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arXiv:1103.1319 · Physical Review Letters

Artificial Atoms Can Do More Than Atoms: Deterministic Single Photon Subtraction from Arbitrary Light Fields

Jens Honer, R. Löw, Hendrik Weimer, Tilman Pfau, Hans Peter Büchler

Published Aug 25, 2011• 134 citations
arXivHTMLPDF

Abstract

We study the interplay of photons interacting with an artificial atom in the presence of a controlled dephasing. Such artificial atoms consisting of several independent scatterers can exhibit remarkable properties superior to single atoms with a prominent example being a superatom based on Rydberg blockade. We demonstrate that the induced dephasing allows for the controlled absorption of a single photon from an arbitrary incoming probe field. This unique tool in photon-matter interaction opens a way for building novel quantum devices, and several potential applications such as a single photon transistor, high fidelity n-photon counters, or the creation of nonclassical states of light by photon subtraction are presented.

DOI
10.1103/physrevlett.107.093601

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We study the interplay of photons interacting with an artificial atom in the presence of a controlled dephasing. Such artificial atoms consisting of several independent scatterers can exhibit remarkable properties superior to single atoms with a prominent example being a superatom based on Rydberg blockade. We demonstrate that the induced dephasing allows for the controlled absorption of a single photon from an arbitrary incoming probe field. This unique tool in photon-matter interaction opens a way for building novel quantum devices, and several potential applications such as a single photon transistor, high fidelity n-photon counters, or the creation of nonclassical states of light by photon subtraction are presented.
The preparation of light pulses with well-defined quantum properties requires precise control at the individual photon level. Here, we demonstrate exact and controlled multi-photon subtraction from incoming light pulses. We employ a cascaded system of tightly confined cold atom ensembles with strong, collectively enhanced coupling of photons to Rydberg states. The excitation blockade resulting from interactions between Rydberg atoms limits photon absorption to one per ensemble and rapid dephasing of the collective excitation suppresses stimulated re-emission of the photon. We experimentally demonstrate subtraction with up to three absorbers. Furthermore, we present a thorough theoretical analysis of our scheme where we identify weak Raman decay of the long-lived Rydberg state as the main source of infidelity in the subtracted photon number and investigate the performance of the multi-photon subtractor for increasing absorber numbers in the presence of Raman decay.
Abstract Quantum optics based on highly excited atoms, also known as Rydberg atoms, has cemented itself as a powerful platform for the manipulation of light at the few-photon level. The Rydberg blockade, resulting from the strong interaction between individual Rydberg atoms, can turn a large ensemble of atoms into a system which collectively resembles a single two-level emitter, a so-called Rydberg superatom. The coupling of this artificial emitter to a driving photonic mode is collectively enhanced by Rydberg interactions, enabling strong coherent coupling at the few-photon level in free-space. The exquisite level of control achievable through this has already demonstrated its utility in applications of quantum computing and information processing. Here, we review the derivation of the collective coupling between a Rydberg superatom and a single light mode and discuss the similarity of this free-space setup to waveguide quantum electrodynamics systems of quantum emitters coupled to photonic waveguides. We also briefly review applications of Rydberg superatoms to quantum optics such as single-photon generation and single-photon subtraction.
We investigate a hybrid quantum system that consists of a superatom coupled to a surface phonon-polariton. We apply this hybrid quantum system to subtract individual photons from a beam of light. Rydberg atom blockade is used to attain absorption of a single photon by an atomic microtrap. Surface phonon-polariton coupling to the superatom then triggers the transfer of the excitation to a storage state, a single Rydberg atom. The approach utilizes the interaction between a superatom and a Markovian bath that acts as a controlled decoherence mechanism to irreversibly project the superatom state into a single Rydberg atom state that can be read out.
We investigate a hybrid quantum system that consists of a superatom coupled to a surface phonon-polariton. We apply this hybrid quantum system to subtract individual photons from a beam of light. A Rydberg atom blockade is used to attain absorption of a single photon by an atomic microtrap. Surface phonon-polariton coupling to the superatom then triggers the transfer of the excitation to a storage state, a single Rydberg atom. The approach utilizes the interaction between a superatom and a Markovian bath that acts as a controlled decoherence mechanism to irreversibly project the superatom state into a single Rydberg atom state that can be read out.
The remarkable progress in control over cold atomic gases has led to a point where people are no longer satisfied with merely studying these systems, but rather put them to use to understand complex quantum many-body systems. The basis of this development is a deep understanding of the interaction between atoms, and how to exploit those in order to engineer interesting and novel quantum-systems. The aim of this particular thesis is to contribute to this third quantum revolution [1] and hence help to understand the inner workings of complex many-body systems. We present a method to control the shape and character of the interaction between cold atoms based on dressing the atomic ground-state with a Rydberg-state. The latter induces a van der Waals interaction between all the atoms in the ensemble, and allows for control via the coupling light-field. We find that with increasing atom densities the ensemble shows a direct transition into a collective regime that preempts the onset of three-body interactions associated with a break-down of the first Born-approximation. The reason for this intriguing behavior is the strong interaction between Rydberg atoms that gives rise to the blockade-mechanism, and prevents the simultaneous excitation to the Rydberg-state for spatially close atoms. The non-trivial behavior of the interaction-potential within the collective regime yields a novel tool for shaping the interaction between ground-state atoms beyond s-wave scattering. We study this collective regime and the resulting interaction-potential between the atoms within a variational/mean-field approach, and discuss its effects on a trapped Bose-Einstein condensate. Artificial atoms show remarkable properties, that are often superior to real atoms. In particular, since they are built out of many constituents, such systems often exhibit an enhanced coupling to the light-field as well as strong optical non-linearities even for small light-fields. On the other hand, noise in quantum-mechanical systems can not only destroy coherence, but rather can be used in order to robustly drive a system into an interesting state. We study the effect of a controlled dephasing onto an artificial atom in the context of an ensemble of atoms coherently coupled to a Rydberg state and demonstrate that such an enhanced artificial atom allows for the deterministic absorption of a single photon from an arbitrary incoming probe field. Such behavior yields a unique tool in light-matter interaction, and opens the path to realise quantum-networks or to fabricate novel quantum-devices. Here, we discuss the applicability of this single-photon absorber as a single-photon transistor, a high fidelity n-photon counter, and a device that allows for the deterministic creation of non-classical states of light via photon-subtraction. A non-trivial topological order of quantum-states leads to conservation of certain properties and, hence, increases their robustness against external perturbations. This can even stabilize quantum-states against local fluctuations. The latter usually corrupts the coherence within a macroscopic object and thereby prevents quantum-phenomena to occur in our macroscopic world. As an example of such a topological state, we study the behavior of vortex-excitations in a two-dimensional superfluid confined to a periodic potential, as can be realised within a cold atomic gas in an optical lattice. For large superfluid filling factors and strong interactions, the healing-length and, accordingly, the vortex core is much smaller than the lattice spacing. As a result, vortices are confined to the plaquettes of the lattice, and can be described in the framework of an effective tight-binding Hamiltonian. Via a first-principle calculation based on coherent-state path-integrals we derive the microscopic parameters of this model and provide an analytic expression for the vortex mass. Moreover, we show that such a quantum vortex is not obliged to follow the superfluid flow, but rather exhibits Bloch-oscillations perpendicular to it, which is a telltale sign for quantum interference of this macroscopic many-body excitation. Recently, Jonathan Simon et al. [2] performed a major step towards simulating quantum many-body systems in cold atomic gases by simulating the paramagnet-antiferro-magnet transition of a one-dimensional Ising-model. Fundamental excitations in the phase with broken translational symmetry are domain-walls carrying fractional statistics. The question is, whether experimentally accessible single-particle excitations, which correspond to two closely-bound domain-walls, decay into fractional excitations or remain closely-bound. By use of perturbation theory, we derive an analytic model for the time-evolution of these fractional excitations in the framework of a tilted Bose-Hubbard model, and demonstrate the existence of a repulsively bound state above a critical center-of-mass momentum. The validity of the perturbative approach is confirmed by the use of t-DMRG simulations. Together with the recent demonstration of single-site addressing and readout in optical lattices, these findings open the path for experimental observation of fractional excitations within cold atomic gases.
We report on the realization of a free-space single-photon absorber, which deterministically absorbs exactly one photon from an input pulse. Our scheme is based on the saturation of an optically thick medium by a single photon due to Rydberg blockade. By converting one absorbed input photon into a stationary Rydberg excitation, decoupled from the light field through fast engineered dephasing, we blockade the full atomic cloud and change our optical medium from opaque to transparent. We show that this results in the subtraction of one photon from the input pulse over a wide range of input photon numbers. We investigate the change of the pulse shape and temporal photon statistics of the transmitted light pulses for different input photon numbers and compare the results to simulations. Based on the experimental results, we discuss the applicability of our single-photon absorber for number resolved photon detection schemes or quantum gate operations.