Alkaline-earth-metal-like atoms with ultranarrow transitions open the door to a new regime of cavity quantum electrodynamics. That regime is characterized by a critical photon number that is many orders of magnitude smaller than what can be achieved in conventional systems. We show that it is possible to achieve superradiance in steady state with such systems. We discuss the basic underlying mechanisms as well as the key experimental requirements.
Alkaline-earth-metal-like atoms with ultranarrow transitions open the door to a new regime of cavity quantum electrodynamics. That regime is characterized by a critical photon number that is many orders of magnitude smaller than what can be achieved in conventional systems. We show that it is possible to achieve superradiance in steady state with such systems. We discuss the basic underlying mechanisms as well as the key experimental requirements.
A superradiant laser, which exploits the clock transition of alkaline-earth-metal-like atoms to generate ultrastable light in the bad-cavity limit, has garnered much attention in the past few decades. Unlike their odd counterpart, the even isotopes of alkaline-earth-metal-like atoms possess simpler structures and longer-lived transitions, which would relax the field control requirements and enhance the frequency stability of the output light. However, due to the absence of hyperfine interaction in even isotopes, the transition from the state 3 P 0 to 1 S 0 is strictly forbidden, leading to a vanishing coupling strength between the cavity mode and the atoms (the state 3 P 0 as a dark state). In this work, we suggest a superradiant laser scheme by dressing this dark state with a small bright component by virtue of a static magnetic field. In contrast to other proposals utilizing natural atomic transitions, our dressed-state protocol can work from the crossover regime (coherence in both atoms and photons) to the superradiant lasing regime (coherence solely in atoms). Specifically, by operating deep into the superradiant lasing regime, our scheme witnesses a dramatic line-narrowing feature (mHz level) while maintaining its power. Furthermore, compared to the crossover regime, the laser frequency in the superradiant lasing regime is more robust against the fluctuations of the cavity length and magnetic field strength. Our proposal demonstrates the potential for extracting ultranarrow light from even isotopes of the alkaline-earth-metal-like atoms and may find its role in frequency stabilization and related precision measurement scenarios.
A new class of laser, which harnesses coherence in both light and atoms, is possible with ultracold alkaline-earth-metal atoms trapped in an optical lattice inside an optical cavity. Different lasing regimes, including superradiance, superradiant, and conventional lasing, are distinguished by the relative coherence stored in the atoms and in the cavity mode. We analyze the physics in two different experimentally achievable regions of the superradiant lasing regime. Our calculations confirm the narrow linewidth of superradiant lasing for the doubly forbidden clock transition ${}^{3}{P}_{0}\ensuremath{\rightarrow}{}^{1}{S}_{0}$ of 87Sr atoms. Under strong driving of the dipole-forbidden transition ${}^{3}{P}_{1}\ensuremath{\rightarrow}{}^{1}{S}_{0}$ of 88Sr atoms, the superradiant linewidth narrows further due to the coherent excitation of the cavity field.
A steady-state superradiant laser can be used to generate ultranarrow-linewidth light, and thus has important applications in the fields of quantum information and precision metrology. However, the light produced by such a laser is still essentially classical. Here, we show that the introduction of a Rydberg medium into a cavity containing atoms with a narrow optical transition can lead to the steady-state superradiant emission of ultranarrow-linewidth nonclassical light. The cavity nonlinearity induced by the Rydberg medium strongly modifies the superradiance threshold, and leads to a Mollow triplet in the cavity output spectrum−this behavior can be understood as an unusual analogue of resonance fluorescence. The cavity output spectrum has an extremely sharp central peak, with a linewidth that can be far narrower than that of a classical superradiant laser. This unprecedented spectral sharpness, together with the nonclassical nature of the light, could lead to new applications in which spectrally pure quantum light is desired.
In this thesis, I describe the theoretical development of the superradiant laser, or laser in the extreme bad-cavity regime. In this regime, the cavity decay rate is much greater than the atomic dynamics. The atoms emit photons into the cavity mode superradiantly in steady state. We develop group-theoretic methods that enable us to exactly solve mesoscopic systems with hundreds of atoms. We demonstrate the synchronization of atomic dipoles in steady-state superradiance. With this synchronized system, we propose conditional Ramsey spectroscopy which allows us to observe Ramsey fringes indefinitely, even in the presence of atomic decoherence. Furthermore, we explore manifestations of synchronization in the quantum realm with two superradiant atomic ensembles. We show that two such ensembles exhibit a dynamical phase transition from two disparate oscillators to quantum phase-locked dynamics. Finally, we study the mechanical eect of the light-atom interaction in the steady-state superradiance. We find efficient many-body cooling of atoms. The work described in this thesis lays the theoretical foundation for the superradiant laser and for a potential future of active optical frequency standards.
Achieving superradiant lasing with an ultranarrow linewidth is crucial for enhancing atomic clock stability in quantum precision measurement. By employing the exceptional point (EP) property of the system, we demonstrate theoretically superradiant lasing with linewidths in the μHz range, sustained at the high-power level. This is achieved by incoherently pumping optical lattice clock transitions with ultracold alkaline-earth strontium-87 atoms in the EP of a PT-symmetric system. Physically, the atomic coherence reaches a maximum in the EP, significantly amplifying the superradiance effect and resulting in superradiant lasing with an ultranarrow linewidth. This linewidth is even three orders of magnitude smaller than that of superradiant lasing in the systems without EP. Our work extends the realm of superradiant lasing by introducing the EP property, and offers promising applications for developing atomic clocks with exceptional stability and accuracy.
In inverted atomic ensembles, photon-mediated interactions give rise to Dicke superradiance, a form of many-body decay that results in a rapid release of energy as a photon burst. While originally studied in pointlike ensembles, this phenomenon persists in extended ordered systems if the interparticle distance is below a certain bound. Here, we investigate Dicke superradiance in a realistic experimental setting using ordered arrays of alkaline-earth(-like) atoms, such as strontium and ytterbium. Such atoms offer exciting new opportunities for light-matter interactions, as their internal structure allows for trapping at short interatomic distances compared to their long-wavelength transitions, providing the potential for collectively enhanced dissipative interactions. Despite their intricate electronic structure, we show that two-dimensional arrays of these atomic species should exhibit many-body superradiance for achievable lattice constants. Moreover, superradiance effectively “closes” transitions, such that multilevel atoms become more two-level like. This occurs because the avalanchelike decay funnels the emission of most photons into the dominant transition, overcoming the single-atom decay ratios dictated by their fine structure and Zeeman branching. Our work represents an important step in harnessing alkaline-earth atoms as quantum optical sources and as platforms to explore many-body dissipative dynamics. Published by the American Physical Society 2024