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arXiv:1003.1788 · Physical Review A

Quantum control of light through an atom-molecule dark state

Hui Jing, Yuangang Deng, Weiping Zhang

Published Aug 4, 2009• 13 citations
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Abstract

We propose to use a quantized version of coherent two-color photoassociation to realize a hybrid device for quantum control of light. The dynamical features of this system are exhibited, including the slowing down or storage of light and the molecular matter-wave solitons. This may indicate a hybrid atom-molecule quantum device for storage and retrieve of optical information.

DOI
10.1103/physreva.80.025601

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Controlled manipulation, storage and retrieval of quantum information is essential for quantum communication and computing. Quantum memories for light, realized with cold atomic samples as the storage medium, are prominent for their high storage efficiencies and lifetime. We demonstrate the controlled transport of stored light over 2.4 mm in such a storage system and show that the transport process and its dynamics only have a minor effect on the coherence of the storage. Extending the presented concept to longer transport distances and augmenting the number of storage sections will allow for the development of novel quantum devices such as optical race track memories or optical quantum registers.
We study coherent photoassociation, phenomena analogous to coherent optical transients in few-level systems, which may take place in photoassociation of an atomic Bose-Einstein condensate but not in a nondegenerate gas. We develop a second-quantized Hamiltonian to describe photoassociation, and apply the Hamiltonian both in the momentum representation and in the position representation (field theory). The solution of the two-mode problem, including only one mode each for the atomic and molecular condensates, displays analogs of Rabi oscillations and rapid adiabatic passage. A classical version of the field theory for atoms and molecules is used to demonstrate that, in the presence of photoassociating light, a joint atom-molecule condensate is unstable against the growth of density fluctuations. Experimental complications, including spontaneous emission and unwanted ``rogue'' photodissociation from a photoassociated molecule, are analyzed. A two-color Raman scheme is studied as a method to set up an effective two-mode scheme with reduced spontaneous-emission losses. We discuss photoassociation rates and photoassociation Rabi frequencies for high-lying vibrational states in alkali dimers both on the basis of molecular-structure calculations, and by comparing with an experiment [Wynar et al., Science 287, 1016 (2000)].
A study of coherent photoassociation is presented for the case of an atomic Bose-Einstein condensate. It is shown that the phenomenon is analogous to coherent optical transient in a few-level system, with a difference that the participating levels have Bose enhanced populations. A second-quantized Hamiltonian in momentum and position representation is developed to describe photoassociation. A classical version of the field theory for atoms and molecules is used to demonstrate that in the presence of photoassociating light, a joint atom-molecule condensate is unstable against the growth of the density fluctuations. ^ A simple mean-field model of atom-molecule Bose-Einstein condensate is constructed and it is shown that in the model there is no collapse, irrespective of the sign of the effective atom-atom scattering length. The properties of the two most important eigenstates, the ground state and the twin state, are determined for different values of the system parameters δ and K, the detuning and the atom-molecule coupling, respectively. It is shown that in a coupled atom-molecule system a collapse is replaced by a dynamical instability. The lines in the parameter space where these instabilities occur are in fact fractures where the underlying eigenstates discontinuously change. The features of instability are in good qualitative agreement with the experimental observations of collapse. ^
We show the quantum state transfer technique in two-color photoassociation (PA) of a Bose-Einstein condensate, where a quantized field is used to couple the free-bound transition from atom state to excited molecular state. Under the weak excitation condition, we find that quantum states of the quantized field can be transferred to the created molecular condensate. The feasibility of this technique is confirmed by considering the atomic and molecular decays discovered in the current PA experiments. The present results allow us to manipulate quantum states of molecules in the photoassociation of a Bose-Einstein condensate.
A new scheme is suggested to manipulate the probe transitions (and hence the optical properties of atomic vapors) via double-control destructive and constructive quantum interferences. The influence of phase coherence between the two control transitions on the probe transition is also studied. The most remarkable feature of the present scheme is that the optical properties (absorption, transparency and dispersion) of an atomic system can be manipulated using this double-control multi-pathway interferences (multiple routes to excitation). It is also shown that a four-level system will exhibit a two-level resonant absorption because the two control levels (driven by the two control fields) form a dark state (and hence a destructive quantum interference occurs between the two control transitions). However, the present four-level system will exhibit electromagnetically induced transparency to the probe field when the three lower levels (including the probe level and the two control levels) form a three-level dark state. The present scenario has potential applications in new devices (e.g. logic gates and sensitive optical switches) and new techniques (e.g. quantum coherent information storage).