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arXiv:1004.3230 · Physical Review A

Spatially resolved excitation of Rydberg atoms and surface effects on an atom chip

Atreju Tauschinsky, Rutger M. T. Thijssen, S. Whitlock, H. B. van Linden van den Heuvell, R. J. C. Spreeuw

Published Jun 10, 2010• 126 citations
arXivHTMLPDF

Abstract

We demonstrate spatially resolved, coherent excitation of Rydberg atoms on an atom chip. Electromagnetically induced transparency (EIT) is used to investigate the properties of the Rydberg atoms near the gold-coated chip surface. We measure distance-dependent shifts ($~$$10$ MHz) of the Rydberg energy levels caused by a spatially inhomogeneous electric field. The measured field strength and distance dependence is in agreement with a simple model for the electric field produced by a localized patch of Rb adsorbates deposited on the chip surface during experiments. The EIT resonances remain narrow ($<4$ MHz) and the observed widths are independent of atom-surface distance down to $~$$20$ $\ensuremath{\mu}$m, indicating relatively long lifetime of the Rydberg states. Our results open the way to studies of dipolar physics, collective excitations, quantum metrology, and quantum information processing involving interacting Rydberg excited atoms on atom chips.

DOI
10.1103/physreva.81.063411

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We demonstrate spatially resolved, coherent excitation of Rydberg atoms on an atom chip. Electromagnetically induced transparency (EIT) is used to investigate the properties of the Rydberg atoms near the gold-coated chip surface. We measure distance-dependent shifts (~$$10 MHz) of the Rydberg energy levels caused by a spatially inhomogeneous electric field. The measured field strength and distance dependence is in agreement with a simple model for the electric field produced by a localized patch of Rb adsorbates deposited on the chip surface during experiments. The EIT resonances remain narrow (<4<4<4 MHz) and the observed widths are independent of atom-surface distance down to ~$$20 \ensuremathμ\ensuremath{\mu}\ensuremathμm, indicating relatively long lifetime of the Rydberg states. Our results open the way to studies of dipolar physics, collective excitations, quantum metrology, and quantum information processing involving interacting Rydberg excited atoms on atom chips.
Abstract We theoretically propose that electromagnetically induced transparency (EIT) with cold Rydberg atoms in the proximity to a metallic chip surface can be applied to detect and investigate the Casimir–Polder effect. The absorption spectrum of the probe laser is numerically computed by the Monte Carlo method, taking into account atom-surface interactions (Casimir–Polder effect). The results show that the Casimir–Polder effect shifts the energy level of the Rydberg state and leads to a shift in the EIT transparency window. The shift of resonant frequency depends on the principal quantum number, atom-surface distance and atomic density. The atom-surface interactions have observable impacts on the nonlinear optic response of the ‘Rydberg EIT medium’ near atom chips.
Rydberg-assisted atomic electrometry with thermal vapors offers a promising approach for detecting external electric fields. However, this technique presents significant challenges for measuring low frequencies due to the effects of metal-alkali atoms adsorbed on the interior surface of the vacuum chamber. In this work, we apply high-contrast Rydberg electromagnetically induced transparency (EIT) spectroscopy to systematically investigate these effects, including the influence of laser power and electric field strength. We demonstrate the ability to measure electric field frequencies ranging from 10 Hz to 1 MHz. Additionally, this study identifies a fundamental limit for data capacity in such measurements. Furthermore, we propose a method for precise Stark shift measurements by locking the coupling laser to Zeeman-split Rydberg EIT peaks. Using the Zeeman shift in a reference cell as a stable frequency reference, we are able to track Stark-induced shifts in a science cell and confirm excellent agreement with theoretical predictions. These results provide valuable insights for future precision measurement techniques and field sensing applications based on Rydberg atom systems.
Trapping a Rydberg atom close to a surface is an important step towards the realisation of many proposals for quantum information processing or hybrid quantum systems. One of the challenges in these experiments is posed by the electric field emanating from contaminations on the surface. Here we report on measurements of an electric field created by 87 Rb atoms adsorbed on a 25 nm thick layer of SiO 2 , covering a 90 nm layer of Au. The electric field is measured using a two-photon transition to the and states. The electric field value that we measure is higher than typical values measured above metal surfaces, but is consistent with a recent measurement above a SiO 2 surface. In addition, we measure the temporal behaviour of the field and observe that we can reduce it in a single experimental cycle, using ultraviolet light or by mildly locally heating the surface with one of the excitation lasers, whereas the buildup of the field takes thousands of cycles. We explain these results by a change in the adatom distribution on the surface. These results indicate that, while the stray electric field can be reduced, achieving field-free conditions above a silica-coated gold chip remains challenging.
We observe the shift of Rydberg levels of rubidium close to a copper surface when atomic clouds are repeatedly deposited on it. We measure transition frequencies of rubidium to SSS and DDD Rydberg states with principal quantum numbers nnn between 31 and 48 using the technique of electromagnetically induced transparency. The spectroscopic measurement shows a strong increase of electric fields towards the surface that evolves with the deposition of atoms. Starting with a clean surface, we measure the evolution of electrostatic fields in the range between 30 and 300 $\ensuremath{\mu}$m\mathrm{m}m from the surface. We find that after the deposition of a few hundred atomic clouds, each containing $\ensuremath{\sim}$106{10}^{6}106 atoms, the field of adsorbates reaches 1 V/cm for a distance of 30 $\ensuremath{\mu}$m from the surface. This evolution of the electrostatic field sets serious limitations on cavity QED experiments proposed for Rydberg atoms on atom chips.
We investigate the behavior of electric fields originating from adsorbates deposited on a cryogenic atom chip as it is cooled from room temperature to cryogenic temperature. Using Rydberg electromagnetically induced transparency, we measure the field strength versus distance from a 1 mm square of yttrium barium copper oxide (YBCO) patterned onto a yttria stabilized zirconia chip substrate. We find a localized and stable dipole field at room temperature and attribute it to a saturated layer of chemically adsorbed rubidium atoms on the YBCO. As the chip is cooled towards 83 K we observe a change in sign of the electric field as well as a transition from a localized to a delocalized dipole density. We relate these changes to the onset of physisorption on the chip surface when the van der Waals attraction overcomes the thermal desorption mechanisms. Our findings suggest that through careful selection of substrate materials, it may be possible to reduce the electric fields caused by atomic adsorption on chips, opening up experiments to controlled Rydberg-surface coupling schemes.
Rydberg atoms possess strong electric dipole transitions and tunable energy levels, making them promising candidates for microwave to optical conversion on integrated superconducting atom chips. Achieving strong coupling of the atoms to e.g. the microwave field of an on-chip resonator requires placing the atoms within tens of micrometers from the chip surface. However, inhomogeneous stray electric fields originating from the surface can induce position-dependent Stark forces, resulting in atomic motion and leading to time-dependent shifts of the Rydberg energy levels. We experimentally investigate these effects using time-of-flight and spectroscopic techniques, observing substantial level shifts and signal loss attributable to field-induced atomic motion. A theoretical model incorporating an exponentially decaying surface field with a superimposed bias accurately reproduces the observed dynamics. To mitigate the level shift, we introduce a Stark echo sequence that dynamically reverses the force. This approach suppresses the atomic motion and maintains the atomic resonance. The method relies solely on global field control and is compatible with atom-resonator coupling architectures, providing a robust strategy for preserving coherence of Rydberg atoms in inhomogeneous electric fields near surfaces.