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arXiv:1003.5502 · Physical Review Letters

Disorder in a Quantum Spin Liquid: Flux Binding and Local Moment Formation

A. J. Willans, J. T. Chalker, Roderich Moessner

Published Jun 8, 2010• 124 citations
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Abstract

We study the consequences of disorder in the Kitaev honeycomb model, considering both site dilution and exchange randomness. We show that a single vacancy binds a flux and induces a local moment. This moment is polarized by an applied field h: in the gapless phase, for small h the local susceptibility diverges as χ(h)∼ln(1/h); for a pair of nearby vacancies on the same sublattice, this even increases to χ(h)∼1/(h[ln(1/h)](3/2)). By contrast, weak exchange randomness does not qualitatively alter the susceptibility but has its signature in the heat capacity, which in the gapless phase is power law in temperature with an exponent dependent on disorder strength.

DOI
10.1103/physrevlett.104.237203

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We study the consequences of disorder in the Kitaev honeycomb model, considering both site dilution and exchange randomness. We show that a single vacancy binds a flux and induces a local moment. This moment is polarized by an applied field h: in the gapless phase, for small h the local susceptibility diverges as χ(h)∼ln(1/h); for a pair of nearby vacancies on the same sublattice, this even increases to χ(h)∼1/(hln(1/h)). By contrast, weak exchange randomness does not qualitatively alter the susceptibility but has its signature in the heat capacity, which in the gapless phase is power law in temperature with an exponent dependent on disorder strength.
We investigate the properties of the Kitaev honeycomb model with both site dilution and exchange randomness. Embarking on this work, we review disorder in some strongly correlated electron systems, including spin-½ and spin-1 Heisenberg antiferromagnetic chains, two dimensional Heisenberg antiferromagnets, the cuprates and graphene. We outline some aspects of resonating valence bond phases, valence bond solids, spin liquids and quantum computation that are pertinent to an understanding of the Kitaev model. The properties of the Kitaev model without disorder are discussed and it is found to be a critical spin liquid, with algebraic correlations in two spin operators sigma^{alpha}_{i}sigma^{alpha}_{j}, where i and j,/em> are either end of a link of type alpha = x, y or z on the honeycomb lattice. The Kitaev model is exactly solvable and we show that this remains so in the presence of site dilution and exchange randomness. We find that vacancies bind a flux. In the gapped phase, a vacancy forms an effective paramagnetic moment. With two or more vacancies we describe the interaction of their effective moments and show that a finite density of vacancies leads to a divergent macroscopic susceptibility at small fields. In the gapless phase the effective moment has a susceptibility that is, to leading order at small fields, chi(h)~log(1/h). Interaction between the moments from two vacancies on opposite sublattices cuts off this divergence in susceptibility at a large but finite constant. Two vacancies on the same sublattice behave quite differently and we find the combined susceptibility is parametrically larger than that of an isolated vacancy, chi(h)sim [h(log(1/h))^{3/2}]^{-1}. We also investigate the effects of slowly varying, quenched disorder in exchange coupling. We demonstrate that this does not qualitatively affect the susceptibility but show that the heat capacity C ~ T^{2/z}, where z is a measure of the disorder and increases from one with increasing disorder strength.
We investigate the properties of the Kitaev honeycomb model with both site dilution and exchange randomness. Embarking on this work, we review disorder in some strongly correlated electron systems, including spin-½ and spin-1 Heisenberg antiferromagnetic chains, two dimensional Heisenberg antiferromagnets, the cuprates and graphene. We outline some aspects of resonating valence bond phases, valence bond solids, spin liquids and quantum computation that are pertinent to an understanding of the Kitaev model. The properties of the Kitaev model without disorder are discussed and it is found to be a critical spin liquid, with algebraic correlations in two spin operators sigma^{alpha}_{i}sigma^{alpha}_{j}, where i and j are either end of a link of type alpha = x, y or z on the honeycomb lattice. The Kitaev model is exactly solvable and we show that this remains so in the presence of site dilution and exchange randomness. We find that vacancies bind a flux. In the gapped phase, a vacancy forms an effective paramagnetic moment. With two or more vacancies we describe the interaction of their effective moments and show that a finite density of vacancies leads to a divergent macroscopic susceptibility at small fields. In the gapless phase the effective moment has a susceptibility that is, to leading order at small fields, chi(h)~log(1/h). Interaction between the moments from two vacancies on opposite sublattices cuts off this divergence in susceptibility at a large but finite constant. Two vacancies on the same sublattice behave quite differently and we find the combined susceptibility is parametrically larger than that of an isolated vacancy, chi(h)sim [h(log(1/h))^{3/2}]^{-1}. We also investigate the effects of slowly varying, quenched disorder in exchange coupling. We demonstrate that this does not qualitatively affect the susceptibility but show that the heat capacity C ~ T^{2/z}, where z is a measure of the disorder and increases from one with increasing disorder strength.
We study the physical consequences of site dilution in Kitaev's honeycomb model, in both its gapped and gapless phases. We show that a vacancy binds a flux of the emergent Z2{Z}_{2}Z2​ gauge field and induces a local moment. In the gapped phase this moment is free while in the gapless phase the susceptibility has the dependence $\ensuremath{\chi}(h)\ensuremath{\sim}\mathrm{ln}(1/h)$ on field strength hhh. Vacancy moments have interactions that depend on their separation, their relative sublattice, and the phase of the model. Strikingly, in the gapless phase, two nearby vacancies on the same sublattice have a parametrically larger $\ensuremath{\chi}(h)\ensuremath{\sim}{(h{[\mathrm{ln}(1/h)]}^{3/2})}^{\ensuremath{-}1}$. In the gapped phase, even a finite density of randomly distributed vacancies remains tractable, via a mapping to a bipartite random hopping problem. This leads to a strong disorder form of the low-energy thermodynamics, with a Dyson-type singularity in the density of states for excitations.
We address the effects of disorder in the Kitaev honeycomb model, focussing on the interplay of disorder and strong interactions in a quantum spin liquid. It is shown that nonmagnetic impurities bind a quantum of the emergent gauge flux. We find the formation of a local moment, which leads to a local magnetic response near the impurity which is parametrically larger than in the bulk. The magnetic response of a pair of impurities can be parametrically larger than that of an isolated one, and can in particular dominate the magnetic response of the system. The role of such impurities as diagnostic of the spin liquid state are emphasized – most remarkably, they provide a direct signature of the emergent gauge field.
The Kitaev honeycomb model supports gapless and gapped quantum spin liquid phases. Its exact solvability relies on extensively many locally conserved quantities. Any real-world manifestation of these phases would include imperfections in the form of disorder and interactions that break integrability. We show that the latter qualitatively alters the properties of vacancies in the gapless Kitaev spin liquid: (i) Isolated vacancies carry a magnetic moment, which is absent in the exactly solvable case. (ii) Pairs of vacancies on even or opposite sublattices gap each other with distinct power laws that reveal the presence of emergent gauge flux.
We study the effect of adding disorder to the Kitaev model on the hyperhoneycomb lattice, which hosts both gapped and gapless spin liquid phases with an emergent Z2{\mathbb{Z}}_{2}Z2​ gauge field. The latter has an unusual gapless spectrum of Majorana fermion excitations, with a co-dimension-two Fermi ring. We thus address the question of the interplay of topological physics and disorder by considering the properties of isolated single and pairs of vacancies. We show that near the vacancies, the local magnetic response to a field hz{h}_{z}hz​ is parametrically enhanced in comparison to the pristine bulk. Unlike the previously studied case of the 2D honeycomb Kitaev model, the vacancies do not bind a flux of the Z2{\mathbb{Z}}_{2}Z2​ gauge field. In the gapped phase, an isolated vacancy gives rise to effectively free spin-half moments with a nonuniversal coupling to an external field. In the gapless phase, the low-field magnetization is suppressed parametrically to ${(\ensuremath{-}ln{h}_{z})}^{\ensuremath{-}1/2}$ because of interactions with the surrounding spin liquid. We also show that a pair of vacancies is subject to a sublattice-dependent interaction on account of coupling through the bulk spin liquid, which is spatially anisotropic even when all Kitaev couplings have equal strength. This coupling is thus exponentially suppressed with distance in the gapped phase. In the gapless phase, two vacancies on the same (opposite) sublattice exhibit an enhanced (suppressed) low-field response, amounting to an effectively (anti-)ferromagnetic interaction.