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arXiv:1007.1152 · Physical Review Letters

Energy Relaxation and Thermalization of Hot Electrons in Quantum Wires

Torsten Karzig, L. I. Glazman, Felix von Oppen

Published Nov 24, 2010• 58 citations
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Abstract

We develop a theory of energy relaxation and thermalization of hot carriers in clean quantum wires. Our theory is based on a controlled perturbative approach for large excitation energies and emphasizes the important roles of the electron spin and finite temperature. Unlike in higher dimensions, relaxation in one-dimensional electron liquids requires three-body collisions and is much faster for particles than holes which relax at nonzero temperatures only. Moreover, comoving carriers thermalize more rapidly than counterpropagating carriers. Our results are quantitatively consistent with a recent experiment.

DOI
10.1103/physrevlett.105.226407

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We develop a theory of energy relaxation and thermalization of hot carriers in clean quantum wires. Our theory is based on a controlled perturbative approach for large excitation energies and emphasizes the important roles of the electron spin and finite temperature. Unlike in higher dimensions, relaxation in one-dimensional electron liquids requires three-body collisions and is much faster for particles than holes which relax at nonzero temperatures only. Moreover, comoving carriers thermalize more rapidly than counterpropagating carriers. Our results are quantitatively consistent with a recent experiment.
We study the problem of energy relaxation in a one-dimensional electron system. The leading thermalization mechanism is due to three-particle collisions. We show that for the case of spinless electrons in a single channel quantum wire the corresponding collision integral can be transformed into an exactly solvable problem. The latter is known as the Schrodinger equation for a quantum particle moving in a Poschl-Teller potential. The spectrum for the resulting eigenvalue problem allows for bound-state solutions, which can be identified with the zero modes of the collision integral, and a continuum of propagating modes, which are separated by a gap from the bound states. The inverse gap gives the time scale at which counterpropagating electrons thermalize.
We study the problem of energy relaxation in a one-dimensional electron system. The leading thermalization mechanism is due to three-particle collisions. We show that for the case of spinless electrons in a single channel quantum wire the corresponding collision integral can be transformed into an exactly solvable problem. The latter is known as the Schrödinger equation for a quantum particle moving in a Pöschl-Teller potential. The spectrum for the resulting eigenvalue problem allows for bound-state solutions, which can be identified with the zero modes of the collision integral, and a continuum of propagating modes, which are separated by a gap from the bound states. The inverse gap gives the time scale at which counterpropagating electrons thermalize.
We consider the problem of relaxation in a one-dimensional system of interacting electrons. In the limit of weak interactions, we calculate the decay rate of a single-electron excitation, accounting for the nonlinear dispersion. The leading processes that determine the relaxation involve scattering of three particles. We elucidate how particular forms of Coulomb interaction, unscreened and screened, lead to different results for the decay rates and identify the dominant scattering processes responsible for relaxation of excitations of different energies. Interestingly, temperatures much smaller than the excitation energy strongly affect the rate. At higher temperatures the quasiparticle relaxes by exciting copropagating electron-hole pairs, whereas at lowest temperatures the relaxation proceeds via excitations of both copropagating and counterpropagating pairs.
Luttinger liquid theory describes one-dimensional electron systems in terms of noninteracting bosonic excitations. In this approximation thermal excitations are decoupled from the current flowing through a quantum wire, and the conductance is quantized. We show that relaxation processes not captured by the Luttinger liquid theory lead to equilibration of the excitations with the current and give rise to a temperature-dependent correction to the conductance. In long wires, the magnitude of the correction is expressed in terms of the velocities of bosonic excitations. In shorter wires it is controlled by the relaxation rate.
This dissertation investigates the non-equilibrium relaxation and thermalization of conduction electrons coupled to bosonic excitations, focusing on whether magnons can provide a relaxation channel analogous to phonons. Using perturbative analysis, exact diagonalization, and semiclassical simulations, we study one-dimensional systems described primarily by the Kondo lattice model. For a single conduction electron in a ferromagnetic background, the weak-coupling dynamics can be understood as the interaction of two electronic levels with a bosonic bath. We then increase the number of available many-body scattering channels by increasing the carrier density or by considering an antiferromagnetic spin background. In both cases, the long-time behavior of local observables becomes consistent with thermalization. These results show how localized spin excitations can mediate electronic relaxation.
Recent advances of experimental nanofabrication techniques draw increasing attention to the non-equilibrium behavior of low dimensional systems. Of particular interest are the strongly interacting one dimensional systems whose description in out of equilibrium situations remains a theoretical challenge. This thesis contributes to the understanding of important elementary processes in the non-equilibrium physics of one dimensional electron systems. Tunneling of an electron into a Luttinger liquid leads to partitioning of its charge and energy into counter-propagating modes. This thesis studies the partitioning of the energy which had previously remained unexplored. It turns out that energy partitioning is essentially independent of the charge partitioning and one can even reach conditions such that energy and charge propagate in opposite directions. Another important difference is their experimental accessibility. In contrast to the charge, energy partitioning provides a measurable characteristic of the tunneling process even in dc setups and we propose experimental geometries that allow for tuning and detecting energy partitioning. At higher excitation energies it becomes necessary to include curvature effects of the electron dispersion. Another part of this thesis discusses the consequences of curvature induced three-body collisions on the relaxation in quantum wires. This is particularly interesting due to the integrability of the Luttinger model which does not allow for thermalization within this paradigm of one dimensional systems. In this thesis we derive energy relaxation rates due to three-body processes beyond the Luttinger model within a well-defined perturbative approach. It turns out that the electron spin and the long range Coulomb interaction are important ingredients for a quantitative description of recent experiments which we provide in this thesis. Furthermore, we study the influence of three-body collisions on the energy relaxation in integer quantum Hall edge states. We specifically address different interaction induced edge reconstruction scenarios and find that edge reconstruction strongly enhances the energy relaxation. This is particularly pronounced when the reconstruction creates additional counter-propagating modes. Finally, we discuss another system which is crucially controlled by non-equilibrium effects. The so called nanoelectromechanical systems show a coupling between the electronic and mechanical degrees of freedom. The electron current can thus influence the mechanical motion which leads to a number of interesting applications. Previous theoretical studies on the basis of non-equilibrium Green's functions showed that these current induced forces can be expressed in terms of intuitive scattering matrix expressions. This thesis sheds considerable light on this observation by providing a much more satisfactory and concise derivation of the scattering theory of current induced forces.