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arXiv:1001.0372 · Journal of Physics A Mathematical and Theoretical

A generalized Landau–Lifshitz equation for an isotropic SU(3) magnet

Julia Bernatska, P Holod

Published Jan 21, 2009• 23 citations
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Abstract

In the paper we obtain equations for large-scale fluctuations of the mean field (the field of magnetization and quadrupole moments) in a magnetic system realized by a square (cubic) lattice of atoms with spin s >= 1 at each site. We use the generalized Heisenberg Hamiltonian with biquadratic exchange as a quantum model. A quantum thermodynamical averaging gives classical effective models, which are interpreted as Hamiltonian systems on coadjoint orbits of Lie group SU(3).

DOI
10.1088/1751-8113/42/7/075401

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In the paper we obtain equations for large-scale fluctuations of the mean field (the field of magnetization and quadrupole moments) in a magnetic system realized by a square (cubic) lattice of atoms with spin s >= 1 at each site. We use the generalized Heisenberg Hamiltonian with biquadratic exchange as a quantum model. A quantum thermodynamical averaging gives classical effective models, which are interpreted as Hamiltonian systems on coadjoint orbits of Lie group SU(3).
We study the quantum and thermal phase transition phenomena of the SU(3) Heisenberg model on triangular lattice in the presence of magnetic fields. Performing a scaling analysis on large-size cluster mean-field calculations endowed with a density-matrix renormalization-group solver, we reveal the quantum phases selected by quantum fluctuations from the massively degenerate classical ground-state manifold. The magnetization process up to saturation reflects three different magnetic phases. The low- and high-field phases have strong nematic nature, and especially the latter is found only via a nontrivial reconstruction of symmetry generators from the standard spin and quadrupolar description. We also perform a semiclassical Monte Carlo simulation to show that thermal fluctuations prefer the same three phases as well. Moreover, we find that exotic topological phase transitions driven by the binding-unbinding of fractional (half-)vortices take place, due to the nematicity of the low- and high-field phases. Possible experimental realization with alkaline-earth-like cold atoms is also discussed.
Abstract Magnetic systems can be described by the classical Landau–Lifshitz (LL) equation or the fully quantum open generalized Heisenberg model. Using the Lindblad master equation and the mean-field approximation, we demonstrate that the open generalized Heisenberg model is reduced to a generalized LL equation. The open dynamic is modeled using spin-boson interactions with a common bosonic reservoir at thermal equilibrium. By tracing out the bosonic degrees of freedom, we obtain two different decoherence mechanisms: on-site dissipation and an effective spin–spin interaction mediated by bosons. Using our approach, we perform hysteresis calculations, closely connected with the Stoner–Wohlfarth theory. We compare the exact numerical master equation and the mean-field model, revealing the role of correlations originated by non-local interactions. Our work opens new horizons for the study of the LL dynamics from an open quantum formalism.
The Landau-Lifshitz equation describes the time evolution of magnetic dipoles and can be derived by taking the classical limit of a quantum mechanical spin Hamiltonian. To take this limit, one constrains the many-body quantum state to a tensor product of coherent states, thereby neglecting entanglement between sites. Expectation values of the quantum spin operators produce the usual classical spin dipoles. One may also consider expectation values of polynomials of the spin operators, leading to quadrupole and higher-order spin moments, which satisfy a dynamical equation of motion that generalizes the Landau-Lifshitz dynamics [Zhang and Batista, Phys. Rev. B 104, 104409 (2021)]. Here we reformulate the dynamics of these ${N}^{2}\ensuremath{-}1$ generalized spin components as a mean-field Schr\"odinger equation on the NNN-dimensional coherent state. This viewpoint suggests efficient integration methods that respect the local symplectic structure of the classical spin dynamics.
There is a version of the Landau–Lifshitz equation that takes into account the Coulomb exchange interactions between atoms, expressed by the term ∼s×△s{\sim}\mathbf{s}\times\triangle\mathbf{s}∼s×△s . On the other hand, ions in magnetic materials have several valence electrons on the ddd -shell, and, therefore, the Hamiltonian of many-electron atoms with spins S>1S>1S>1 should include a biquadratic exchange interaction. We propose a novel fundamental microscopic derivation of the spin density evolution equation with an explicit form of biquadratic exchange interaction using the method of many-particle quantum hydrodynamics. The equation for the spin density evolution is obtained from the many-particle Schrödinger–Pauli equation and contains the contributions of the usual Coulomb exchange interaction and the biquadratic exchange. Furthermore, the derived biquadratic exchange torque in the spin density evolution equation is proportional to the nematic tensor for the medium of atoms with spin S=1S=1S=1 . Our method may be very attractive for further studies of the magnetoelectric effect in multiferroics.
The statistical thermodynamics of the quantum spin- s XXZ Heisenberg model in the Weiss (mean-field) limit rests on the outer multiplicities of the irreducible representations in the Clebsch–Gordan decomposition of the n -fold spin- s tensor product, which determine the energy-level degeneracies and hence the partition function. Using known closed forms for these multiplicities in terms of generalized binomial coefficients of order 2 s + 1 , we write the exact finite-size partition function of the effective collective Hamiltonian and evaluate its thermodynamic limit by a large-deviation (Laplace) analysis validated against direct summations for systems of up to n = 10 4 spins. The free energy then follows from a two-parameter variational principle in the total spin and the magnetization per site. The ferromagnetic ordering is driven by the rotationally invariant part of the Hamiltonian, so that the Curie temperature T c = 1 3 J s ( s + 1 ) is independent of the anisotropy Δ, and the transition is of second order for every spin s , with classical mean-field exponents. The anisotropy reshapes the phase diagram: for Δ < 1 the field-driven first-order line of the isotropic ( Δ = 1 ) model opens into a dome of easy-plane ferromagnetic order, bounded by a continuous transition that restores the residual U(1) symmetry, and no first-order transitions or metastability occur throughout − 1 ≤ Δ < 1 ; the isotropic Curie-Weiss ferromagnet is recovered as Δ → 1. In two appendices we detail the asymptotics of the outer multiplicities down to the Gaussian-fluctuation prefactor and discuss the q -number and Jacobi-theta structures underlying the model, including the partial-theta-type structure that obstructs a standard theta-function reduction of the residual total-spin sum.
The phase diagram of the Heisenberg ferromagnetic model in the presence of a magnetic random field (we have used bimodal distribution) of spin S=1/2 (quantum case) and $S=\infty $ (classical case) on a simple cubic lattice is studied within the framework of the effective-field theory in finite cluster (we have chosen N=2 spins). Integrating out the part of order parameter (equation of state), we obtained an effective Landau expansion for the free energy written in terms of the order parameter Ψ(m)Ψ(m)Ψ(m). Using Maxwell construction we have obtained the phase diagram in the T−HT-HT−H plane for all interval of field. The first-order transition temperature is calculated by the discontinuity of the magnetization at Tc∗(H)T_{c}^{\ast}(H)Tc∗​(H), on the other hand in the continuous transition the magnetization is null at T=Tc(H)T=T_{c}(H)T=Tc​(H). At null temperature (T=0) we have found the \textbf{coexistence} field Hc=3.23JH_{c}=3.23JHc​=3.23J that is independent of spin value. The transition temperature Tc(H)T_{c}(H)Tc​(H) for the classical case ($S=\infty $), in the T−HT-HT−H plane, is larger than the quantum case (S=1/2).