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arXiv:1102.3560 · Physical Review A

Storing entanglement of nuclear spins via Uhrig dynamical decoupling

Soumya S. Roy, T. S. Mahesh, G. S. Agarwal

Published Jun 21, 2011• 28 citations
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Abstract

Stroboscopic spin flips have already been shown to prolong the coherence times of quantum systems under noisy environments. Uhrig's dynamical decoupling scheme provides an optimal sequence for a quantum system interacting with a dephasing bath. Several experimental demonstrations have already verified the efficiency of such dynamical decoupling schemes in preserving single-qubit coherences. In this work we describe the experimental study of Uhrig's dynamical decoupling in preserving two-qubit entangled states using an ensemble of spin-1/2 nuclear pairs in solution state. We find that the performance of odd-order Uhrig sequences in preserving entanglement is superior to both even-order Uhrig sequences and periodic spin-flip sequences. We also find that there exists an optimal order of the Uhrig sequence in which a singlet state can be stored at high correlation for about 30 seconds.

DOI
10.1103/physreva.83.062326

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Stroboscopic spin flips have already been shown to prolong the coherence times of quantum systems under noisy environments. Uhrig's dynamical decoupling scheme provides an optimal sequence for a quantum system interacting with a dephasing bath. Several experimental demonstrations have already verified the efficiency of such dynamical decoupling schemes in preserving single-qubit coherences. In this work we describe the experimental study of Uhrig's dynamical decoupling in preserving two-qubit entangled states using an ensemble of spin-1/2 nuclear pairs in solution state. We find that the performance of odd-order Uhrig sequences in preserving entanglement is superior to both even-order Uhrig sequences and periodic spin-flip sequences. We also find that there exists an optimal order of the Uhrig sequence in which a singlet state can be stored at high correlation for about 30 seconds.
Uhrig's dynamical decoupling pulse sequence has emerged as a universal and highly promising approach to decoherence suppression. So far, both the theoretical and experimental studies have examined single-qubit decoherence only. This work extends Uhrig's universal dynamical decoupling from one-qubit to two-qubit systems and even to general multilevel quantum systems. In particular, we show that by designing appropriate control Hamiltonians for a two-qubit or a multilevel system, Uhrig's pulse sequence can also preserve a generalized quantum coherence measure to the order of 1+O(TN+1)1+O({T}^{N+1})1+O(TN+1) with only NNN pulses. Our results lead to a very useful scheme for efficiently locking two-qubit entangled states. Future important applications of Uhrig's pulse sequence in preserving the quantum coherence of multilevel quantum systems can also be anticipated.
Avoiding the loss of coherence of quantum mechanical states is an important prerequisite for quantum information processing. Dynamical decoupling (DD) is one of the most effective experimental methods for maintaining coherence, especially when one can access only the qubit system and not its environment (bath). It involves the application of pulses to the system whose net effect is a reversal of the system-environment interaction. In any real system, however, the environment is not static, and therefore the reversal of the system-environment interaction becomes imperfect if the spacing between refocusing pulses becomes comparable to or longer than the correlation time of the environment. The efficiency of the refocusing improves therefore if the spacing between the pulses is reduced. Here, we quantify the efficiency of different DD sequences in preserving different quantum states. We use 13C^{13}\mathrm{C}13C nuclear spins as qubits and an environment of 1H^{1}\mathrm{H}1H nuclear spins as the environment, which couples to the qubit via magnetic dipole-dipole couplings. Strong dipole-dipole couplings between the proton spins result in a rapidly fluctuating environment with a correlation time of the order of 100 $\ensuremath{\mu}$s. Our experimental results show that short delays between the pulses yield better performance if they are compared with the bath correlation time. However, as the pulse spacing becomes shorter than the bath correlation time, an optimum is reached. For even shorter delays, the pulse imperfections dominate over the decoherence losses and cause the quantum state to decay.
In quantum information processing, it is vital to protect the coherence of qubits in noisy environments. Dynamical decoupling (DD), which applies a sequence of flips on qubits and averages the qubit-environment coupling to zero, is a promising strategy compatible with other desired functionalities, such as quantum gates. Here, we review the recent progresses in theories of dynamical decoupling and experimental demonstrations. We give both semiclassical and quantum descriptions of the qubit decoherence due to coupling to noisy environments. Based on the quantum picture, a geometrical interpretation of DD is presented. The periodic Carr-Purcell-Meiboom-Gill DD and the concatenated DD are reviewed, followed by a detailed exploration of the recently developed Uhrig DD, which employs the least number of pulses in an unequally spaced sequence to suppress the qubit-environment coupling to a given order of the evolution time. Some new developments and perspectives are also discussed.
Dynamical decoupling (DD) sequences were invented to eliminate the direct coupling between a qubit and its environment. We further investigate the possibility of decoupling the indirect qubit–qubit interaction induced by a common environment, and successfully find simplified solutions that preserve the bipartite quantum states to arbitrary order. Through analysing the exact dynamics of the controlled two-qubit density matrix, we have proven that applying independent Uhrig DD (UDD) on each qubit will effectively eliminate both the qubit–environment and indirect qubit–qubit couplings to the same order as in the single-qubit case, only if orders of the two UDD sequences have different parities. More specifically, UDD( n ) on one qubit with UDD( m ) on another are able to produce min ( n , m )th-order suppression while n + m is odd. Our results can be used to reduce the pulse number in relevant experiments for protecting bipartite quantum states, or dynamically manipulating the indirect interaction within a certain quantum gate and quantum bus.
Maintaining quantum coherence is a crucial requirement for quantum computation; hence protecting quantum systems against their irreversible corruption due to environmental noise is an important open problem. Dynamical decoupling (DD) is an effective method for reducing decoherence with a low control overhead. It also plays an important role in quantum metrology, where, for instance, it is employed in multiparameter estimation. While a sequence of equidistant control pulses [the Carr-Purcell-Meiboom-Gill (CPMG) sequence] has been ubiquitously used for decoupling, Uhrig recently proposed that a nonequidistant pulse sequence [the Uhrig dynamic decoupling (UDD) sequence] may enhance DD performance, especially for systems where the spectral density of the environment has a sharp frequency cutoff. On the other hand, equidistant sequences outperform UDD for soft cutoffs. The relative advantage provided by UDD for intermediate regimes is not clear. In this paper, we analyze the relative DD performance in this regime experimentally, using solid-state nuclear magnetic resonance. Our system qubits are 13C^{13}\mathrm{C}13C nuclear spins and the environment consists of a 1H^{1}\mathrm{H}1H nuclear spin bath whose spectral density is close to a normal (Gaussian) distribution. We find that in the presence of such a bath, the CPMG sequence outperforms the UDD sequence. An analogy between dynamical decoupling and interference effects in optics provides an intuitive explanation as to why the CPMG sequence performs better than any nonequidistant DD sequence in the presence of this kind of environmental noise.
Dynamical decoupling (DD) sequences were invented to eliminate the direct coupling between a qubit and its environment. We further investigate the possibility of decoupling the indirect qubit–qubit interaction induced by a common environment, and successfully find simplified solutions that preserve the bipartite quantum states to arbitrary order. Through analysing the exact dynamics of the controlled two-qubit density matrix, we have proven that applying independent Uhrig DD (UDD) on each qubit will effectively eliminate both the qubit–environment and indirect qubit–qubit couplings to the same order as in the single-qubit case, only if orders of the two UDD sequences have different parities. More specifically, UDD(n) on one qubit with UDD(m) on another are able to produce min (n, m)th-order suppression while n + m is odd. Our results can be used to reduce the pulse number in relevant experiments for protecting bipartite quantum states, or dynamically manipulating the indirect interaction within a certain quantum gate and quantum bus.