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arXiv:1004.2693 · Physical Review B

Schwinger boson mean field theories of spin liquid states on a honeycomb lattice: Projective symmetry group analysis and critical field theory

Fa Wang

Published Jul 16, 2010• 120 citations
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Abstract

Motivated by the recent numerical evidence [Z. Meng, T. Lang, S. Wessel, F. Assaad, and A. Muramatsu, Nature (London) 464, 847 (2010)] of a short-range resonating valence bond state in the honeycomb lattice Hubbard model, we consider Schwinger boson mean field theories of possible spin liquid states on honeycomb lattice. From general stability considerations the possible spin liquids will have gapped spinons coupled to ${Z}_{2}$ gauge field. We apply the projective symmetry group method to classify possible ${Z}_{2}$ spin liquid states within this formalism on honeycomb lattice. It is found that there are only two relevant ${Z}_{2}$ states, differed by the value of gauge flux, zero or $\ensuremath{\pi}$, in the elementary hexagon. The zero-flux state is a promising candidate for the observed spin liquid and continuous phase transition into commensurate N\'eel order. We also derive the critical field theory for this transition, which is the well-studied O(4) invariant theory [A. V. Chubukov, T. Senthil, and S. Sachdev, Phys. Rev. Lett. 72, 2089 (1994); A. V. Chubukov, S. Sachdev, and T. Senthil, Nucl. Phys. B 426, 601 (1994); S. V. Isakov, T. Senthil, and Y. B. Kim, Phys. Rev. B 72, 174417 (2005)], and has an irrelevant coupling between Higgs and boson fields with cubic power of spatial derivatives as required by lattice symmetry. This is in sharp contrast to the conventional theory [S. Sachdev and N. Read, Int. J. Mod. Phys. B 5, 219 (1991)], where such transition generically leads to incommensurate magnetic order. In this scenario the ${Z}_{2}$ spin liquid could be close to a tricritical point. Soft boson modes will exist at seven different wave vectors. This will show up as low-frequency dynamical spin susceptibility peaks not only at the $\ensuremath{\Gamma}$ point (the N\'eel order wave vector) but also at Brillouin-zone-edge center $M$ points and twelve other points. Some simple properties of the $\ensuremath{\pi}$-flux state are studied as well. Symmetry allowed further neighbor mean field ansatz are derived in appendices which can be used in future theoretical works along this direction.

DOI
10.1103/physrevb.82.024419

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Motivated by the recent numerical evidence [Z. Meng, T. Lang, S. Wessel, F. Assaad, and A. Muramatsu, Nature (London) 464, 847 (2010)] of a short-range resonating valence bond state in the honeycomb lattice Hubbard model, we consider Schwinger boson mean field theories of possible spin liquid states on honeycomb lattice. From general stability considerations the possible spin liquids will have gapped spinons coupled to Z2{Z}_{2}Z2​ gauge field. We apply the projective symmetry group method to classify possible Z2{Z}_{2}Z2​ spin liquid states within this formalism on honeycomb lattice. It is found that there are only two relevant Z2{Z}_{2}Z2​ states, differed by the value of gauge flux, zero or \ensuremathπ\ensuremath{\pi}\ensuremathπ, in the elementary hexagon. The zero-flux state is a promising candidate for the observed spin liquid and continuous phase transition into commensurate N'eel order. We also derive the critical field theory for this transition, which is the well-studied O(4) invariant theory [A. V. Chubukov, T. Senthil, and S. Sachdev, Phys. Rev. Lett. 72, 2089 (1994); A. V. Chubukov, S. Sachdev, and T. Senthil, Nucl. Phys. B 426, 601 (1994); S. V. Isakov, T. Senthil, and Y. B. Kim, Phys. Rev. B 72, 174417 (2005)], and has an irrelevant coupling between Higgs and boson fields with cubic power of spatial derivatives as required by lattice symmetry. This is in sharp contrast to the conventional theory [S. Sachdev and N. Read, Int. J. Mod. Phys. B 5, 219 (1991)], where such transition generically leads to incommensurate magnetic order. In this scenario the Z2{Z}_{2}Z2​ spin liquid could be close to a tricritical point. Soft boson modes will exist at seven different wave vectors. This will show up as low-frequency dynamical spin susceptibility peaks not only at the \ensuremathΓ\ensuremath{\Gamma}\ensuremathΓ point (the N'eel order wave vector) but also at Brillouin-zone-edge center MMM points and twelve other points. Some simple properties of the \ensuremathπ\ensuremath{\pi}\ensuremathπ-flux state are studied as well. Symmetry allowed further neighbor mean field ansatz are derived in appendices which can be used in future theoretical works along this direction.
We study possible spin liquids on square lattice that respect all lattice symmetries and time-reversal symmetry within the framework of Schwinger boson (mean-field) theory. Such spin liquids have spin gap and emergent Z2{Z}_{2}Z2​ gauge field excitations. We classify them by the projective symmetry group method, and find six spin-liquid states that are potentially relevant to the ${J}_{1}\text{\ensuremath{-}}{J}_{2}$ Heisenberg model. The properties of these states are studied under mean-field approximation. Interestingly we find a spin-liquid state that can go through continuous phase transitions to either the N\'eel magnetic order or magnetic orders of the wave vector at the Brillouin zone edge center. We also discuss the connection between our results and the Abrikosov fermion spin liquids.
Spin liquids are novel states of matter with fractionalized excitations. A recent numerical study of Hubbard model on a honeycomb lattice\cite{Meng2010} indicates that a gapped spin liquid phase exists close to the Mott transition. Using Projective Symmetry Group, we classify all the possible spin liquid states by Schwinger fermion mean-field approach. We find there is only one fully gapped spin liquid candidate state: "Sublattice Pairing State" that can be realized up to the 3rd neighbor mean-field amplitudes, and is in the neighborhood of the Mott transition. We propose this state as the spin liquid phase discovered in the numerical work. To understand whether SPS can be realized in the Hubbard model, we study the mean-field phase diagram in the J1−J2J_1-J_2J1​−J2​ spin-1/2 model and find an s-wave pairing state. We argue that s-wave pairing state is not a stable phase and the true ground state may be SPS. A scenario of a continuous phase transition from SPS to the semimetal phase is proposed. This work also provides guideline for future variational studies of Gutzwiller projected wavefunctions.
A symmetry-based analysis (projective symmetry group) is used to study spin-liquid phases on the triangular and Kagom\'e lattices in the Schwinger boson framework. A maximum of eight distinct Z2{Z}_{2}Z2​ spin-liquid states are found for each lattice, which preserve all symmetries. Out of these only a few have nonvanishing nearest-neighbor amplitudes, which are studied in greater detail. On the triangular lattice, only two such states are present---the first (zero-flux state) is the well-known state introduced by Sachdev, which on condensation of spinons leads to the 120\ifmmode^\circ\else\textdegree\fi{} ordered state. The other solution, which we call the $\ensuremath{\pi}$-flux state has not previously been discussed. Spinon condensation leads to an ordering wave vector at the Brillouin zone edge centers, in contrast to the 120\ifmmode^\circ\else\textdegree\fi{} state. While the zero-flux state is more stable with just nearest-neighbor exchange, we find that the introduction of either next-neighbor antiferromagnetic exchange or four-spin ring exchange (of the sign obtained from a Hubbard model) tends to favor the $\ensuremath{\pi}$-flux state. On the Kagom\'e lattice four solutions are obtained---two have been previously discussed by Sachdev, which on spinon condensation give rise to the q=0q=0q=0 and $\sqrt{3}\ifmmode\times\else\texttimes\fi{}\sqrt{3}$ spin-ordered states. In addition we find two states with significantly larger values of the quantum parameter at which magnetic ordering occurs. For one of them this even exceeds unity ${\ensuremath{\kappa}}_{c}\ensuremath{\approx}2.0$ in a nearest-neighbor model, indicating that if stabilized, could remain spin disordered for physical values of the spin. This state is also stabilized by ring-exchange interactions with signs as derived from the Hubbard model.
In a Schwinger-fermion representation we classify all 128 possible spin liquids that preserves SU(2)\mathit{SU}(2)SU(2) spin-rotational symmetry, honeycomb lattice group symmetry, and time-reversal symmetry. Among them we identify a Z2{Z}_{2}Z2​ spin liquid called the sublattice-pairing state (SPS) as the spin liquid phase discovered in recent numerical study on a honeycomb lattice [Meng et al., Nature (London) 464, 847 (2010)]. Our method provides a systematic way to identify spin liquids close to Mott transition. We also show that the SPS is identical to the zero-flux Z2{Z}_{2}Z2​ spin liquid in Schwinger-boson representation [Wang, Phys. Rev. B 82, 024419 (2010)]. through an explicit duality transformation. SPS is connected to an unusual antiferromagnetic ordered phase, which we term the chiral-antiferromagnetic (CAF) phase, by an O(4)O(4)O(4) critical point. The CAF phase breaks the SU(2)\mathit{SU}(2)SU(2) spin rotational symmetry completely and has three Goldstone modes. Our results indicate that there is likely a hidden phase transition between the CAF phase and the simple antiferromagnetic phase at large U/tU/tU/t. We also propose numerical measurements to reveal the CAF phase and the hidden phase transition.
Due to strong geometric frustration and quantum fluctuation, the S=1/2S=1/2S=1/2 quantum Heisenberg antiferromagnet on the kagome\text{kagome}kagome lattice has long been considered as an ideal platform to realize a spin liquid (SL), a phase exhibiting fractionalized excitations without any symmetry breaking. A recent numerical study (Yan et al., e-print arXiv:1011.6114) of the Heisenberg S=1/2,kagomeS=1/2,\text{kagome}S=1/2,kagome lattice model (HKLM) shows, in contrast to earlier results, that the ground state is a singlet-gapped SL with signatures of Z2{\mathbb{Z}}_{2}Z2​ topological order. Motivated by this numerical discovery, we use the projective symmetry group to classify all 20 possible Schwinger fermion mean-field states of Z2{\mathbb{Z}}_{2}Z2​ SLs on the kagome\text{kagome}kagome lattice. Among them we found only one gapped Z2{\mathbb{Z}}_{2}Z2​ SL (which we call the ${\mathbb{Z}}_{2}[0,\ensuremath{\pi}]\ensuremath{\beta}$ state) in the neighborhood of the U(1) Dirac SL state. Since its parent state, i.e., the U(1) Dirac SL, was found [Ran et al., Phys. Rev. Lett. 98, 117205 (2007)] to be the lowest among many other candidate U(1) SLs, including the uniform resonating-valence-bond states, we propose this ${\mathbb{Z}}_{2}[0,\ensuremath{\pi}]\ensuremath{\beta}$ state to be the numerically discovered SL ground state of the HKLM.
Quantum spin liquids are novel phases of matter whose physical properties cannot be captured within the conventional framework of phase transitions. These quantum states are characterized by excitations, called spinons, carrying a fractional value of the integer spin. A description based on a mean-field approximation leads to effective gauge theory. Due to this gauge freedom symmetry group operations act via projective symmetry group (PSG) representations, which can be used to classify quantum states beyond the conventional method. This introducing discussion is found in Chapters 2-6. A preceding PSG classification on the square lattice, which took spin rotational symmetry breaking terms into account, showed that the resulting mean-field states could exhibit topologically non-trivial spinon bands. In Chapter 7, only those el- ements of this Classification are studied, which lead to short-ranged mean-field models. The mutual effect of spinons and visons is scrutinized by adding static configurations of a background gauge field. Spinons and visons form composite ob- jects, which in the case of topological spinon bands, are described by Majorana zero modes. An exact mapping corroborates the relation to topological supercon- ductors and vortices. The effect of multiple visons is investigated, and a possible experimental signature is exposed. Chapter 8 explains how spinon mean-field theory can be used to derive a phe- nomenological effective model for the compound Ca 10 Cr 7 O 28 . A material that was recently proposed as a quantum spin liquid. This low-energy theory consists of spinon hopping processes. The underlying bilayer kagome structure can be simpli- fied to an effective honeycomb lattice. The dynamical spin structure factor is calcu- lated and compared to neutron scattering data. It is discussed how f -wave pairing of spinons can explain small deviations from a linear temperature dependency observed in heat capacity measurements at the low temperatures. This pairing mechanism breaks the U (1) invariance group of the pure hopping model and renders a coherent picture of Ca 10 Cr 7 O 28 being a Z 2 quantum spin liquid. Chapter 9 carries out a PSG classification for the simple-, body centered-, and face centered cubic lattices. Despite a large number of possible PSG representations, only very few describe short-ranged mean-field states. These mean-field models are constructed up to third neighbor couplings and calculated in a self-consistent manner. It is found that the energy is lower for non-trivial sign patterns induced by non-trivial representations of the symmetry generators. Higher neighbor extensions, including pairing terms, yield lower mean-field ground state energies compared to extensions with only hopping terms. For the fcc lattice, a first neighbor state could be identified, which exhibits symmetry protected zero-energy modes.