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arXiv:1006.5615 · Physical Review B

Ultrafast sequential charge transfer in a double quantum dot

A. Putaja, E. Räsänen

Published Oct 29, 2010• 20 citations
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Abstract

We use optimal control theory to construct external electric fields that coherently transfer the electronic charge in a double quantum-dot system. Without truncation of the eigenstates we operate on desired superpositions of the states in order to prepare the system to a localized state and to coherently transfer the charge from one well to another. Within a fixed time interval, the optimal processes are shown to occur through several excited states. The obtained yields are generally between 99% and 99.99% depending on the field constraints, and they are not dramatically affected by strict frequency filters which make the fields (e.g., laser pulses) closer to experimental realism. Finally we demonstrate that our scheme provides simple access to hundreds of sequential processes in charge localization while preserving the high fidelity.

DOI
10.1103/physrevb.82.165336

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We use optimal control theory to construct external electric fields that coherently transfer the electronic charge in a double quantum-dot system. Without truncation of the eigenstates we operate on desired superpositions of the states in order to prepare the system to a localized state and to coherently transfer the charge from one well to another. Within a fixed time interval, the optimal processes are shown to occur through several excited states. The obtained yields are generally between 99% and 99.99% depending on the field constraints, and they are not dramatically affected by strict frequency filters which make the fields (e.g., laser pulses) closer to experimental realism. Finally we demonstrate that our scheme provides simple access to hundreds of sequential processes in charge localization while preserving the high fidelity.
We propose an efficient control protocol for charge transfer in a double quantum dot. We consider numerically a two-dimensional model system, where the quantum dots are subjected to time-dependent electric fields corresponding to experimental gate voltages. Our protocol enables navigation in the charge stability diagram from a state to another through controllable variation of the fields. We show that the well-known adiabatic Landau-Zener transition-when supplemented with a time-dependent field tailored with optimal control theory-can remarkably improve the transition speed. The results also lead to a simple control scheme obtained from the experimental charge stability diagram that requires only a single parameter. Eventually, we can achieve the ultrafast performance of the composite pulse protocol that allows the system to be driven at the quantum speed limit.
We apply quantum optimal control theory to establish a local voltage-control scheme that operates in conjunction with the numerically exact solution of the time-dependent Schr\"odinger equation. The scheme is demonstrated for high-fidelity coherent control of electronic charge in semiconductor double quantum dots. We find tailored gate voltages in the viable gigahertz regime that drive the system to a desired charge configuration with >99>99%>99 yield. The results could be immediately verified in experiments and would play an important role in applications towards solid-state quantum computing.
Abstract Semiconductor quantum dots are ideal candidates for quantum information applications in solid-state technology. However, advanced theoretical and experimental tools are required to coherently control, for example, the electronic charge in these systems. Here we demonstrate how quantum optimal control theory provides a powerful way to manipulate the electronic structure of coupled quantum dots with an extremely high fidelity. As alternative control fields we apply both laser pulses as well as electric gates, respectively. We focus on double and triple quantum dots containing a single electron or two electrons interacting via Coulomb repulsion. In the two-electron situation we also briefly demonstrate the challenges of timedependent density-functional theory within the adiabatic local-density approximation to produce comparable results with the numerically exact approach.
Coherent single-electron control in a realistic semiconductor double quantum dot is studied theoretically. Using optimal-control theory, we show that the energy spectrum of a two-dimensional double quantum dot has a fully controllable transition line. We find that optimized picosecond laser pulses generate population transfer at significantly higher fidelities (>0.99)(>0.99)(>0.99) than conventional sinusoidal pulses. Finally, we design a robust and fast charge switch driven by optimal pulses that are within reach of terahertz laser technology.
For a two-level double quantum-dot (DQD) system, we proposed an alternative ultrafast manipulation approach, Lyapunov-based control method, to transfer the charge qubit from the initial charge state |R) to the target charge state |L) on the picosecond scale. Better control performance is obtained compared with that via Landau-Zener-Stu̅ckberge-Majorana interference, and the designed control fields can be implemented in the actual experiment facility. The control process is composed of three parts: first, a slope pulse takes the system from a positive detuning adiabatically to the anticrossing point, which corresponds to the resonance state of the system; then, a Lyapunov-based control pulse drives the charge qubit transfer nonadiabatically; finally, another slope pulse takes the system away from the anticrossing point to keep the system stable. The charge qubit transfer performance and the function of Lyapunov-based control pulse were studied under different control parameters. Simulation results showed that the designed Lyapunov-based control pulse has a rise time ~20 ps, which is in the scope of the Tektronix AWG70000A series arbitrary waveform generator and results in a significant probability ~96% for the transition from the initial charge state |R) to the target charge state |L). The fidelity of the control process designed can achieve ~94%. This is the first result directly applicable for a DQD charge qubit transfer using the Lyapunov-based control method.
We present theory and calculations for coherent high-fidelity quantum control of many-particle states in semiconductor quantum wells. We show that coupling a two-electron double quantum dot to a terahertz optical source enables targeted excitations that are one to two orders of magnitude faster and significantly more accurate than those obtained with electric gates. The optical fields subject to physical constraints are obtained through quantum optimal control theory that we apply in conjunction with the numerically exact solution of the time-dependent Schr\"odinger equation. Our ability to coherently control arbitrary two-electron states, and to maximize the entanglement, opens up further perspectives in solid-state quantum information.