Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

arXiv:1005.3141 · Physical Review Letters

BCS Wave-Function Approach to the BEC-BCS Crossover of Exciton-Polariton Condensates

Tim Byrnes, Tomoyuki Horikiri, Natsuko Ishida, Y. Yamamoto

Published Oct 26, 2010• 71 citations
arXivHTMLPDF

Abstract

The crossover between low and high density regimes of exciton-polariton condensates is examined using a BCS wave-function approach. Our approach is an extension of the BEC-BCS crossover theory for excitons, but includes a cavity photon field. The approach can describe both the low density limit, where the system can be described as a Bose-Einstein condensate (BEC) of exciton-polaritons, and the high density limit, where the system enters a photon-dominated regime. In contrast to the exciton BEC-BCS crossover where the system approaches an electron-hole plasma, the polariton high density limit has strongly correlated electron-hole pairs. At intermediate densities, there is a regime with BCS-like properties, with a peak at nonzero momentum of the singlet pair function. We calculate the expected photoluminescence and give several experimental signatures of the crossover.

DOI
10.1103/physrevlett.105.186402

Related papers

BETWEEN QUANTUM CORRELATIONS AND PHASE TRANSITIONS IN AN EXCITON-POLARITON BEC CONFINED IN A NANOCAVITY

Guillermo A. Guirales, Boris A. Rodríguez, Herbert Vinck Posada

Recently, the two-dimensional nanocavity exciton-polariton system confined in semiconductor nanocavities has emerged as a promising alternative of BoseEinstein Condensate (BEC). The strong quantum correlations presents in this system, make it an unique candidate for studying entanglement and quantum phase transitions —qualitative changes in the ground state properties—. In this work, we review previous evidence, obtained by us, in the phase transitions of a finite exciton-polariton system. First, by using a BCS wave function to compute the ground state energy of N excitons without the photonic field, a crossover from the high-density electron-hole phase to the BCS excitonic phase is found, at a density which is roughly four times the close-packing density of excitons. Second, by means of a self-consistent procedure with a trial function composed of a coherent photon field and a BCS function for the electron-hole pairs, we obtain the scaling of the critical temperature with the number of polaritons. Using the method proposed originally by Olliver and Zurek, and subsequently developed by Bo Li and Zhi-Xi Wang , we calculate the discord for a generalized density operator, proposed by Blaizot

•Jan 1, 2013•0 citations

Phase diagram of microcavity exciton-polariton condensates

Dinh-Hoi Bui, Van-Nham Phan

In this work, we study the exciton-polariton condensate phase transition in a microcavity matter-light system in which electron-hole Coulomb interaction and matter-light coupling effects are treated on an equal footing. In the framework of the unrestricted Hartree-Fock approximation applying the two-dimensional exciton-polariton model, we derive the self-consistent equations determining simultaneously the excitonic and the photonic condenstate order parameters. In the thermal-equilibrium limit, we find a condensed state of the exciton-polariton systems and phase diagrams are then constructed. At a given low temperature, the condensate by its nature shows a crossover from an excitonic to a polaritonic and finally photonic condensed state as the excitation density increases at large detuning. Without the detuning, the excitonic condensed state disappears whereas the polaritonic or photonic phases dominate. The crossover is also found by lowering the Coulomb interaction at a finite matter-light coupling. Lowering the Coulomb interaction or increasing the temperature, the excitonic Mott transition occurs, at which the exciton-polariton condensates dissociate to free electron-hole/photon. Depending on temperature and excitation density, the phase transition of the exciton-polariton condensates is also addressed in signatures of photoluminescence mapping to the photonic momentum distribution.

arXiv:1702.03659•Europhysics Letters (EPL)•Dec 1, 2016•4 citations

Excitonic BCS-BEC crossover at finite temperature: Effects of repulsion and electron-hole mass difference

Yuh Tomio, Kotaro Honda, Tetsuo Ogawa

The BCS to Bose-Einstein condensation (BEC) crossover of electron-hole $(e\text{\ensuremath{-}}h)$ pairs in optically excited semiconductors is studied using the two-band Hubbard model with both repulsive and attractive interactions. Applying the self-consistent $t$-matrix approximation combined with a local approximation, we examine the properties of a normal phase and an excitonic instability. The transition temperature from the normal phase to an $e\text{\ensuremath{-}}h$ pair condensed one is studied to clarify the crossover from an $e\text{\ensuremath{-}}h$ BCS-like state to an excitonic Bose-Einstein condensation, which takes place on increasing the $e\text{\ensuremath{-}}h$ attraction strength. To investigate effects of the repulsive interaction and the $e\text{\ensuremath{-}}h$ mass difference, we calculate the transition temperature for various parameters of the interaction strengths, the $e\text{\ensuremath{-}}h$ particle density, and the mass difference. While the transition temperature in the $e\text{\ensuremath{-}}h$ BCS regime is sufficiently suppressed by the repulsive interaction, that of the excitonic BEC is largely insensitive to it. We also show quantitatively that in the whole regime the mass difference leads to large suppression of the transition temperature.

arXiv:cond-mat/0606100•Physical Review B•Jun 12, 2006•28 citations

A BCS-BEC crossover in the extended Falicov-Kimball model: Variational cluster approach

Kazuhiro Seki, Tatsuya Kaneko, S Yamaki +2 more

Motivated by recent experimental and theoretical studies of excitonic insulators, we use the variational cluster approximation to calculate the single-particle Green's function and anomalous Green's function of the Falicov-Kimball model extended by including a finite valence bandwidth. We thus determine the single-particle excitation gap due to the bound-state formation of an electron and a hole. We also evaluate the order parameter of the excitonic insulating state indicating quantum coherence of condensed excitons. We thereby discuss the excitonic insulator that typifies either a BCS condensate of electron-hole pairs (weak-coupling regime) or a Bose-Einstein condensate of preformed excitons (strong-coupling regime). A BCS-BEC crossover of the model thus manifests itself as a function of the Coulombic coupling strength.

Journal of Physics Conference Series•Dec 17, 2012•0 citations

Second Thresholds in BEC-BCS-Laser Crossover of Exciton-Polariton Systems

Makoto Yamaguchi, Kenji Kamide, Ryota Nii +2 more

The mechanism of second thresholds observed in several experiments is theoretically revealed by studying the BEC-BCS-laser crossover in exciton-polariton systems. We find that there are two different types of second thresholds: one is a crossover within quasiequilibrium phases and the other is into nonequilibrium (lasing). In both cases, the light-induced band renormalization causes gaps in the conduction and valence bands, which indicates the existence of bound electron-hole pairs in contrast to earlier expectations. We also show that these two types can be distinguished by the gain spectra.

arXiv:1301.4838•Physical Review Letters•Jul 12, 2013•62 citations

Generating functional approach for spontaneous coherence in semiconductor electron-hole-photon systems

Makoto Yamaguchi, Ryota Nii, Kenji Kamide +2 more

Electrons, holes, and photons in semiconductors are interacting fermions and bosons. In this system, a variety of ordered coherent phases can be formed through the spontaneous phase symmetry breaking because of their interactions. The Bose-Einstein condensation (BEC) of excitons and polaritons is one of such coherent phases, which can potentially cross over into the Bardeen-Cooper-Schrieffer (BCS) type ordered phase at high densities under quasiequilibrium conditions, known as the BCS-BEC crossover. In contrast, one can find the semiconductor laser, superfluorescence (SF), and superradiance as relevant phenomena under nonequilibrium conditions. In this paper, we present a comprehensive generating functional theory that yields nonequilibrium Green's functions in a rigorous way. The theory gives us a starting point to discuss these phases in a unified view with a diagrammatic technique. Comprehensible time-dependent equations are derived within the Hartree-Fock approximation, which generalize the Maxwell-semiconductor-Bloch equations under the relaxation time approximation. With the help of this formalism, we clarify the relationship among these cooperative phenomena and we show theoretically that the Fermi-edge SF is directly connected to the e-h BCS phase. We also discuss the emission spectra as well as the gain-absorption spectra.

arXiv:1412.5298•Physical Review B•Mar 16, 2015•21 citations
The crossover between low and high density regimes of exciton-polariton condensates is examined using a BCS wave-function approach. Our approach is an extension of the BEC-BCS crossover theory for excitons, but includes a cavity photon field. The approach can describe both the low density limit, where the system can be described as a Bose-Einstein condensate (BEC) of exciton-polaritons, and the high density limit, where the system enters a photon-dominated regime. In contrast to the exciton BEC-BCS crossover where the system approaches an electron-hole plasma, the polariton high density limit has strongly correlated electron-hole pairs. At intermediate densities, there is a regime with BCS-like properties, with a peak at nonzero momentum of the singlet pair function. We calculate the expected photoluminescence and give several experimental signatures of the crossover.
Recently, the two-dimensional nanocavity exciton-polariton system confined in semiconductor nanocavities has emerged as a promising alternative of BoseEinstein Condensate (BEC). The strong quantum correlations presents in this system, make it an unique candidate for studying entanglement and quantum phase transitions —qualitative changes in the ground state properties—. In this work, we review previous evidence, obtained by us, in the phase transitions of a finite exciton-polariton system. First, by using a BCS wave function to compute the ground state energy of N excitons without the photonic field, a crossover from the high-density electron-hole phase to the BCS excitonic phase is found, at a density which is roughly four times the close-packing density of excitons. Second, by means of a self-consistent procedure with a trial function composed of a coherent photon field and a BCS function for the electron-hole pairs, we obtain the scaling of the critical temperature with the number of polaritons. Using the method proposed originally by Olliver and Zurek, and subsequently developed by Bo Li and Zhi-Xi Wang , we calculate the discord for a generalized density operator, proposed by Blaizot
In this work, we study the exciton-polariton condensate phase transition in a microcavity matter-light system in which electron-hole Coulomb interaction and matter-light coupling effects are treated on an equal footing. In the framework of the unrestricted Hartree-Fock approximation applying the two-dimensional exciton-polariton model, we derive the self-consistent equations determining simultaneously the excitonic and the photonic condenstate order parameters. In the thermal-equilibrium limit, we find a condensed state of the exciton-polariton systems and phase diagrams are then constructed. At a given low temperature, the condensate by its nature shows a crossover from an excitonic to a polaritonic and finally photonic condensed state as the excitation density increases at large detuning. Without the detuning, the excitonic condensed state disappears whereas the polaritonic or photonic phases dominate. The crossover is also found by lowering the Coulomb interaction at a finite matter-light coupling. Lowering the Coulomb interaction or increasing the temperature, the excitonic Mott transition occurs, at which the exciton-polariton condensates dissociate to free electron-hole/photon. Depending on temperature and excitation density, the phase transition of the exciton-polariton condensates is also addressed in signatures of photoluminescence mapping to the photonic momentum distribution.
The BCS to Bose-Einstein condensation (BEC) crossover of electron-hole $(e\text{\ensuremath{-}}h)$ pairs in optically excited semiconductors is studied using the two-band Hubbard model with both repulsive and attractive interactions. Applying the self-consistent ttt-matrix approximation combined with a local approximation, we examine the properties of a normal phase and an excitonic instability. The transition temperature from the normal phase to an $e\text{\ensuremath{-}}h$ pair condensed one is studied to clarify the crossover from an $e\text{\ensuremath{-}}h$ BCS-like state to an excitonic Bose-Einstein condensation, which takes place on increasing the $e\text{\ensuremath{-}}h$ attraction strength. To investigate effects of the repulsive interaction and the $e\text{\ensuremath{-}}h$ mass difference, we calculate the transition temperature for various parameters of the interaction strengths, the $e\text{\ensuremath{-}}h$ particle density, and the mass difference. While the transition temperature in the $e\text{\ensuremath{-}}h$ BCS regime is sufficiently suppressed by the repulsive interaction, that of the excitonic BEC is largely insensitive to it. We also show quantitatively that in the whole regime the mass difference leads to large suppression of the transition temperature.
Motivated by recent experimental and theoretical studies of excitonic insulators, we use the variational cluster approximation to calculate the single-particle Green's function and anomalous Green's function of the Falicov-Kimball model extended by including a finite valence bandwidth. We thus determine the single-particle excitation gap due to the bound-state formation of an electron and a hole. We also evaluate the order parameter of the excitonic insulating state indicating quantum coherence of condensed excitons. We thereby discuss the excitonic insulator that typifies either a BCS condensate of electron-hole pairs (weak-coupling regime) or a Bose-Einstein condensate of preformed excitons (strong-coupling regime). A BCS-BEC crossover of the model thus manifests itself as a function of the Coulombic coupling strength.
The mechanism of second thresholds observed in several experiments is theoretically revealed by studying the BEC-BCS-laser crossover in exciton-polariton systems. We find that there are two different types of second thresholds: one is a crossover within quasiequilibrium phases and the other is into nonequilibrium (lasing). In both cases, the light-induced band renormalization causes gaps in the conduction and valence bands, which indicates the existence of bound electron-hole pairs in contrast to earlier expectations. We also show that these two types can be distinguished by the gain spectra.
Electrons, holes, and photons in semiconductors are interacting fermions and bosons. In this system, a variety of ordered coherent phases can be formed through the spontaneous phase symmetry breaking because of their interactions. The Bose-Einstein condensation (BEC) of excitons and polaritons is one of such coherent phases, which can potentially cross over into the Bardeen-Cooper-Schrieffer (BCS) type ordered phase at high densities under quasiequilibrium conditions, known as the BCS-BEC crossover. In contrast, one can find the semiconductor laser, superfluorescence (SF), and superradiance as relevant phenomena under nonequilibrium conditions. In this paper, we present a comprehensive generating functional theory that yields nonequilibrium Green's functions in a rigorous way. The theory gives us a starting point to discuss these phases in a unified view with a diagrammatic technique. Comprehensible time-dependent equations are derived within the Hartree-Fock approximation, which generalize the Maxwell-semiconductor-Bloch equations under the relaxation time approximation. With the help of this formalism, we clarify the relationship among these cooperative phenomena and we show theoretically that the Fermi-edge SF is directly connected to the e-h BCS phase. We also discuss the emission spectra as well as the gain-absorption spectra.