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arXiv:0911.5165 · Physical Review B

Functional renormalization group study of the interacting resonant level model in and out of equilibrium

Christoph Karrasch, Mikhail Pletyukhov, L. Borda, V. Meden

Published Mar 24, 2010• 70 citations
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Abstract

We investigate equilibrium and steady-state nonequilibrium transport properties of a spinless resonant level locally coupled to two conduction bands of width $\ensuremath{\sim}\ensuremath{\Gamma}$ via a Coulomb interaction $U$ and a hybridization ${t}^{\ensuremath{'}}$. In order to study the effects of finite bias voltages beyond linear response, a generalization of the functional renormalization group to Keldysh frequency space is employed. Being mostly unexplored in the context of quantum impurity systems out of equilibrium, we benchmark this method against recently published time-dependent density matrix renormalization group data. We thoroughly investigate the scaling limit $\ensuremath{\Gamma}\ensuremath{\rightarrow}\ensuremath{\infty}$ characterized by the appearance of power laws. Most importantly, at the particle-hole symmetric point the steady-state current decays like $J\ensuremath{\sim}{V}^{\ensuremath{-}{\ensuremath{\alpha}}_{J}}$ as a function of the bias voltage $V⪢{t}^{\ensuremath{'}}$, with an exponent ${\ensuremath{\alpha}}_{J}(U)$ that we calculate to leading order in the Coulomb interaction strength. In contrast, we do not observe a pure power-law (but more complex) current-voltage-relation if the energy $ϵ$ of the resonant level is pinned close to either one of the chemical potentials $\ifmmode\pm\else\textpm\fi{}V/2$.

DOI
10.1103/physrevb.81.125122

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We investigate equilibrium and steady-state nonequilibrium transport properties of a spinless resonant level locally coupled to two conduction bands of width \ensuremath∼\ensuremathΓ\ensuremath{\sim}\ensuremath{\Gamma}\ensuremath∼\ensuremathΓ via a Coulomb interaction UUU and a hybridization t\ensuremath′{t}^{\ensuremath{'}}t\ensuremath′. In order to study the effects of finite bias voltages beyond linear response, a generalization of the functional renormalization group to Keldysh frequency space is employed. Being mostly unexplored in the context of quantum impurity systems out of equilibrium, we benchmark this method against recently published time-dependent density matrix renormalization group data. We thoroughly investigate the scaling limit \ensuremathΓ\ensuremath→\ensuremath∞\ensuremath{\Gamma}\ensuremath{\rightarrow}\ensuremath{\infty}\ensuremathΓ\ensuremath→\ensuremath∞ characterized by the appearance of power laws. Most importantly, at the particle-hole symmetric point the steady-state current decays like J\ensuremath∼V\ensuremath−\ensuremathαJJ\ensuremath{\sim}{V}^{\ensuremath{-}{\ensuremath{\alpha}}_{J}}J\ensuremath∼V\ensuremath−\ensuremathαJ​ as a function of the bias voltage V⪢t\ensuremath′V⪢{t}^{\ensuremath{'}}V⪢t\ensuremath′, with an exponent \ensuremathαJ(U){\ensuremath{\alpha}}_{J}(U)\ensuremathαJ​(U) that we calculate to leading order in the Coulomb interaction strength. In contrast, we do not observe a pure power-law (but more complex) current-voltage-relation if the energy ϵϵϵ of the resonant level is pinned close to either one of the chemical potentials \ifmmode±\else\textpm\fiV/2\ifmmode\pm\else\textpm\fi{}V/2\ifmmode±\else\textpm\fiV/2.
Using a real-time renormalization group method we study the minimal model of a quantum dot dominated by charge fluctuations, the two-lead interacting resonant level model, at finite bias voltage. We develop a set of RG equations to treat the case of weak and strong charge fluctuations, together with the determination of power-law exponents up to second order in the Coulomb interaction. We derive analytic expressions for the charge susceptibility, the steady-state current, and the conductance in the situation of arbitrary system parameters, in particular away from the particle-hole symmetric point and for asymmetric Coulomb interactions. In the asymmetric situation we find that power laws can be observed for the current only as a function of the level position (gate voltage) but in general not as a function of the voltage except for extremely large voltages. Furthermore, we study the quench dynamics after sudden switch-on of the level-lead couplings. The time evolution of the dot occupation and current is governed by exponential relaxation accompanied by voltage-dependent oscillations and characteristic algebraic decay.
The resonant-level model represents a paradigmatic quantum system which serves as a basis for many other quantum impurity models. We provide a comprehensive analysis of the nonequilibrium transport near a quantum phase transition in a spinless dissipative resonant-level model, extending earlier work [Phys. Rev. Lett 102, 216803 (2009)]. A detailed derivation of a rigorous mapping of our system onto an effective Kondo model is presented. A controlled energy-dependent renormalization-group approach is applied to compute the nonequilibrium current in the presence of a finite bias voltage VVV. In the linear-response regime $V\ensuremath{\rightarrow}0$, the system exhibits as a function of the dissipative strength a localized-delocalized quantum transition of the Kosterlitz-Thouless (KT) type. We address fundamental issues of the nonequilibrium transport near the quantum phase transition: Does the bias voltage play the same role as temperature to smear out the transition? What is the scaling of the nonequilibrium conductance near the transition? At finite temperatures, we show that the conductance follows the equilibrium scaling for V<TV<TV<T, while it obeys a distinct nonequilibrium profile for V>TV>TV>T. We furthermore provide different signatures of the transition in the finite-frequency current noise and ac conductance via a recently developed functional renormalization group (FRG) approach. The generalization of our analysis to nonequilibrium transport through a resonant level coupled to two chiral Luttinger liquid leads, generated by fractional quantum Hall edge states, is discussed. Our work on the dissipative resonant level has direct relevance to experiments on a quantum dot coupled to a resistive environment, such as H. Mebrahtu et al., [Nature (London) 488, 61 (2012)].
We investigate nonequilibrium properties of the single-impurity Anderson model by means of the functional renormalization group (fRG) within Keldysh formalism. We present how the level broadening $\ensuremath{\Gamma}/2$ can be used as flow parameter for the fRG. This choice preserves important aspects of the Fermi-liquid behavior that the model exhibits in case of particle-hole symmetry. An approximation scheme for the Keldysh fRG is developed which accounts for the frequency dependence of the two-particle vertex in a way similar but not equivalent to a recently published approximation to the equilibrium Matsubara fRG. Our method turns out to be a flexible tool for the study of weak to intermediate on-site interactions $U\ensuremath{\lesssim}3\ensuremath{\Gamma}$. In equilibrium we find excellent agreement with numerical RG results for the linear conductance at finite gate voltage, magnetic field, and temperature. In nonequilibrium, our results for the current agree well with time-dependent density-matrix RG. For the nonlinear conductance as function of the bias voltage, we propose reliable results at finite magnetic field and finite temperature. Furthermore, we demonstrate the exponentially small scale of the Kondo temperature to appear in the second-order derivative of the self-energy. We show that the approximation is, however, not able to reproduce the scaling of the effective mass at large interactions.
We study the nonlinear steady-state transport of spinless fermions through a quantum dot with a local two-particle interaction. The dot degree of freedom is in addition coupled to a phonon mode. This setup combines the non-equilibrium physics of the interacting resonant level model and that of the Anderson-Holstein model. The fermion-fermion interaction defies a perturbative treatment. We mainly focus on the antiadiabatic limit, with the phonon frequency being larger than the lead-dot tunneling rate. In this regime also the fermion-boson coupling cannot be treated perturbatively. Our goal is two fold. We investigate the competing roles of the fermion-fermion and fermion-boson interactions on the emergent low-energy scale TK{T}_{\mathrm{K}}TK​ and show how TK{T}_{\mathrm{K}}TK​ manifests in the transport coefficients as well as the current-voltage characteristics. For small to intermediate interactions, the latter is in addition directly affected by both interactions independently. With increasing fermion-boson interaction the Franck-Condon blockade suppresses the current at small voltages and the emission of phonons leads to shoulders or steps at multiples of the phonon frequency, while the local fermion-fermion interaction implies a negative differential conductance at voltages larger than TK{T}_{\mathrm{K}}TK​. We, in addition, use the model to investigate the limitations of our low-order truncated functional renormalization group approach on the Keldysh contour. In particular, we quantify the role of the broken current conservation.
We study transport properties of quantum impurity systems using the functional renormalization group. The latter is an RG-based diagrammatic tool to treat Coulomb interactions in a fast and flexible way. Prior applications, which employed a simple first-order (Hartree-Fock-like) scheme to truncate the FRG flow equations within the Matsubara formalism, succeeded in accurately describing linear transport of various quantum dot geometries at zero temperature T=0. In a nutshell, advance in this Thesis is three-fold. First, we introduce a frequency-dependent second-order approximation in order to eventually compute finite-energy properties such as the conductance at T>0 (mainly focusing on the single impurity Anderson model). Second, a generalisation of the Hartree-Fock-like approach to Keldysh space allows for addressing the non-equilibrium steady-state dynamics of the interacting resonant level model. Third, we investigate the physics of a quantum dot Josephson junction as well as the charging of a single narrow level using the first-order scheme.
We develop a low-order conserving approximation for the interacting resonant-level model (IRLM), and apply it to (i) thermal equilibrium, (ii) nonequilibrium steady state, and (iii) nonequilibrium quench dynamics. Thermal equilibrium is first used to carefully gauge the quality of the approximation by comparing the results with other well-studied methods, and finding good agreement for small values of the interaction. We analytically show that the power-law exponent of the renormalized level width usually derived using renormalization group approaches can also be correctly obtained in our approach in the weak interaction limit. A closed expression for the nonequilibrium steady-state current is derived and analytically and numerically evaluated. We find a negative differential conductance at large voltages, and the exponent of the power-law suppression of the steady-state current is calculated analytically at zero temperature. The response of the system to quenches is investigated for a single lead as well as for two-lead setup at finite voltage bias at particle-hole symmetry using a self-consistent two-times Keldysh Green function approach, and results are presented for the time-dependent current for different bias and contact interaction strength.