We study the quantum phase transition in f-electron systems as a quantum Lifshitz transition driven by selective-Mott localization in a realistic extended Anderson lattice model. Using dynamical mean-field theory (DMFT), we find that a quantum critical phase with anomalous ω/T scaling separates a heavy Landau-Fermi liquid from ordered phase(s). This non-Fermi liquid state arises from a lattice orthogonality catastrophe originating from orbital-selective Mott localization. Fermi surface reconstruction occurs via the interplay between and penetration of the Green function zeros to the poles, leading to violation of Luttinger's theorem in the strange metal. We show how this naturally leads to scale-invariant responses in transport. Thus, our work represents a specific DMFT realization of the hidden-FL and FL* theories, and holds promise for the study of 'strange' metal phases in quantum matter.
We study the quantum phase transition in f-electron systems as a quantum Lifshitz transition driven by selective-Mott localization in a realistic extended Anderson lattice model. Using dynamical mean-field theory (DMFT), we find that a quantum critical phase with anomalous ω/T scaling separates a heavy Landau-Fermi liquid from ordered phase(s). This non-Fermi liquid state arises from a lattice orthogonality catastrophe originating from orbital-selective Mott localization. Fermi surface reconstruction occurs via the interplay between and penetration of the Green function zeros to the poles, leading to violation of Luttinger's theorem in the strange metal. We show how this naturally leads to scale-invariant responses in transport. Thus, our work represents a specific DMFT realization of the hidden-FL and FL* theories, and holds promise for the study of 'strange' metal phases in quantum matter.
We study the quantum phase transition in f -electron systems as a quantum Lifshitz transition driven by selective Mott localization in a realistic extended Anderson lattice model.Using DMFT, we find that a quantum critical phase with anomalous ω/T scaling separates a heavy Landau-Fermi liquid from ordered phase(s).Fermi surface reconstruction occurs via the interplay between, and penetration of the Green function zeros to the poles, leading to violation of Luttinger's theorem in the selective-Mott phase .We show how this naturally leads to scale-invariant responses in transport.Our work is represents a specific (DMFT) realization of the hidden-FL and FL * theories, and holds promise for study of "strange" metal phases in quantum matter.
We study paramagnetic quantum criticality in the periodic Anderson model (PAM) using cellular dynamical mean-field theory (CDMFT), with the numerical renormalization group (NRG) as a cluster impurity solver. The PAM describes itinerant c electrons hybridizing with a lattice of localized f electrons. At zero temperature, it exhibits a much-studied quantum phase transition from a Kondo phase to a Ruderman-Kittel-Kasuya-Yosida (RKKY) phase when the hybridization is decreased through a so-called Kondo breakdown quantum critical point (KB QCP). There, Kondo screening of f spins by c electrons breaks down, so that f excitations change their character from somewhat itinerant to mainly localized, while c excitations remain itinerant. Building on , which interpreted the KB transition as an orbital-selective Mott transition, we here elucidate its nature in great detail by performing a high-resolution, real-frequency study of various dynamical quantities (susceptibilities, self-energies, and spectral functions). NRG allows us to study the quantum critical regime governed by the QCP and located between two temperature scales, T FL < T NFL . In this regime, we find fingerprints of non-Fermi-liquid (NFL) behavior in several dynamical susceptibilities. Surprisingly, CDMFT self-consistency is essential to stabilize the QCP and the NFL regime. The Fermi-liquid (FL) scale T FL decreases toward and vanishes at the KB QCP; at temperatures below T FL , FL behavior emerges. At T = 0 , we find the following properties. The KB transition is continuous. The f quasiparticle weight decreases continuously as the transition is approached from either side, vanishing only at the KB QCP. Therefore, the quasiparticle weight of the f band is nonzero not only in the Kondo phase, but also in the RKKY phase; hence, the FL quasiparticles comprise c f electrons in both phases. The Fermi surface (FS) volumes in the two phases differ, implying a FS reconstruction at the KB QCP. Whereas the large-FS Kondo phase has a two-band structure as expected, the small-FS RKKY phase unexpectedly has a three-band structure. We provide a detailed analysis of quasiparticle properties of both the Kondo and, for the first time, also the RKKY phase and uncover their differences. The FS reconstruction is accompanied by the appearance of a Luttinger surface on which the f self-energy diverges. The volumes of the Luttinger and Fermi surfaces are related to the charge density by a generalized Luttinger sum rule. We interpret the small FS volume and the emergent Luttinger surface as evidence for f -electron fractionalization in the RKKY phase. Finally, we compute the temperature dependence of the Hall coefficient and the specific heat, finding good qualitative agreement with experiments. Published by the American Physical Society 2024
Recent experimental work has brought the twin issues of the origin of non-Lifshitz-Kosevich scaling in de Haas van Alphen (dHvA) and its precise relation to anomalously broad non-quasiparticle spectral features in "strange" metals, to the forefront. Here, we revisit these issues in the specific context of a "local" quantum critical phase in an extended periodic Anderson model (EPAM). In contrast to the famed Kondo-RKKY scenarios for local quantum criticality, strong local valence fluctuations cause Kondo destruction in the EPAM. We uncover a common underlying element, namely, the Kondo-destruction-driven infra-red continuum branch-cut behavior in the one-electron propagator, as the relevant feature that governs both non-Lifshitz-Kosevich scaling in dHvA and anomalously broad non-quasiparticle spectral responses in such a "strange" metal. Employing a non-perturbative scheme to treat effects of non-magnetic disorder in this version of a local strange metal, we propose a modified Dingle scaling that can also be used to test "local" criticality scenarios. Thus, our findings potentially afford an internally consistent description of novel fermiology expected to manifest in strange metals arising as a result of Kondo-destruction coming from an underlying orbital-selective Mott transition.
While a specific kind of strange metal is increasingly found to be the "normal" states in a wide variety of unconventional superconductors, its microscopic origin is presently a hotly debated enigma. Using dynamical mean-field theory (DMFT) based on hybridization expansion of continuous-time quantum Monte-Carlo (CTQMC) solver for an extended two-band Hubbard model (2BHM), we investigate the conditions underlying the emergence of such a metal. Specifically, we tie strange metallicity to an orbital-selective Mottness in 2BHM or momentum-selective Mott phase (OSMP) in 2D Hubbard models inspired by a cluster-to-orbital mapping. We find (i) disparate spin and charge responses, (ii) fractional power-law behavior and ω/T-scaling in the charge and spin fluctuation responses, and (iii) very good accord with optical conductivity and nuclear magnetic relaxation rates in the slightly underdoped normal states of cuprates and Fe-arsenides. We analyze the local problem using bosonization to show that such anomalous responses arise from a lattice orthogonality catastrophe specifically in the OSMP. Our work establishes the intimate link between strange metallicity and selective Mottness in quantum matter.
The quantum critical point (QCP) in YbRh2Si2 is an enigma for the itinerant view of QCP. In an alternative view, this QCP is intimately linked to the selective Mott localization of the heavy f electrons. Following a perusal of this unusual QCP, I study an Extended Periodic Anderson Model (EPAM) within DMFT. A quantum phase transition (FQPT), accompanied by a rapid change in the Fermi volume, is found near the quantum-critical end-point of the selective Mott transition in the f-electron sector. The theory accounts for a wide range of unusual, singular non-Fermi liquid features exhibited at this QCP in YbRh2Si2 in a natural way.
We investigate quantum phase transitions in the extended periodic Anderson model, which includes electron correlations within and between itinerant and localized bands. We calculate zero and finite temperature properties of the system using the combination of dynamical mean-field theory and the numerical renormalization group. At half filling, a first-order phase transition between a Mott insulating state and a Kondo insulating state occurs in the strong-coupling regime. We furthermore find that a metallic state is stabilized in the weak-coupling regime. This state should be adiabatically connected to the orbital selective Mott state with one orbital-localized and the other itinerant. The effect of hole doping is also addressed.