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arXiv:1004.1161 · Physical Review A

Hyperfine and optical barium ion qubits

Matthew Dietrich, Nathan Kurz, T. Noel, Gang Shu, B. B. Blinov

Published May 20, 2010• 41 citations
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Abstract

State preparation, qubit rotation, and high fidelity readout are demonstrated for two different $^{137}\mathrm{Ba}{}^{+}$ qubit types. First, an optical qubit on the narrow $6{S}_{1/2}$ to $5{D}_{5/2}$ transition at 1.76 $\ensuremath{\mu}$m is implemented. Then, leveraging the techniques developed there for readout, a ground-state hyperfine qubit using the magnetically insensitive transition at 8 GHz is accomplished.

DOI
10.1103/physreva.81.052328

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State preparation, qubit rotation, and high fidelity readout are demonstrated for two different 137Ba+^{137}\mathrm{Ba}{}^{+}137Ba+ qubit types. First, an optical qubit on the narrow 6S1/26{S}_{1/2}6S1/2​ to 5D5/25{D}_{5/2}5D5/2​ transition at 1.76 \ensuremathμ\ensuremath{\mu}\ensuremathμm is implemented. Then, leveraging the techniques developed there for readout, a ground-state hyperfine qubit using the magnetically insensitive transition at 8 GHz is accomplished.
We present a method for achieving high fidelity state preparation and measurement (SPAM) using trapped ion hyperfine qubits with nuclear spins higher than I=1/2I=1/2I=1/2. The ground states of these higher nuclear spin isotopes do not afford a simple frequency-selective state preparation scheme. We circumvent this limitation by stroboscopically driving strong and weak transitions, blending fast optical pumping using dipole transitions, and narrow microwave or optical quadrupole transitions. We demonstrate this method with the I=3/2I=3/2I=3/2 isotope 137Ba+^{137}{\mathrm{Ba}}^{+}137Ba+ to achieve a SPAM infidelity of $(9.0\ifmmode\pm\else\textpm\fi{}1.3)\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}5}$ ($\ensuremath{-}40.5\ifmmode\pm\else\textpm\fi{}0.6\text{ }\text{ }\mathrm{dB}$), facilitating the use of a wider range of ion isotopes with favorable wavelengths and masses for quantum computation.
High-fidelity operation of a radioactive trapped-ion qubit, 133^{133}133Ba+^++
133^{133}133Ba+^++ has been identified as an attractive ion for quantum information processing due to the unique combination of its spin-1/2 nucleus, visible wavelength electronic transitions, and long D-state lifetimes ($\\tau\\sim 1 min).Usingamicrogramsourceofradioactivematerial,wetrapandlaser−coolthesynthetictextitA=133radioisotopeofbariumII(1~min). Using a microgram source of radioactive material, we trap and laser-cool the synthetic \\textit{A} = 133 radioisotope of barium II (1 min).Usingamicrogramsourceofradioactivematerial,wetrapandlaser−coolthesynthetictextitA=133radioisotopeofbariumII(\\tau_{1/2} \\approx 10.5 yr)inaradio−frequencyiontrap.Todemonstratehighfidelityqubitoperations,anumberofunknownstateenergieswereneeded.Wemeasuretheisotopeshiftandhyperfinestructureofthe6~yr) in a radio-frequency ion trap. To demonstrate high fidelity qubit operations, a number of unknown state energies were needed. We measure the isotope shift and hyperfine structure of the 6 yr)inaradio−frequencyiontrap.Todemonstratehighfidelityqubitoperations,anumberofunknownstateenergieswereneeded.Wemeasuretheisotopeshiftandhyperfinestructureofthe6^2PPP_{1/2}\\leftrightarrow 5^2DDD_{3/2}$ electronic transition needed for laser cooling, state preparation, and state detection of the clock-state hyperfine and optical qubits. For high-fidelity operations with electron shelving, we report measurements of the 62^22P3/2_{3/2}3/2​ and 525^252D5/2_{5/2}5/2​ hyperfine splittings, as well as the~62^22P3/2 leftrightarrow 62_{3/2}~\\leftrightarrow~6^23/2​ leftrightarrow 62S1/2_{1/2}1/2​ and ~62^22P3/2 leftrightarrow 52_{3/2}~\\leftrightarrow~5^23/2​ leftrightarrow 52D5/2_{5/2}5/2​ transition frequencies. Using these transitions, we demonstrate high-fidelity \\ba \\ hyperfine qubit manipulation with electron shelving detection to benchmark qubit state preparation and measurement (SPAM). Using single-shot, threshold discrimination, we measure an average SPAM fidelity of mathcalF=0.99971(3)\\mathcal{F} = 0.99971(3)mathcalF=0.99971(3), a factor of approx\\approxapprox 2 improvement over the best reported performance of any qubit.Finally, we report the 62^22P1/2leftrightarrow52_{1/2}\\leftrightarrow 5^21/2​leftrightarrow52D3/2_{3/2}3/2​ electronic transition isotope shift for the rare \\textit{A} = 130 and 132 barium nuclides, completing the spectroscopic characterization necessary for laser cooling all long-lived barium II isotopes.
Atomic ions can be isolated from their environment through laser-cooling and trapping, making them useful for quantum information processing, measurement, and sensing. A variety of atomic ion species have been used as qubits. Hyperfine qubits with nuclear spin I = 1/2 have demonstrated the long qubit coherence times with simple, robust laser manipulation. Other qubits (I ≠ 1/2) have easily-prepared, long-lived metastable electronic excited states, and simple discrimination between these states allows high fidelity readout. However, none of the naturally- occurring, atomic ions with nuclear spin I = 1/2 have these excited states that are simultaneously long-lived and easy to prepare. We demonstrate loading, cooling, and qubit manipulation of an artificial, I = 1/2 species of barium with visible wavelength lasers: 133Ba+. We achieved a single shot qubit state preparation and readout fidelity of F = 0.9997, the lowest error rate ever achieved by any qubit on any platform.
We demonstrate the use of trapped ytterbium ions as quantum bits for quantum information processing. We implement fast, efficient state preparation and state detection of the first-order magnetic field-insensitive hyperfine levels of 171Yb+^{171}\mathrm{Yb}^{+}171Yb+, with a measured coherence time of 2.5s2.5\phantom{\rule{0.3em}{0ex}}\mathrm{s}2.5s. The high efficiency and high fidelity of these operations is accomplished through the stabilization and frequency modulation of relevant laser sources.
We propose and demonstrate a protocol for high-fidelity indirect readout of trapped ion hyperfine qubits, where the state of a 9Be+^{9}{\mathrm{Be}}^{+}9Be+ qubit ion is mapped to a 25Mg+^{25}{\mathrm{Mg}}^{+}25Mg+ readout ion using laser-driven Raman transitions. By partitioning the 9Be+^{9}{\mathrm{Be}}^{+}9Be+ ground-state hyperfine manifold into two subspaces representing the two qubit states and choosing appropriate laser parameters, the protocol can be made robust to spontaneous photon scattering errors on the Raman transitions, enabling repetition for increased readout fidelity. We demonstrate combined readout and back-action errors for the two subspaces of ${1.2}_{\ensuremath{-}0.6}^{+1.1}\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}4}$ and ${0}_{\ensuremath{-}0}^{+1.9}\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}5}$ with 68% confidence while avoiding decoherence of spectator qubits due to stray resonant light that is inherent to direct fluorescence detection.
Quantum state preparation for trapped-ion qubits often relies on high-quality circularly polarized light, which may be difficult to achieve with chip-based integrated optics technology. We propose and implement a hybrid optical and microwave scheme for intermediate-field hyperfine qubits which instead relies on frequency selectivity. Experimentally, we achieve 99.94 % fidelity for linearly polarized ( σ + / σ − ) light, using Ca + 43 at 28.8 mT. We find that the fidelity remains above 99.8 % for a mixture of all polarizations ( σ + / σ − / π ) . We calculate that the method is capable of 99.99 % fidelity in Ca + 43 , and even higher fidelities in heavier ions such as Ba + 137 . Published by the American Physical Society 2024