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arXiv:1009.1888 · Physical Review B

Stability of quantum critical points in the presence of competing orders

Jian-Huang She, Jan Zaanen, A. R. Bishop, Alexander V. Balatsky

Published Oct 28, 2010• 47 citations
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Abstract

We investigate the stability of quantum critical points (QCPs) in the presence of two competing phases. These phases near QCPs are assumed to be either classical or quantum and assumed to repulsively interact via square-square interactions. We find that for any dynamical exponents and for any dimensionality strong enough interaction renders QCPs unstable and drives transitions to become first order. We propose that this instability and the onset of first-order transitions lead to spatially inhomogeneous states in practical materials near putative QCPs. Our analysis also leads us to suggest that there is a breakdown of conformal field theory scaling in the Anti de Sitter models, and in fact these models contain first-order transitions in the strong-coupling limit.

DOI
10.1103/physrevb.82.165128

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We investigate the stability of quantum critical points (QCPs) in the presence of two competing phases. These phases near QCPs are assumed to be either classical or quantum and assumed to repulsively interact via square-square interactions. We find that for any dynamical exponents and for any dimensionality strong enough interaction renders QCPs unstable and drives transitions to become first order. We propose that this instability and the onset of first-order transitions lead to spatially inhomogeneous states in practical materials near putative QCPs. Our analysis also leads us to suggest that there is a breakdown of conformal field theory scaling in the Anti de Sitter models, and in fact these models contain first-order transitions in the strong-coupling limit.
Deconfined quantum critical points (DQCPs) are putative phase transitions beyond the Landau paradigm with emergent fractionalized degrees of freedom. The original example of a DQCP is the spin-12\frac{1}{2}21​ quantum antiferromagnet on the square lattice which features a second-order transition between valence bond solid (VBS) and N\'eel order. The VBS order breaks a lattice symmetry, and the corresponding VBS order parameter may couple to lattice distortion modes (phonons) at appropriate momenta. We investigate a field-theoretic description of the DQCP in the presence of such a spin-lattice coupling. We show that treating phonons as classical lattice distortions leads to a relevant monopole-phonon interaction inducing an instability towards a distorted lattice by an analogous mechanism to the spin-Peierls instability in one dimension. Consequently, there is a breakdown of the DQCP which generally becomes a strong first-order transition. Taking into account the full quantum nature of the phonons, we argue that the continuous DQCP persists above a critical phonon frequency. Lastly, we comment on the connection to general gapless, deconfined gauge theories.
We study phase diagrams of a class of doped quantum dimer models on the square lattice with ground-state wave functions whose amplitudes have the form of the Gibbs weights of a classical doped dimer model. In this dimer model, parallel neighboring dimers have attractive interactions, whereas neighboring holes either do not interact or have a repulsive interaction. We investigate the behavior of this system via analytic methods and by Monte Carlo simulations. At zero doping, we confirm the existence of a Kosterlitz-Thouless transition from a quantum critical phase to a columnar phase. At low hole densities, we find a dimer-hole liquid phase and a columnar phase, separated by a phase boundary which is a line of critical points with varying exponents. We demonstrate that this line ends at a multicritical point where the transition becomes first order and the system phase separates. The first-order transition coexistence curve is shown to become unstable with respect to more complex inhomogeneous phases in the presence of direct hole-hole interactions. We also use a variational approach to determine the spectrum of low-lying density fluctuations in the dimer-hole fluid phase.
We explore the dynamical behavior at and near a special class of two-dimensional quantum critical points. Each is a conformal quantum critical point (CQCP), where in the scaling limit the equal-time correlators are those of a two-dimensional conformal field theory. The critical theories include the square-lattice quantum dimer model, the quantum Lifshitz theory, and a deformed toric code model. We show that under generic perturbation the latter flows toward the ordinary Lorentz-invariant (2+12+12+1)-dimensional Ising critical point, illustrating that CQCPs are generically unstable. We exploit a correspondence between the classical and quantum-dynamical behavior in such systems to perform an extensive numerical study of two lines of CQCPs in a quantum eight-vertex model or, equivalently, two coupled deformed toric codes. We find that the dynamical critical exponent zzz remains 2 along the U(1)-symmetric quantum Lifshitz line, while it continuously varies along the line with only Z2{\mathbb{Z}}_{2}Z2​ symmetry. This illustrates how two CQCPs can have very different dynamical properties, despite identical equal-time ground-state correlators. Our results equally apply to the dynamics of the corresponding purely classical models.
We resolve the nature of the quantum phase transition between antiferromagnetic and valence-bond solid ground states in square-lattice spin-1/2 magnets - the putative deconfined quantum-critical point. Using quantum Monte Carlo simulations of J-Q models, in which Heisenberg exchange J competes with multi-spin interactions Qn formed by n singlet projectors, we demonstrate first-order discontinuities increasing with n. For n=2 and n=3, the first-order signatures are very weak and we extract universal scaling dimensions of a proximate multicritical point. Their values coincide closely with known bounds for an SO(5) symmetric conformal field theory (CFT) containing a relevant SO(5) singlet operator that destabilizes the generic deconfined critical point. We characterize the emergent SO(5) symmetry by its scaling dimensions of the leading irrelevant perturbations. Using the J-Q2-Q6 model, we tune the transition from weak to stronger first-order and find scaling of the coexisting order parameters with a large exponent beta ~ 0.85, in agreement with the relevant scaling dimensions of the multicritical point. The exponent that had previously been identified with the correlation length does not have a corresponding CFT level, and we explain it as pseudo-critical length scale of bubbles of one phase inside the other that are compressed in size by an SO(5)-violating irrelevant repulsive interaction between the two order parameters. The bubble scale reflects a hierarchy of excitation gaps generated by the SO(5) perturbation in the neighborhood of the first-order transition, akin to a Higgs mechanism. We argue that the multicritical point is the tip of a gapless spin liquid phase in frustrated Heisenberg models into which the J-Q models can be deformed, but the spin liquid, and perhaps the multicritical point itself, exist outside the regime amenable to sign-free simulations.
Abstract The study of the competition or coexistence of different ground states in many-body systems is an exciting and actual topic of research, both experimentally and theoretically. Quantum fluctuations of a given phase can suppress or enhance another phase depending on the nature of the coupling between the order parameters, their dynamics and the dimensionality of the system. The zero temperature phase diagrams of systems with competing scalar order parameters with quartic and bilinear coupling terms have been previously studied for the cases of a zero temperature bicritical point and of coexisting orders. In this work, we apply the Matsubara summation technique from finite temperature quantum field theory to introduce the effects of thermal fluctuations on the effective potential of these systems. This is essential to make contact with experiments. We consider two and three-dimensional materials characterized by a Lorentz invariant quantum critical theory, i.e., with dynamic critical exponent z = 1, such that time and space scale in the same way. We obtain that in both cases, thermal fluctuations lead to weak first-order temperature phase transitions, at which coexisting phases arising from quantum corrections become unstable. We show that above this critical temperature ( T c ), the system presents scaling behavior consistent with that approaching a quantum critical point. Below the transition the specific heat has a thermally activated contribution with a gap related to the size of the domains of the ordered phases. We obtain that T c decreases as a function of the distance to the zero temperature classical bicritical point (ZTCBP) in the coexistence region, implying that in our approach, the system attains the highest T c above the fine tuned value of this ZTCBP.
Deconfined quantum critical points (DQCPs) describe continuous transitions between ordered phases beyond the Landau paradigm. A simple example is the Néel antiferromagnet (AFM) to valence bond solid (VBS) transition in a 1D antiferromagnetic J1−J2J_1-J_2J1​−J2​ model. In analogy to the spin-Peierls instability of critical spin chains, DQCPs are predicted to be unstable towards lattice distortions below a critical phonon frequency. In this work, we use tensor network simulations to investigate this instability in the antiferromagnetic J1−J2J_1-J_2J1​−J2​ model coupled to lattice vibrations. We confirm the stability of DQCP for large phonon frequencies and demonstrate that the transition turns strongly first-order below a critical frequency. The instability is caused by a reduction of the Luttinger parameter due to spin-phonon interactions and we identify the effective theory of the behavior as the double sine-Gordon model. The same effective theory is known to describe the classical Ashkin-Teller model, which enables us to show that the critical endpoint is in the four-state Potts universality class. We argue based on non-linear bosonization that the sign of the double-frequency term is fixed, which provides a microscopic justification for the first-order transition. Furthermore, we provide quantitative numerical scaling results for the phonon spectral function, offering an experimental signature to probe DQCP-phonon coupling in low-dimensional materials.