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arXiv:1010.4870

On-demand control of photon echoes far exceeding the spin coherence constraint via coherence swapping between optical and spin transitions

Byoung Seung HAM

Published Oct 23, 2010• 2 citations
arXivHTMLPDF

Abstract

Using on-demand coherence conversion via optical locking in conventional stimulated (three-pulse) photon echoes, ultralong, ultraefficient photon storage has been observed in a rare-earth Pr3+ doped Y2SiO5, where storage time is several orders of magnitude longer and retrieval efficiency is enhanced by fifty times. Compared with the same method applied to two-pulse photon echoes for a rephasing halt, use of spectral grating in the stimulated photon echoes offers a phase-independent coherence conversion between optical and spin states. Eventually an ultralong spin population decay-dependent photon storage protocol is achieved by applying optical locking to a spectral grating in conventional stimulated photon echoes. The present breakthrough in both photon storage time and retrieval efficiency opens a door to long-distance quantum communications utilizing quantum repeaters.

DOI
10.48550/arxiv.1010.4870

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Using on-demand coherence conversion via optical locking in conventional stimulated (three-pulse) photon echoes, ultralong, ultraefficient photon storage has been observed in a rare-earth Pr3+ doped Y2SiO5, where storage time is several orders of magnitude longer and retrieval efficiency is enhanced by fifty times. Compared with the same method applied to two-pulse photon echoes for a rephasing halt, use of spectral grating in the stimulated photon echoes offers a phase-independent coherence conversion between optical and spin states. Eventually an ultralong spin population decay-dependent photon storage protocol is achieved by applying optical locking to a spectral grating in conventional stimulated photon echoes. The present breakthrough in both photon storage time and retrieval efficiency opens a door to long-distance quantum communications utilizing quantum repeaters.
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Using on-demand coherence conversion via optical locking, a dynamic coherent control of the collective atom phase has been demonstrated for longer photon storage beyond the critical constraint of spin phase decay time, where the storage time can be extended up to hours in a rare-earth-doped solid. Coherent transient phenomena such as photon echoes have been investigated for frozen phase decay via coherent population transfer using a simple deshelving optical pulse pair. Unlike the rephasing halt applied to two-pulse photon echoes, where optical decoherence is accelerated by spin inhomogeneous broadening, a completely atom phase-locked coherence conversion has been observed in three-pulse photon echoes, resulting in spin dephasing-free coherence control. Here, the mechanism of the atom phase-locked coherence conversion via optical locking has been investigated in a solid medium whose optical transition is imperfect, where partial coherence is lost via optical depth-dependent imperfect population transfer. The relationship between coherence loss and optical depth is analyzed, where nearly perfect photon echo efficiency can be obtained for ultralong photon storage in an optically thick medium.
To overcome the fundamental limitations of the $\ensuremath{\pi}$ optical pulse-induced population inversion and optical decay-caused short storage time in conventional photon echoes, a coherent control of collective atoms is studied for inversion-free, optical decay-halted photon echoes, where the constraint of photon storage time is now replaced by a spin population decay process. Using phase-controlled double rephasing, an inversion-free photon echo scheme is obtained, where no spontaneous or stimulated emission-driven quantum noise exists. Thus, the present method can be applied for ultralong quantum memories in quantum repeaters for long-distance quantum communications.
For the last decade quantum memories have been intensively studied for potential applications to quantum information and communications using atomic and ionic ensembles. With the importance of a multimode storage capability in quantum memories, on-demand control of reversible inhomogeneous broadening of an optical medium has been broadly investigated recently. However, the photon storage time in these researches is still too short to apply for long-distance quantum communications. In this paper, we demonstrate new physics of spin population decay dependent ultralong photon storage method, where spin population decay time is several orders of magnitude longer than the conventional constraint of spin phase decay time.
Quantum storage of light in a collective ensemble of atoms plays an important role in quantum information processing. Consisting of a quantum repeater together with quantum entanglement swapping, quantum memory has been intensively studied recently. Conventional photon echoes have been limited by extremely low retrieval efficiency and short storage time confined by the optical phase decay process. Here, we report a storage time-extended near perfect photon echo protocol using a phase locking method via an auxiliary spin state, where the phase locking acts as a conditional stopper of the rephasing process resulting in extension of storage time determined by the spin dephasing process. We experimentally prove the proposed phase locked photon echo protocol in a Pr3+ doped Y2SiO5 in a quasi phase conjugate scheme, where the phase conjugate gives the important benefit of aberration corrections when dealing with quantum images.
A novel method of multi-bit quantum optical data storage is presented, where the storage time can be lengthened far beyond the spin phase-decay time in a reversible spin inhomogeneous system excited by consecutive resonant Raman optical data pulses. The ultralong storage time is obtained by an optical population locking mechanism of modified rephasing process. This gives potentials to quantum repeaters utilizing quantum memories for long distance quantum communications, in which ultralong storage time plays a major role.