The physics of quantum dots is depicted succinctly by the universal Hamiltonian, where only zero-mode interactions are included. In the case in which the latter involve charging and isotropic spin-exchange terms, this would lead to a non-Abelian action. Here we address an Ising spin-exchange interaction, which leads to an Abelian action. The analysis of this simplified yet nontrivial model shed light on a more general case of charge and spin entanglement. We present a calculation of the tunneling density of states and dynamic magnetic susceptibility. We explain how the latter can be used for an experimental determination of the exchange interaction strength.
The physics of quantum dots is depicted succinctly by the universal Hamiltonian, where only zero-mode interactions are included. In the case in which the latter involve charging and isotropic spin-exchange terms, this would lead to a non-Abelian action. Here we address an Ising spin-exchange interaction, which leads to an Abelian action. The analysis of this simplified yet nontrivial model shed light on a more general case of charge and spin entanglement. We present a calculation of the tunneling density of states and dynamic magnetic susceptibility. We explain how the latter can be used for an experimental determination of the exchange interaction strength.
In the last years, the electron spin in quantum dots has become a most promising candidate for the realization of qubits, the basic element for quantum computation. In quantum dot spin qubits the exchange interaction implements a fundamental two qubit gate, which originates in the Coulomb interaction and the Pauli principle. Compared to single qubit gates, the exchange based gates are much faster and easier to control locally, motivating the solely exchange energy based quantum computation. The control is based on the exponential sensitivity of the exchange energy on the interparticle distance. Manipulation then can proceed, for example, shifting the single particle states electrically or compressing them magnetically. The practical manipulation schemes require quantitative knowledge of the exchange energy. The spin-orbit interaction plays an important role in this nano-system. Indeed the usual exchange interaction changes its magnitude, while a new term, called anisotropic exchange, appears. In this thesis we propose an accurate effective spin Hamiltonian for modeling spin-orbit-induced spin dynamics in the presence of the magnetic field. We have also performed numerically exact calculations of the isotropic and anisotropic exchange coupling in realistic two-electron GaAs coupled quantum dots in the presence of both Dresselhaus and Bychkov-Rashba spin-orbit interactions. The numerics allow us to establish the goodness of our model and to see the limits of previous statements. Furthermore we find that in zero magnetic field the second-order spin-orbit effects are absent at all interdot couplings.
Solid state based quantum information processing is focused on physical implementation of all necessary elements of quantum computation and quantum information in solid state systems, mainly due to their scalability compared to e.g. optical systems. Among many proposals to realize these types of devices, such as quantum dots as charge qubits or Josephson junction circuits, we study here one of the most promising candidates, i.e., the spin of an electron confined to a quantum dot as a qubit. Experimentally, it has been shown that the relaxation rate of this two level system can be pushed above few seconds in low magnetic fields. Moreover, using spin echo techniques, \nthe spin dephasing time can be maximized up to milliseconds with the current technology. This long spin decay time is one of the main reasons that make this system desirable for quantum computation and quantum information purposes. \nWe reexamined the recent measurement based proposal called one-way quantum computation which exploits entanglement and local measurements as tools to perform quantum computation on N qubits. Although it was suggested in the original work to entangle the qubits via the nearest neighbor Ising interaction, we investigated how one can generate the so-called cluster states with the Heisenberg interaction. We extended our method to include more general forms of Heisenberg interaction such as asymmetric coupling of adjacent qubits. These forms of couplings, rather than Ising interaction, are more encountered in solid state devices, and therefore make it possible to perform one-way quantum computation with electron spins in quantum dots coupled via exchange interaction to their adjacent spins. \n \nChapters II, III, and IV of my thesis are devoted to the study of the spin-orbit interaction in heterostructure quantum dots and its effect on the spin dynamics. We observed that one can actually use spin-orbit interaction to manipulate the spin state of an electron on time scales much smaller than the spin dephasing time. Specifically, in chapter II, we studied the effect of a nearby functioning quantum point contact (QPC) on the relaxation of the electron spin and show that the charge fluctuations in QPC lead to spin relaxation of the confined electron in the presence of spin-orbit interactiom and an applied magnetic field. We also addressed the relation of this rate to the microscopic parameters of the system and found some geometrical dependence of the spin relaxation time on the orientation of the QPC on the substrate. Moreover, we showed in chapters III and IV that the spin-orbit interaction can play a positive role, in order to rotate the spin around the Bloch sphere. We considered different mechanisms, particularly, Electron Dipole Spin Resonance (EDSR) and holonomic unitary gates in quantum dots. We verified that these mechanisms of spin manipulation can be realized in solid state systems with the state of the art semiconductor technologies. \n \nChapter V of the thesis covers a slightly different topic and focuses on the role of the Coulomb interaction in electronic transport. There, we reviewed the non-analytic corrections to the Fermi liquid behavior and their consequences on the momentum occupation number of the electrons in a two dimensional electron gas (2DEG). As an example, we calculated the tunneling rate from an interacting electron reservoir onto a quantum dot and compared our result to the corresponding case for electron tunneling between bilayer 2DEGs. Moreover, within RPA approximation, we found that the electron-plasmon coupling leads to a quadratic frequency dependence of the electron self-energy at low frequencies at the Fermi surface. This correction suppresses the same order corrections due to the particle-hole bubble. \n \n \n
Abstract This study investigates the entanglement properties of quantum dots (QDs) under a universal Hamiltonian where the Coulomb interaction between particles (electrons or holes) decouples into charging energy and exchange coupling terms. Although this formalism typically decouples the charge and spin components, confinement‐induced energy splitting can induce unexpected entanglement within the system. By analyzing the dynamic susceptibility and quantum Fisher information (QFI), significant behaviors are uncovered influenced by exchange constants, temperature variations, and confinement effects. In QDs with Ising exchange interactions, far below the Stoner instability (SI) point, where the QD is in a disordered paramagnetic phase, temperature reductions lead to decreased entanglement, challenging conventional expectations. These findings demonstrate that for QDs with small exchange interactions, the responses of easy‐plane () and easy‐axis () configurations are similar, with increased anisotropy broadening susceptibility and shifting its maximum to higher frequencies. For large exchange interactions, the susceptibility differences between easy‐plane and easy‐axis QDs become significant, with easy‐plane QDs exhibiting a higher susceptibility magnitude. Additionally, the study reveals that temperature variations affect the dynamic response functions differently in easy‐axis and easy‐plane QDs. In easy‐plane QDs, QFI consistently decreases with increasing temperature, whereas in easy‐axis QDs, QFI behavior is highly dependent on the strengths of and , showing either an increase or decrease with temperature based on specific coupling conditions. Conversely, at low temperatures, anisotropic Heisenberg models exhibit enhanced entanglement near isotropic points. Overall, this work contributes to advancing the understanding of entanglement in QDs and its potential applications in quantum technologies.
Semiconductor quantum dot systems offer a promising platform for quantum computation. And these quantum computation candidates are normally based on spin or charge properties of electrons. In these systems, we focus on quantum computation based on electron spins since these systems has good scalability, long coherence times, and rapid gate operations. And this thesis focuses on building a theoretical description of quantum dot systems and the link between theory and experiments. In many quantum dot systems, exchange interactions are the primary mechanism used to control spins and generate entanglement. And exchange energies are normally positive, which limits control flexibility. However, recent experiments show that negative exchange interactions can arise in a linear three-dot system when a two-electron double quantum dot is exchange coupled to a larger quantum dot containing on the order of one hundred electrons. The origin of this negative exchange can be traced to the larger quantum dot exhibiting a spin triplet-like rather than singlet-like ground state. Here we show using a microscopic model based on the configuration interaction (CI) method that both triplet-like and singlet-like ground states are realized depending on the number of electrons. In the case of only four electrons, a full CI calculation reveals that triplet-like ground states occur for sufficiently large dots. These results hold for symmetric and asymmetric quantum dots in both Si and GaAs, showing that negative exchange interactions are robust in few-electron double quantum dots and do not require large numbers of electrons. Recent experiments also show the potential to utilize large quantum dots to mediate superexchange interaction and generate entanglement between distant spins. This opens up a possible mechanism for selectively coupling pairs of remote spins in a larger network of quantum dots. Taking advantage of this opportunity requires a deeper understanding of how to control superexchange interactions in these systems. Here, we consider a triple-dot system arranged in linear and triangular geometries. We use CI calculations to investigate the interplay of superexchange and nearest-neighbor exchange interactions as the location, detuning, and electron number of the mediating dot are varied. We show that superexchange processes strongly enhance and increase the range of the net spin-spin exchange as the dots approach a linear configuration. Furthermore, we show that the strength of the exchange interaction depends sensitively on the number of electrons in the mediator. Our results can be used as a guide to assist further experimental efforts towards scaling up to larger, two-dimensional quantum dot arrays.
We consider a quantum-gate mechanism based on electron spins in coupled semiconductor quantum dots. Such gates provide a general source of spin entanglement and can be used for quantum computers. We determine the exchange coupling J in the effective Heisenberg model as a function of magnetic (B) and electric fields, and of the interdot distance a within the Heitler-London approximation of molecular physics. This result is refined by using sp hybridization, and by the Hund-Mulliken molecular-orbit approach, which leads to an extended Hubbard description for the two-dot system that shows a remarkable dependence on B and a due to the long-range Coulomb interaction. We find that the exchange J changes sign at a finite field (leading to a pronounced jump in the magnetization) and then decays exponentially. The magnetization and the spin susceptibilities of the coupled dots are calculated. We show that the dephasing due to nuclear spins in GaAs can be strongly suppressed by dynamical nuclear-spin polarization and/or by magnetic fields.
The time evolution of spin states of two electrons interacting with a nuclear spin bath in a quantum dot system is studied. The hyperfine interaction between the electrons and the nuclear spins is modeled by an isotropic Heisenberg interaction, and the interaction between the electron spins by Heisenberg exchange. Depending on the extent of the overlap between the spatial wave functions of the electrons, there are two physically different cases, namely, the two qubits either interact with the same set of nuclear spins or they see different nuclear spin environments. In the two cases, the decoherence of the two-qubit state is studied analytically. We have identified a class of two-qubit states that have a rich dynamics when the exchange interaction between the qubits becomes large in comparison to the hyperfine interaction strengths. The decoherence time scale is determined as a function of the bath-spin distribution and the polarizations of the initial two-qubit state. States with large decoherence times are identified by performing a minimization over all the two-qubit pure states.