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arXiv:1003.5858 · New Journal of Physics

Dynamical crystal creation with polar molecules or Rydberg atoms in optical lattices

Johannes Schachenmayer, Igor Lesanovsky, Andrea Micheli, Andrew J. Daley

Published Oct 29, 2010• 130 citations
arXivHTMLPDF

Abstract

We investigate the dynamical formation of crystalline states with systems of polar molecules or Rydberg atoms loaded into a deep optical lattice. External fields in these systems can be used to couple the atoms or molecules between two internal states: one that is weakly interacting and one that exhibits a strong dipole–dipole interaction. By appropriate time variation of the external fields, we show that it is possible to produce crystalline states of the strongly interacting states with high filling fractions chosen via the parameters of the coupling. We study the coherent dynamics of this process in one dimension (1D) using a modified form of the time-evolving block decimation (TEBD) algorithm, and obtain crystalline states for system sizes and parameters corresponding to realistic experimental configurations. For polar molecules these crystalline states will be long-lived, assisting in a characterization of the state via the measurement of correlation functions. We also show that as the coupling strength increases in the model, the crystalline order is broken. This is characterized in 1D by a change in density–density correlation functions, which decay to a constant in the crystalline regime, but show different regions of exponential and algebraic decay for larger coupling strengths.

DOI
10.1088/1367-2630/12/10/103044

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We investigate the dynamical formation of crystalline states with systems of polar molecules or Rydberg atoms loaded into a deep optical lattice. External fields in these systems can be used to couple the atoms or molecules between two internal states: one that is weakly interacting and one that exhibits a strong dipole–dipole interaction. By appropriate time variation of the external fields, we show that it is possible to produce crystalline states of the strongly interacting states with high filling fractions chosen via the parameters of the coupling. We study the coherent dynamics of this process in one dimension (1D) using a modified form of the time-evolving block decimation (TEBD) algorithm, and obtain crystalline states for system sizes and parameters corresponding to realistic experimental configurations. For polar molecules these crystalline states will be long-lived, assisting in a characterization of the state via the measurement of correlation functions. We also show that as the coupling strength increases in the model, the crystalline order is broken. This is characterized in 1D by a change in density–density correlation functions, which decay to a constant in the crystalline regime, but show different regions of exponential and algebraic decay for larger coupling strengths.
We study a LiCs strongly-interacting molecular gas loaded into an one-dimensional optical lattice at quarter filling. The molecules are in the lowest electronic and vibrational state, X1ΣX^{1}ΣX1Σ (ν=0ν=0ν=0). Due to the large intermolecular distance and low filling, dipole-dipole interaction in the nearest-neighbor approximation governs the dynamics of the rotational excitations. For low DC electric field strengths, the full set of rotational levels N=0,1N=0,1N=0,1 must be taken into account, nevertheless, our calculations show that very weak fields act as field-selectors disclosing two- and three-level systems out of the original four-level one. The dynamics and the generated von Neumann entanglement entropy among the internal rotational states throughout the evolution are presented for low, moderate and strong fields . We observe a sharp and monotonous growth of the entanglement as the dynamics take place showing the potential of these molecular systems to be used in quantum information protocols. The numerical simulations are performed by means of the Time-Evolving Block Decimation algorithm based on the Matrix Product State formalism and the Susuki-Trotter decomposition.
In this thesis, we consider the forms of non-equilibrium phenomena that can arise in atoms or polar molecules trapped in a deep optical lattice and coupled by dipolar internal degrees of freedom. We specifically focus on only two internal states, which results in the systems studied behaving as spin−1/2-1/2−1/2 models with long-range interactions. We first study a closed system with both static and resonant near-field dipole interactions under an external drive. By studying the uniform mean-field dynamics of the system, we find the dynamics are given by Rabi oscillations, with a bifurcation in the dynamics as a function of drive strength between small scale and large scale oscillations. Analysing the stability of these oscillations to small fluctuations reveals that interactions tend to cause the oscillations to decohere. However, we find parameter regimes where coherent oscillations can persist for high enough intensity drive. We then consider the effects of an environment on the non-equilibrium dynamics of the near-field dipole model. We find that within the mean-field approximation, an environment causes the system to relax to many novel steady state spin configurations, such as spin density waves, antiferromagnetism and long-time oscillations, as well as bistabilities between these phases. To assess the validity of the mean-field approximation, we compare our mean-field results to small quantum systems. We carry out a similar analysis on a system with far-field dipole interactions, where it is necessary to introduce nonlocal dissipation, which results in several decay modes into the environment. These decay modes lead to instabilities of many of the steady state phases that occurred in the near-field dipole system, leading to the emergence of more spin density wave and oscillatory phases. Finally, we examine the dynamics on the approach to steady state in a dissipative dipolar system by studying Rydberg atoms coupled to a photonic crystal waveguide, which mediates an effective dipole-dipole interaction between the atoms. We find that if two excitations exist in the system, then bound states can form, with nonlocal dissipation resulting in a momentum dependent decay rate of the bound states and also greater freedom in engineering the bound state energy dispersion.
We study the growth dynamics of ordered structures of strongly interacting polar molecules in optical lattices. Using a dipole blockade of microwave excitations, we map the system onto an interacting spin-1/2 model possessing ground states with crystalline order, and describe a way to prepare these states by nonadiabatically driving the transitions between molecular rotational levels. The proposed technique bypasses the need to cross a phase transition and allows for the creation of ordered domains of considerably larger size compared to approaches relying on adiabatic preparation.
The creation of a gas of ultracold polar molecules with a high phase space density brings new possibilities beyond experiments with ultracold atomic gases. In particular, long-range, anisotropic, and tunable dipole-dipole interactions open the way for novel quantum gases, with applications including strongly correlated many-body systems, and ultracold chemistry. This thesis will present the final steps to complete control over both internal and external degrees of freedom of the molecule which allows us to control, and even completely suppress, the chemical reactions between molecules. First, the control over internal states has been achieved through coherent state transfer to the ro-vibronic ground state and coherent manipulations of the hyperfine and rotational states with microwave radiation. Second, external degrees of freedom are controlled by loading the gas into an optical lattice. With the molecules loaded into a one-dimensional lattice, the orientation of the molecular collisions is controlled by manipulating both internal (hyperfine states) and external (motional states in the direction of tight confinement) degrees of freedom. Most striking is that by preparing the molecules all in the lowest band of the lattice in the same internal state, the molecular collisions can only occur in a side-by-side" orientation, where the chemical reaction rate is suppressed by the repulsive dipole-dipole interactions. The chemical reaction can be suppressed completely by further constraining the motion in the trap in a strong 3D lattice. Here we see lifetimes longer than 20 s, limited by o-resonant light scattering. Finally, the ac polarizability of the molecules is explored and controlled. The different rotational states of the molecule have different polarizabilities and will experience a different trapping force in both the optical dipole trap or lattice. We show that there is a magic angle" between the quantization axis and the polarization of the trapping laser at which the polarizabilities of two different rotational states can be matched, eliminating dephasing and allowing for coherent manipulations between rotational states.
We describe the emergence of strong spatial correlations, akin to liquidlike behavior and crystallization effects, in low- (one- and two-)dimensional gases of cold Rydberg atoms. The presence of an external electric field permanently polarizes the atoms, which became highly correlated due to the long-range dipole-dipole interaction. We describe a theoretical approach particularly suited for strongly coupled systems and numerically obtain both the two-particle distribution function and the static structure factor. The experimental implementation of such highly interacting systems is discussed, including detailed calculations of the interaction strength for different Rydberg states. The results provide insights into many-body effects associated with strongly interacting Rydberg atoms, including the possibility of observing highly ordered phases.
We show that indirect spin-spin interactions between effective spin-1/2 systems can be realized in two parallel one-dimensional optical lattices loaded with polar molecules and/or Rydberg atoms. The effective spin can be encoded into low-energy rotational states of polar molecules or long-lived states of Rydberg atoms, tightly trapped in a deep optical lattice. The spin-spin interactions can be mediated by Rydberg atoms, placed in a parallel shallow optical lattice, interacting with the effective spins by charge-dipole (for polar molecules) or dipole-dipole (for Rydberg atoms) interaction. Indirect XXXXXX, Ising, and XXZXXZXXZ interactions with interaction coefficients ${J}^{\ensuremath{\perp}}$ and Jzz{J}^{zz}Jzz sign varying with interspin distance can be realized, in particular, the ${J}_{1}\ensuremath{-}{J}_{2} XXZ$ model with frustrated ferro-(antiferro-)magnetic nearest (next-nearest) neighbor interactions.