We study theoretically a ring of three quantum dots mutually coupled by antiferromagnetic exchange interactions and tunnel-coupled to two metallic leads: the simplest model in which the consequences of local frustration arising from internal degrees of freedom may be studied within a two-channel environment. Two-channel Kondo (2CK) physics is found to predominate at low energies in the mirror-symmetric models considered, with a residual spin-$\frac{1}{2}$ overscreened by coupling to both leads. It is however shown that two distinct 2CK phases, with different ground-state parities, arise on tuning the interdot exchange couplings. In consequence a frustration-induced quantum phase transition occurs, the 2CK phases being separated by a quantum critical point for which an effective low-energy model is derived. Precisely at the transition, parity mixing of the quasidegenerate local trimer states acts to destabilize the 2CK fixed points; and the critical fixed point is shown to consist of a free pseudospin together with effective one-channel spin quenching, itself reflecting underlying channel anisotropy in the inherently two-channel system. Numerical renormalization group techniques and physical arguments are used to obtain a detailed understanding of the problem, including study of both thermodynamic and dynamical properties of the system.
We study theoretically a ring of three quantum dots mutually coupled by antiferromagnetic exchange interactions and tunnel-coupled to two metallic leads: the simplest model in which the consequences of local frustration arising from internal degrees of freedom may be studied within a two-channel environment. Two-channel Kondo (2CK) physics is found to predominate at low energies in the mirror-symmetric models considered, with a residual spin-21 overscreened by coupling to both leads. It is however shown that two distinct 2CK phases, with different ground-state parities, arise on tuning the interdot exchange couplings. In consequence a frustration-induced quantum phase transition occurs, the 2CK phases being separated by a quantum critical point for which an effective low-energy model is derived. Precisely at the transition, parity mixing of the quasidegenerate local trimer states acts to destabilize the 2CK fixed points; and the critical fixed point is shown to consist of a free pseudospin together with effective one-channel spin quenching, itself reflecting underlying channel anisotropy in the inherently two-channel system. Numerical renormalization group techniques and physical arguments are used to obtain a detailed understanding of the problem, including study of both thermodynamic and dynamical properties of the system.
We investigate systems comprising chains and rings of quantum dots, coupled to two metallic leads. Such systems allow to study the competition between orbital and spin degrees of freedom in a nanodevice, and the effect this subtle interplay has on two-channel Kondo (2CK) physics. We demonstrate that a rich range of strongly correlated electron behaviour results, with non-Fermi liquid 2CK phases and non-trivial phase transitions accessible. We employ physical arguments and the numerical renormalization group (NRG) technique to analyse these systems in detail, examining in particular both thermodynamic and dynamical properties. When leads are coupled to either end of a chain of dots, we show that the resulting behaviour on low temperature/energy scales can be understood in terms of simpler paradigmatic quantum `impurity' models. An effective low-energy single-spin 2CK model is derived for all odd-length chains, while the behaviour of even-length chains is related fundamentally to that of the classic `two-impurity Kondo' model. In particular, for small interdot coupling, we show that an effective coupling mediated though incipient single-channel Kondo states drives all odd chains to the 2CK fixed point (FP) on the lowest temperature/energy scales. A theory is also developed to describe a phase transition in even chains. We derive an effective channel-anisotropic 2CK model, which indicates that the critical FP of such models must be the 2CK FP. This physical picture is confirmed using NRG for various chain systems. We also examine the effect of local frustration on 2CK physics in mirror-symmetric ring systems. The importance of geometry and symmetry is demonstrated clearly in the markedly different physical behaviour that arises in systems where two leads are either connected to the same dot, or to neighbouring dots. In the latter case, we show for all odd-membered rings that two distinct 2CK phases, with different ground state parities, arise on tuning the interdot couplings. A frustration-induced phase transition thus occurs, the 2CK phases being separated by a novel critical point for which an effective low-energy model is derived. Precisely at the transition, parity mixing of the quasidegenerate local trimer states acts to destabilise the 2CK FPs, and the critical FP is shown to consist of a free pseudospin together with effective single-channel spin quenching. While connecting both leads to the same dot again results in two parity-distinct phases, a simple level-crossing transition now results due to the symmetry of the setup. The proposed geometry also allows access to a novel ferromagnetically-coupled two-channel local moment phase. Driven by varying the interdot couplings and occurring at the point of inherent magnetic frustration, such transitions in ring structures provide a striking example of the subtle interplay between internal spin and orbital degrees of freedom in coupled quantum dot systems, and the resulting effect on Kondo physics.
We investigate theoretically the possibility of observing two-channel Kondo (2CK) physics in tunnel-coupled double quantum dots (TCDQDs), at both zero and finite magnetic fields; taking the two-impurity Anderson model as the basic TCDQD model, together with effective low-energy models arising from it by Schrieffer-Wolff transformations to second and third order in the tunnel couplings. The models are studied primarily using Wilson's numerical renormalization group. At zero field our basic conclusion is that while 2CK physics arises in principle provided the system is sufficiently strongly correlated, the temperature window over which it could be observed is much lower than is experimentally feasible. This finding disagrees with recent work on the problem, and we explain why. At finite field, we show that the quantum phase transition known to arise at zero field in the two-impurity Kondo model, with an essentially 2CK quantum critical point, persists at finite fields. This raises the prospect of access to 2CK physics by tuning a magnetic field, although preliminary investigation suggests this to be even less feasible than at zero field.
We investigate a system of three tunnel-coupled semiconductor quantum dots in a triangular geometry, one of which is connected to a metallic lead, in the regime where each dot is essentially singly occupied. Both ferromagnetic and antiferromagnetic spin-21 Kondo regimes, separated by a quantum phase transition, are shown to arise on tuning the interdot tunnel couplings and should be accessible experimentally. Even in the ferromagnetically-coupled local moment phase, the Kondo effect emerges in the vicinity of the transition at finite temperatures. Physical arguments and numerical renormalization group techniques are used to obtain a detailed understanding of the problem.
We investigate theoretically the quantum phase transition (QPT) between the one-channel Kondo (1CK) and two-channel Kondo (2CK) fixed points in a quantum dot coupled to helical edge states of interacting 2D topological insulators (2DTI) with Luttinger parameter 0 < K < 1 . The model was studied by Law et al (2010 Phys. Rev. B 81 041305(R) ), and was mapped onto an anisotropic two-channel Kondo model via bosonization. For K < 1 , the strong coupling 2CK fixed point was argued to be stable for infinitesimally weak tunnelings between the dot and the 2DTI based on a simple scaling dimensional analysis (Law et al 2010 Phys. Rev. B 81 041305(R) . We re-examine this model beyond the bare scaling dimension analysis via a one-loop renormalization group (RG) approach combined with bosonization and re-fermionization techniques near weak-coupling and strong-coupling (2CK) fixed points. We find for a fixed value of K < 1 that the 2CK fixed point can be unstable towards the 1CK fixed point and the system is expected to undergo a quantum phase transition between 1CK and 2CK fixed points with changing Kondo couplings. Our RG approach is controlled near K = 1. In general, this QPT can also occur upon tuning the Luttinger parameter K to a critical value K c smaller than unity ( 0 < K c < 1 ) for fixed Konodo couplings. The QPT in our model comes as a result of the combined Kondo and the helical Luttinger physics in 2DTI, and it serves as the first example of the 1CK-2CK QPT that is accessible by the controlled RG approach. We extract quantum critical and crossover behaviors from various thermodynamical quantities near the transition. Our results are robust against particle-hole asymmetry for 1 2 < K < 1 .
The two-channel Kondo (2CK) effect with its exotic ground state properties has remained difficult to realize in physical systems. At low energies, a quantum impurity with orbital degree of freedom, like a proton bound in an interstitial lattice space, comprises a 3-level system with a unique ground state and (at least) doubly degenerate rotational excitations with excitation energy Delta0. When immersed in a metal, electronic angular momentum scattering induces transitions between any two of these levels (couplings J), while the electron spin is conserved. We show by extensive numerical renormalization group (NRG) calculations that without fine-tuning of parameters this system exhibits a 2CK fixed point, due to Kondo correlations in the excited-state doublet whose degeneracy is stabilized by the host lattice parity, while the channel symmetry (electron spin) is guaranteed by time reversal symmetry. We find a pronounced plateau in the entropy at S(TK<T<Delta0)=kBln2 between the high-T value, S(TggDelta0)=kBln3, and the 2CK ground state value, S(0)=kBlnsqrt2. This indicates a downward renormalization of the doublet below the non-interacting ground state, thus realizing the 2CK fixed point, in agreement with earlier conjectures. We mapped out the phase diagram of the model in the J−Delta0 plane. The Kondo temperature TK shows non-monotonic J-dependence, characteristic for 2CK systems.newline indent Beside the two-channel Kondo effect of the model, we also study the single-channel version, which is realized by applying a strong magnetic field to the conduction band electrons so that their degeneracy is lifted and consequently having only one kind of electrons scattering off the impurity. This single-channel case is easier to analyze since the Hilbert space is not as large as that of the 2CK. We equally find a downward renormalization of the excited state energy by the Kondo correlations in the SU(2) doublet. In a wide range of parameter values this stabilizes the single-channel Kondo fixed point and a phase diagram is also mapped out for the model. In the single-channel version a plateau is found in the entropy at S(TK<T<Delta0)=kBln2 between high-T value, S(TggDelta0)=kBln3, and the single-channel Kondo ground state value, S(0)=kBln1.
We study the low-temperature physics arising in models of a strongly correlated, tunnel-coupled double quantum dot (DQD), particularly the two-impurity Anderson model (2AIM) and the two-impurity Kondo model (2IKM), employing a combination of physical arguments and the Numerical Renormalisation Group. These models exhibit a rich range of Kondo physics. In the regime with essentially one electron on each dot, there is a competition between the Kondo effect and the interdot exchange interaction. This competition gives rise to a quantum phase transition (QPT) between local singlet and Kondo singlet phases in the 2IKM, which becomes a continuous crossover in the 2AIM as a result of the interlead charge transfer present. The 2IKM is known to exhibit two-channel Kondo (2CK) physics at the QPT, and we investigate whether this is also the case for the 2AIM at the crossover. We find that while in principle 2CK physics can be observed in the 2AIM, extremely low temperatures are required, such that it is unlikely that 2CK physics will be observed in an experimental DQD system in the near future. We have studied the effect of a magnetic field on the 2AIM and the 2IKM, finding that both the zero-field QPT in the 2IKM and the zero-field crossover in the 2AIM, persist to finite field. This presents the possibility of observing 2CK physics in an experimental DQD at finite field, but we find that the temperatures required to do so are extremely low. We show that longer even-numbered chains of spins also exhibit QPTs at finite field, and argue that a 2N-spin chain should undergo N QPTs as field is increased (starting deep in the local singlet phase at zero field). We have also carried out a joint theoretical-experimental study of a carbon nanotube based DQD, in collaboration with Dr. Mark Buitelaar et al. The agreement between experimental and theoretical results is good, and the experiments are able to access the crossover present in the 2AIM at finite field. Furthermore, the experiments show the wide range of physics exhibited by DQD systems, and illustrate the utility of such systems in probing correlated electron physics.