N\'eel-VBS transition have found consistency with the deconfined critical point scenario with no direct evidence for first-order behavior. In contrast to the S=1/2S=1/2S=1/2 case, in our quantum Monte Carlo simulations for the S=1S=1S=1 model, we present unambiguous evidence for a direct conventional first-order quantum phase transition. Classic signs of a first-order transition demonstrating coexistence including double-peaked histograms and switching behavior are observed. The sharp contrast from the S=1/2S=1/2S=1/2 case is remarkable; we hypothesize that this is a striking demonstration of the role of the size of the quantum spin in the phase diagram of two-dimensional lattice models.
We propose quantum phase transitions beyond the Landau's paradigm of Sp(4) spin Heisenberg models on the triangular and square lattices motivated by the exact $\text{Sp}(4)\ensuremath{\simeq}\text{SO}(5)$ symmetry of spin-3/2 fermionic cold atomic system with only sss-wave scattering. On the triangular lattice, we study a phase transition between the $\sqrt{3}\ifmmode\times\else\texttimes\fi{}\sqrt{3}$ spin ordered phase and a Z2{Z}_{2}Z2​ spin liquid phase; this phase transition is described by an O(8) sigma model in terms of fractionalized spinon fields, with significant anomalous scaling dimensions of spin order parameters. On the square lattice, we propose a deconfined critical point between the Neel order and the valence bond solid (VBS) order, which is described by the CP(3) model, and the monopole effect of the compact U(1) gauge field is expected to be suppressed at the critical point.